The final disposal of NORM wastes in conventional landfill generally determines problems of acceptance by the landfill operators, since their willingness to accept Naturally Occurring Radioactive Material (NORM) is often limited due to their concern about the radiological risks and reluctance of the local community to have at local landfills material that despite being cleared is still perceived as 'radioactive'. In order to raise awareness among landfill operators, and also among other stakeholders on the actual radiological risk of exempted or cleared NORM wastes, it is of interest to estimate the mass of annual wastes containing NORM that can be disposed of in a landfill for conventional waste complying with the annual dose criterion of 1 mSv. A methodology was developed considering a hypothetical homogeneous large landfill and assuming that NORM wastes are delivered with an initial activity concentration of 1 kBq kg.
View Article and Find Full Text PDFBackground: In a context of environmental monitoring around installations related to the nuclear fuel cycle, the Diffusive Gradient in Thin-films (DGT) technique captures the integrated concentration of U isotopes in their native environment, yielding comprehensive data on U origin (anthropogenic vs natural), total concentration, and mobility. However, for common deployment times (4-5 days) in moderately basic waters, none of the commercially available binding gels is adapted to measure the total U concentration. So, the development of novel DGT binding gels is timely.
View Article and Find Full Text PDFNaturally occurring radioactive materials (NORM) are present worldwide and under certain circumstances (e.g., human activities) may give radiation exposure to workers, local public or occasional visitors and non-human biota (NHB) of the surrounding ecosystems.
View Article and Find Full Text PDFAluminum (Al) is a major limiting factor for crop production on acidic soils, inhibiting root growth and plant development. At acidic pH (pH < 5.5), Al ions are the main form of Al present in the media.
View Article and Find Full Text PDFJ Environ Radioact
March 2022
Cs is one of the most persistent radioactive contaminants in soil after a nuclear accident. It can be taken up by plants and enter the human food chain generating a potential human health hazard. Although a large amount of literature has highlighted the role of the different processes involved in Cs uptake by plants, there is still no simple way to predict its transfer for a specific plant from a particular soil.
View Article and Find Full Text PDFDue to mining activities, concentration of uranium (U) in the environment nearby former and operating sites can be higher than in other areas. The derivation of quality criteria for U in freshwater ecosystems, rivers and lakes includes the consideration of contaminated sediments and the associated risk to the benthic life. Therefore, the derivation of a quality criteria for sediment has been viewed as a logical and necessary extension of the work already done to establish water quality criteria.
View Article and Find Full Text PDFUranium is a naturally occurring radionuclide. Its redistribution, primarily due to human activities, can have adverse effects on human and non-human biota, which poses environmental concerns. The molecular mechanisms of uranium tolerance and the cellular response induced by uranium exposure in bacteria are not yet fully understood.
View Article and Find Full Text PDFFor the first time, Diffusive Gradient in Thin-films (DGT) focuses on the inorganic iodine species iodate (IO) and iodide (I). A silver-doped Cl resin (AgdCl), which is known to selectively accumulate I, was used to make a binding gel. Laboratory investigations were designed to verify the suitability of the AgdCl-DGT method to measure the total I concentration in environmental waters.
View Article and Find Full Text PDFActinide-based mineral phases occurring in contaminated soils can be solubilized by organic chelators excreted by plants, such as citrate. Herein, the efficiency of citrate towards U and Pu extraction is compared to that of siderophores, whose primary function is the acquisition of iron(III) as an essential nutrient and growth factor for many soil microorganisms. To that end, we selected desferrioxamine B (DFB) as an emblematic bacterial trishydroxamic siderophore and a synthetic analog, abbreviated (L)H, of the tetradentate rhodotorulic acid (RA) produced by yeasts.
View Article and Find Full Text PDFJ Environ Radioact
September 2021
The aim of this paper is to assess the suitability of DGT to extract kinetic rates of desorption of cesium (Cs) from soils. For this purpose, laboratory experiments with a natural soil spiked with Cs were carried out under three different contamination conditions, reflecting either an increase in Cs contamination level or an ageing of the contamination within the soil. The experimental results, i.
