Leveraging almost hydrophobic PVDF membrane and in-situ ozonation in O/UF/BAC system for superior anti-fouling and rejection performance in drinking water treatment.

The almost hydrophobic PVDF membrane (PVDF matrix) commonly exhibited excellent performance in pollutant rejection but with poor anti-fouling performance. This study intended to develop the rejection performance and enhance anti-fouling of the PVDF membrane in an O/UF/BAC system for high quality water production through leveraging the advantages of in-situ ozonation and the nature of the PVDF membrane. Reduced density gradient (RDG) analysis demonstrated that the PVDF membrane exhibited excellent ozone resistance by reducing hydrogen bonds and electrostatic interactions between the membrane surface and ozone.

"Bamboo-like" strong and tough sodium alginate/polyacrylate hydrogel fiber with directional controlled release for wound healing promotion.

Skin, as the biggest organ and outermost surface of the human body, is prone to injury due to various challenges, especially the expanding potential of accidents, which bring a huge social and economic burden. Hydrogels are emerging as the most promising candidate for wound dressings, which not only fulfill the varied requirements of dressings but also serve as drug carriers. But limited breathability, rapid drug release, and inadequate mechanical properties remains a significant challenge.

A triple-crosslinking strategy for high-performance regenerated cellulose fibers derived from waste cotton textiles.

Regenerated cellulose fibers has attracted increasing attention for high-grade textile raw materials and industrial textiles, but the low mechanical property caused by differences in regenerated raw materials and production levels limits its commercial application in the product diversity. Herein, we proposed a novel triple-crosslinking strategy by coupling with hydrogen bonds, chemical crosslinking, and internal mineralization from multiple pulsed vapor phase infiltration (MPI) to improve the mechanical performance of regenerated cellulose fibers. A binary solvent composed of ionic liquid (IL) and dimethyl sulfoxide (DMSO) is used to dissolve waste cotton textile and then wet spinning.

Confined Water Dominates Ion/Molecule Transport in Hydrogel Nanochannels.

Current artificial nanochannels rely more on charge interactions for intelligent mass transport. Nevertheless, popular charged nanochannels would lose their advantages in long-term applications. Confined water, an indispensable transport medium in biological nanochannels, dominating the transport process in the uncharged nanochannels perfectly provides a new perspective.

Research on transformer fault diagnosis based on an IWHO optimized MS1DCNN algorithm and LIF spectrum.

Accurate diagnosis of transformer faults can effectively improve the enduring reliability of power grid operation. Aiming at overcoming the problems of long time consumption and low diagnostic rate in the past diagnosis methods, this article designs a laser-induced fluorescence (LIF) detection system, which can be combined with a multi-scale one-dimensional convolution neural network (MS1DCNN) to diagnose transformer fault categories. The structural parameters of MS1DCNN are optimized using the improved wild horse optimizer (IWHO).

Target Recognition of Coal and Gangue Based on Improved YOLOv5s and Spectral Technology.

Aiming at the problems of long detection time and low detection accuracy in the existing coal gangue recognition, this paper proposes a method to collect the multispectral images of coal gangue using spectral technology and match with the improved YOLOv5s (You Only Look Once Version-5s) neural network model to apply it to coal gangue target recognition and detection, which can effectively reduce the detection time and improve the detection accuracy and recognition effect of coal gangue. In order to take the coverage area, center point distance and aspect ratio into account at the same time, the improved YOLOv5s neural network replaces the original GIou Loss loss function with CIou Loss loss function. At the same time, DIou NMS replaces the original NMS, which can effectively detect overlapping targets and small targets.

Transformer fault diagnosis research based on LIF technology and IAO optimization of LightGBM.

