Publications by authors named "Fangtao Huang"

The vapor-phase alkylation of phenol with methanol was investigated on X zeolites and modified X zeolites. First, the difference of product distribution was tested between acid zeolite (HZSM-5, HX, HMCM-22, and Hβ) and basic zeolite X (KX and CsX). Then, X zeolites were modified with Li, K, Cs, Ca, Mg, La, and Ce ion exchange to adjust the acid-base properties of the zeolites.

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ZSM-5 zeolites with modified acidity and diffusivity are employed as catalysts for the shape-selective alkylation of toluene with ethanol to -ethyltoluene (-ET). To avoid pore blocking and loss of active sites caused by traditional methods of enhancing -selectivity using modifiers, here, we constructed twin intergrowth structured ZSM-5 (Z5-T), achieving modulation of the inherent acidity and diffusivity through interface engineering. The characterization results demonstrate that due to the intergrowth interface, the Z5-T catalyst forms more inherent Lewis acid sites and also renders more sinusoidal channels opened to the surface.

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