View Article and Find Full Text PDFSci Total Environ
November 2019
This study aimed to determine uranium (U) pollution over time using otoliths as a marker of fish U contamination. Experiments were performed in field contamination (~20 μg L: encaged fish: 15d, 50d and collected wild fish) and in laboratory exposure conditions (20 and 250 μg L, 20d). We reported the U seasonal concentrations in field waterborne exposed roach fish (Rutilus rutilus), in organs and otoliths.
View Article and Find Full Text PDFThis study deals with further and systematic laboratory evaluation of the already known ammonium 12-molybdophosphate (AMP)-diffusive gradient in thin film (DGT) method, which is used for measuring total Cs concentration in environmental waters. This study confirms that the AMP-binding gel is not stable for pH > 6. In order to reveal a potential impact of AMP degradation on DGT application, time-series experiments were performed by deploying AMP-DGT samplers in Cs-doped moderately basic soft and hard water up to total AMP-binding gel degradation (60 and 175 h of deployment time, respectively).
View Article and Find Full Text PDFAfter the Chernobyl nuclear power plant accident in 1986, contaminated soils, vegetation from the Red Forest and other radioactive debris were buried within trenches. In this area, trench T22 has long been a pilot site for the study of radionuclide migration in soil. Here, we used 454 pyrosequencing of 16S rRNA genes to obtain a comprehensive view of the bacterial and archaeal diversity in soils collected inside and in the vicinity of the trench T22 and to investigate the impact of radioactive waste disposal on prokaryotic communities.
View Article and Find Full Text PDFActinides determination in urine samples is part of the analyses performed to monitor internal contamination in case of an accident or a terrorist attack involving nuclear matter. Mineralisation is the first step of any of these analyses. It aims at reducing the sample volume and at destroying all organic compounds present.
View Article and Find Full Text PDFAlthough uranium (U) is naturally found in the environment, soil remediation programs will become increasingly important in light of certain human activities. This work aimed to identify U(VI) detoxification mechanisms employed by a bacteria strain isolated from a Chernobyl soil sample, and to distinguish its active from passive mechanisms of interaction. The ability of the Microbacterium sp.
View Article and Find Full Text PDFJ Environ Radioact
January 2013
With intentions of integrating a portion of their respective research efforts into a trans-national programme that will enhance radioecology, eight European organisations recently formed the European Radioecology ALLIANCE (www.er-alliance.org).
View Article and Find Full Text PDFThis study investigated the influence of uranium on the indigenous bacterial community structure in natural soils with high uranium content. Radioactive soil samples exhibiting 0.26% - 25.
View Article and Find Full Text PDFIn a context of environmental risk assessment of nuclear (79)Se radionuclide, the impact of low Se-selenite concentrations (0.008 and 8 mg kg(-1)) on bacterial communities of two soils, a silty clay loam and a sandy soil, was investigated over a 6-month incubation time. This Se-selenite was partially labelled with (75)Se.
View Article and Find Full Text PDFThe aim of this study was to investigate the role of microorganisms on the behaviour of selenium in natural soil maintained under strictly aerobic conditions. Six-day batch experiments were performed with soils constrained to different microbiological states, either by sterilisation or by adding organic substrates. Selenium was added to the soil as selenite.
View Article and Find Full Text PDFIEEE Trans Pattern Anal Mach Intell
January 2008
We present a family of scale-invariant local shape features formed by chains of k connected, roughly straight contour segments (kAS), and their use for object class detection. kAS are able to cleanly encode pure fragments of an object boundary, without including nearby clutter. Moreover, they offer an attractive compromise between information content and repeatability, and encompass a wide variety of local shape structures.
View Article and Find Full Text PDFThe chemical and physical processes involved in the retention of 10(-2)M Zn, Pb and Cd in a calcareous medium were studied under saturated dynamic (column) and static (batch) conditions. Retention in columns decreased in order: Pb>>Cd approximately Zn. In the batch experiments, the same order was observed for a contact time of less than 40h and over, Pb>>Cd>Zn.
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