Field emission of electrons generated by the near field of strongly coupled plasmons.

Field emission of electrons is generated solely by the ultrastrong near-field of strongly coupled plasmons without the help of a noticeable dc field. Strongly coupled plasmons are excited at Au nanoparticles in subnanometer distance to a Au film by femtosecond laser pulses. Field-emitted electrons from individual nanoparticles are detected by means of photoelectron emission microscopy and spectroscopy.

Near field of strongly coupled plasmons: uncovering dark modes.

Strongly coupled plasmons in a system of individual gold nanoparticles placed at subnanometer distance to a gold film (nanoparticle-on-plane, NPOP) are investigated using two complementary single particle spectroscopy techniques. Optical scattering spectroscopy exclusively detects plasmon modes that couple to the far field via their dipole moment (bright modes). By using photoemission electron microscopy (PEEM), we detect in the identical NPOPs near-field modes that do not couple to the scattered far field (dark modes) and are characterized by a strongly enhanced nonlinear electron emission process.