Ferroelectric materials commonly serve as gate insulators in typical field-effect transistors, where their polarization reversal enables effective modulation of the conductivity state of the channel material, thereby realizing non-volatile memory. Currently, novel 2D ferroelectrics unlock new prospects in next-generation electronics and neuromorphic computation. However, the advancement of these materials is impeded by limited selectivity and narrow memory windows.
View Article and Find Full Text PDFThe design and fabrication of materials that can concurrently respond to light and gas within the dual-modal recognition domain present a significant challenge due to contradictory structural requirements. This innovative strategy introduces a type-I heterojunction, combining the properties of SbTe and WSe nanosheets, to overcome these obstacles. The heterojunction is prepared through a precise stacking approach to create a single-side barrier on the valence band and a near-zero offset on the conduction band.
View Article and Find Full Text PDFExcitonic devices based on interlayer excitons in van der Waals heterobilayers are a promising platform for advancing photoelectric interconnection telecommunications. However, the absence of exciton emission in the crucial telecom C-band has constrained their practical applications. Here, this limitation is addressed by reporting exciton emission at 0.
View Article and Find Full Text PDFFerroelectric photovoltaics driven by spontaneous polarization (P ) holds a promise for creating the next-generation optoelectronics, spintronics and non-volatile memories. However, photoactive ferroelectrics are quite scarce in single homogeneous phase, owing to the severe P fatigue caused by leakage current of photoexcited carriers. Here, through combining inorganic and organic components as building blocks, we constructed a series of ferroelectric semiconductors of 2D hybrid perovskites, (HA) (MA) Pb Br (n=1-5; HA=hexylamine and MA=methylamine).
View Article and Find Full Text PDFβ-Ag Te has attracted considerable attention in the application of electronics and optoelectronics due to its narrow bandgap, high mobility, and topological insulator properties. However, it remains a significant challenge to synthesize 2D Ag Te because of the non-layered structure of Ag Te. Herein, the synthesis of large-size, ultrathin single crystal topological insulator 2D Ag Te via the van der Waals epitaxial method for the first time is reported.
View Article and Find Full Text PDFDeveloping low-cost and high-efficiency electrocatalysts to electrolyze water is an effective method for large-scale hydrogen production. For large-scale commercial applications, it is crucial to call for more efficient electrocatalysts with high-current density (≥1000 mA cm). However, it is challenging to simultaneously promote the large-scale production and hydrogen evolution reaction (HER) activity of these hydrogen catalysts.
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