Publications by authors named "Francesc Salvat-Pujol"

Scanning electron microscopy (SEM) is a practical tool to determine the dimensions of nanometer-scale features. Conventional width measurements use arbitrary criteria, e.g.

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The aim of the present overview article is to raise awareness of an essential aspect that is usually not accounted for in the modelling of electron transport for focused-electron-beam-induced deposition (FEBID) of nanostructures: Surface excitations are on the one hand responsible for a sizeable fraction of the intensity in reflection-electron-energy-loss spectra for primary electron energies of up to a few kiloelectronvolts and, on the other hand, they play a key role in the emission of secondary electrons from solids, regardless of the primary energy. In this overview work we present a general perspective of recent works on the subject of surface excitations and on low-energy electron transport, highlighting the most relevant aspects for the modelling of electron transport in FEBID simulations.

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Dramatic volume collapses under pressure are fundamental to geochemistry and of increasing importance to fields as diverse as hydrogen storage and high-temperature superconductivity. In transition metal materials, collapses are usually driven by so-called spin-state transitions, the interplay between the single-ion crystal field and the size of the magnetic moment. Here we show that the classical S = 5/2 mineral hauerite (MnS2) undergoes an unprecedented (ΔV ~ 22%) collapse driven by a conceptually different magnetic mechanism.

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We present a numerical investigation of energy and charge distributions during electron-beam-induced growth of tungsten nanostructures on SiO2 substrates by using a Monte Carlo simulation of the electron transport. This study gives a quantitative insight into the deposition of energy and charge in the substrate and in the already existing metallic nanostructures in the presence of the electron beam. We analyze electron trajectories, inelastic mean free paths, and the distribution of backscattered electrons in different compositions and at different depths of the deposit.

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Supersurface electron scattering, i.e., electron energy losses and associated deflections in vacuum above the surface of a medium, is shown to contribute significantly to electron spectra.

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We present a numerical study of the zero-temperature response of the Gaussian random-field Ising model to a slowly varying external field, allowing the system to be trapped in microscopic configurations that are not fully metastable. This modification of the standard single-spin-flip dynamics results in an increase in dissipation (hysteresis) somewhat similar to that observed with a finite driving rate. We then study the distribution of avalanches along the hysteresis loop and perform a finite-size scaling analysis that shows good evidence that the critical exponents associated to the disorder-induced phase transition are not modified.

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