Transformer fault diagnosis is a necessary operation to ensure the stable operation of a power system. In view of the problems of the low diagnostic rate and long time needed in traditional methods, such as the dissolved gas in oil method, a laser-induced fluorescence (LIF) spectral technology is proposed in this paper, which incorporated an improved aquila optimizer (IAO) and light gradient boosting machine (LightGBM), to predict the types of transformer faults. The original AO was improved using the Nelder Mead (NM) simple search method and opposition-based learning (OBL) mechanism, which could improve the parameter optimization ability of the model.

Chemi-Mechanically Peeling the Unstable Surface States of α-FAPbI.

Surface states are one of the crucial factors determining the phase stability of formamidinium-based perovskites. Compared with other compositions, exclusive lattice strain in FAPbI perovskite generates defects at the surface more readily, making them more vulnerable at the surface and easier to trigger the phase transition from α-phase to the non-perovskite δ-phase. In order to regulate the surface quality, here, a chemi-mechanical cleavage approach is reported, i.

Superdurable and fire-retardant structural coloration of carbon nanotubes.

Carbon nanotubes (CNTs) are promising candidates for numerous cutting-edge fields because of their excellent properties. However, the inherent black color of CNTs cannot satisfy the aesthetic/fashion requirement, and the flammability of CNTs severely restricts their application in high-temperature environments with oxygen. Here, we realized a structural coloration of CNTs by coating them with amorphous TiO layers.

A Facile Strategy To Construct Au@VO Nanoflowers as a Multicolor Electrochromic Material for Adaptive Camouflage.

Transition metal oxides (TMOs) are promising inorganic electrochromic materials (ECMs) that can be widely used in electronic displays and adaptive camouflage. However, there are still huge challenges for TMOs to simultaneously achieve multicolor transformation capability and good cycling stability. Herein, we assemble Au-modified (0.

Ultrasensitive Airflow Sensors Based on Suspended Carbon Nanotube Networks.

High-performance airflow sensors are in great demand in numerous fields but still face many challenges, such as slow response speed, low sensitivity, large detection threshold, and narrow sensing range. Carbon nanotubes (CNTs) exhibit many advantages in fabricating airflow sensors due to their nanoscale diameters, excellent mechanical and electrical properties, and so on. However, the intrinsic extraordinary properties of CNTs are not fully exhibited in previously reported CNT-based airflow sensors due to the mixed structures of macroscale CNT assemblies.

Fast In-Situ Optical Visualization of Carbon Nanotubes Assisted by Smoke.

The fast visualization and manipulation of individual carbon nanotubes (CNTs) has always been a significant technology for their fundamental research. Here, a fast and facile approach is proposed to realize the optical observation of individual suspended CNTs and CNT networks under conventional optical microscopes with the assistance of tar nanodroplets from smoke. The nanodroplets deposited on CNTs render them with strong light scattering to visible light, thus making the CNTs visible under optical microscopes.

Bio-inspired structural colors and their applications.

Structural colors, generated by the interaction of interference, diffraction, and scattering between incident light and periodic nanostructured surfaces with features of the same scale with incident visible light wavelengths, have recently attracted intense interest in a wide range of research fields, due to their advantages such as various brilliant colors, long-term stability and environmental friendliness, low energy consumption, and mysterious biological functions. Tremendous effort has been made to design structural colors and considerable progress has been achieved in the past few decades. However, there are still significant challenges and obstacles, such as durability, portability, compatibility, recyclability, mass production of structural-color materials, , that need to be solved by rational structural design and novel manufacturing strategies.

Discovery of new genetic loci for male sexual orientation in Han population.

Epidemiological studies have demonstrated that the genetic factors partly influence the development of same-sex sexual behavior, but most genetic studies have focused on people of primarily European ancestry, potentially missing important biological insights. Here, we performed a two-stage genome-wide association study (GWAS) with a total sample of 1478 homosexual males and 3313 heterosexual males in Han Chinese populations and identified two genetic loci (rs17320865, Xq27.3, FMR1NB, P = 8.

Light-driven directional ion transport for enhanced osmotic energy harvesting.

Light-driven ion (proton) transport is a crucial process both for photosynthesis of green plants and solar energy harvesting of some archaea. Here, we describe use of a TiO/CN semiconductor heterojunction nanotube membrane to realize similar light-driven directional ion transport performance to that of biological systems. This heterojunction system can be fabricated by two simple deposition steps.

Regulation of Hole Concentration and Mobility and First-Principle Analysis of Mg-Doping in InGaN Grown by MOCVD.

This work studied the regulation of hole concentration and mobility in p-InGaN layers grown by metalorganic chemical vapor deposition (MOCVD) under an N-rich environment. By adjusting the growth temperature, the hole concentration can be controlled between 6 × 10/cm and 3 × 10/cm with adjustable hole mobility from 3 to 16 cm/V.s.

Unparalleled Armour for Aramid Fiber with Excellent UV Resistance in Extreme Environment.

Aramid fibers are widely used in many cutting-edge fields, including space, aviation, military, and electronics. However, their poor UV resistance and surface inertness seriously hinder their utilization, especially in harsh environments. Here, a dual-layer ultrathin AlO-TiO coating with a thickness of 70-180 nm is fabricated on aramid fibers by a modified atomic layer deposition (ALD) method.

Feasibility of N Reduction on the V Anchored 1T-MoS Monolayer: A Density Functional Theory Study.

The front cover artwork is provided by the groups of Prof. BeiBei, Xiao and Lei, Yang (Jiangsu University of Science and Technology, China) as well as Dr. ErHong, Song (Shanghai Institute of Ceramics, Chinese Academy of Sciences, China).

Feasibility of N Reduction on the V Anchored 1T-MoS Monolayer: A Density Functional Theory Study.

Developing efficient electrocatalysts for nitrogen reduction reaction (NRR) at ambient conditions is crucial for NH synthesis. In this manuscript, the NRR performance of the transition metal anchored MoS monolayer with 1T atomic structure (1T-MoS ) is systematically evaluated by density functional theory computations. Our results reveal that the V decorated 1T-MoS exhibits the outstanding catalytic activity toward NRR via distal mechanism where the corresponding onset potential is 0.

Facile and Effective Fabrication of Highly UV-Resistant Silk Fabrics with Excellent Laundering Durability and Thermal and Chemical Stabilities.

As the most favored high-quality biopolymer, silk fiber is widely used in the textile and medical industries owing to its impressive mechanical properties, wear comfort properties, and biocompatibility. However, its photoinstability, chemical instability, and thermal instability seriously hinder its utilization in luxurious fashionable apparels. Therefore, we herein report the preparation of an ultrathin and uniform TiO-AlO cloth with a thickness of just six in a thousand of fiber on silkworm silk fiber via atomic layer deposition.

Exploring the ring-opening reactions of imidazo[1,5-a]quinolines for the synthesis of imides under photochemical conditions.

The ring-opening reaction of imidazo[1,5-a]quinolines under photoredox conditions has been described. With Eosin Y as the organophotoredox catalyst, synthetically useful and medicinally important imides were obtained in moderate to excellent yields under mild reaction conditions.

Overcoming diffusion-related limitations in semiconductor defect imaging with phonon-plasmon-coupled mode Raman scattering.

Carrier diffusion is of paramount importance in many semiconductor devices, such as solar cells, photodetectors, and power electronics. Structural defects prevent such devices from reaching their full performance potential. Although a large carrier diffusion length indicates high material quality, it also implies increased carrier depletion by an individual extended defect (for instance, a dislocation) and obscures the spatial resolution of neighboring defects using optical techniques.

Geometry modulation of ion diffusion through layered asymmetric graphene oxide membranes.

The asymmetric ion diffusion phenomenon through a 2D nanofluidic thickness gradient membrane under a concentration gradient is reported. The preferential direction for ion diffusion is from the thick side toward the thin side of the geometry-asymmetric graphene oxide membranes, which is attributed to the difference in charge selectivity.