The Kerr nonlinearity allows for exact analytic soliton solutions in 1+1D. While nothing excludes that these solitons form in naturally occurring real-world 3D settings as solitary walls or stripes, their observation had previously been considered unfeasible because of the strong transverse instability intrinsic to the extended nonlinear perturbation. We report the observation of solitons that are fully compatible with the 1+1D Kerr paradigm limit hosted in a 2+1D system.
View Article and Find Full Text PDFWe report the observation of a two-dimensional (2D) dam break flow of a photon fluid in a nonlinear optical crystal. By precisely shaping the amplitude and phase of the input wave, we investigate the transition from one-dimensional (1D) to 2D nonlinear dynamics. We observe wave breaking in both transverse spatial dimensions with characteristic timescales determined by the aspect ratio of the input box-shaped field.
View Article and Find Full Text PDFWe experimentally and theoretically investigate thermal domain evolution in near-transition KTN:Li. Results allow us to establish how polarization supercrystals form, a hidden 3D topological phase composed of hypervortex defects. These are the result of six converging polarization vortices, each associated to one orientation of the 3D broken inversion symmetry.
View Article and Find Full Text PDFExtreme waves are intense and unexpected wavepackets ubiquitous in complex systems. In optics, these rogue waves are promising as robust and noise-resistant beams for probing and manipulating the underlying material. Localizing large optical power is crucial especially in biomedical systems, where, however, extremely intense beams have not yet been observed.
View Article and Find Full Text PDFNanomaterials (Basel)
February 2023
We report a spectroscopic investigation of potassium-lithium-tantalate-niobate (KTN:Li) across its room-temperature ferroelectric phase transition, when the sample manifests a supercrystal phase. Reflection and transmission results indicate an unexpected temperature-dependent enhancement of average index of refraction from 450 nm to 1100 nm, with no appreciable accompanying increase in absorption. Second-harmonic generation and phase-contrast imaging indicate that the enhancement is correlated to ferroelectric domains and highly localized at the supercrystal lattice sites.
View Article and Find Full Text PDFWe experimentally and numerically explore the role of dimensionality in multiple (three or more) soliton fusion supported by nonreciprocal energy exchange. Three-soliton fusion into an intense wave is found when an extra dimension, with no broken inversion symmetry, is involved. The phenomenon is observed for 2+1D spatial waves in photorefractive crystals, where solitons are supported by a spatially local saturated Kerr-like self-focusing and fusion is driven by the leading nonlocal correction, the spatial analog of the nonlinear Raman effect.
View Article and Find Full Text PDFA hyperbolic medium will transfer super-resolved optical waveforms with no distortion, support negative refraction, superlensing, and harbor nontrivial topological photonic phases. Evidence of hyperbolic effects is found in periodic and resonant systems for weakly diffracting beams, in metasurfaces, and even naturally in layered systems. At present, an actual hyperbolic propagation requires the use of metamaterials, a solution that is accompanied by constraints on wavelength, geometry, and considerable losses.
View Article and Find Full Text PDFWe observe chaotic optical wave dynamics characterized by erratic energy transfer and soliton annihilation and creation in the aftermath of a three-soliton collision in a photorefractive crystal. Irregular dynamics are found to be mediated by the nonlinear Raman effect, a coherent interaction that leads to nonreciprocal soliton energy exchange. Results extend the analogy between solitons and particles to the emergence of chaos in three-body physics and provide new insight into the origin of the irregular dynamics that accompany extreme and rogue waves.
View Article and Find Full Text PDFWe perform percolation analysis of crossed-polarizer transmission images in a biased nanodisordered bulk KTN:Li perovskite. Two distinct percolative transitions are identified at two electric field thresholds. The low-field transition involves a directional fractal chain of dimension D=1.
View Article and Find Full Text PDFWe demonstrate experimentally in biased photorefractive crystals that collisions between random-amplitude optical spatial solitons produce long-tailed statistics from input Gaussian fluctuations. The effect is mediated by Raman nonlocal corrections to Kerr self-focusing that turn soliton-soliton interaction into a Maxwell demon for the output wave amplitude.
View Article and Find Full Text PDFFrom optics to hydrodynamics, shock and rogue waves are widespread. Although they appear as distinct phenomena, transitions between extreme waves are allowed. However, these have never been experimentally observed because control strategies are still missing.
View Article and Find Full Text PDFAn ideal illumination for light sheet fluorescence microscopy entails both a localized and a propagation invariant optical field. Bessel beams and Airy beams satisfy these conditions, but their non-diffracting feature comes at the cost of the presence of high-energy side lobes that notably degrade the imaging contrast and induce photobleaching. Here, we demonstrate the use of a light droplet illumination whose side lobes are suppressed by interfering Bessel beams of specific k-vectors.
View Article and Find Full Text PDFA landmark of statistical mechanics, spin-glass theory describes critical phenomena in disordered systems that range from condensed matter to biophysics and social dynamics. The most fascinating concept is the breaking of replica symmetry: identical copies of the randomly interacting system that manifest completely different dynamics. Replica symmetry breaking has been predicted in nonlinear wave propagation, including Bose-Einstein condensates and optics, but it has never been observed.
View Article and Find Full Text PDFUsing temperature-resolved dielectric spectroscopy in the range of 75-320 K we have inspected the solid-like and liquid-like arrangements of nanometric dipoles (polar nanoregions) embedded in sodium-enriched potassium-tantalate-niobate (KNTN), a chemically-substituted complex perovskite crystal hosting inherent substitutional disorder. The study of order versus direction is carried out using Fröhlich entropy measurements and indicates the presence of four long-range symmetry phases, two of which are found to display profoundly anisotropic features. Exotic phases are found for which the dipoles at one fixed temperature manifest a liquid reorientational response along one crystal axis and a solid-like behavior along another axis.
View Article and Find Full Text PDFA single-photon beating with itself can produce even the most elaborate optical fringe pattern. However, the large amount of information enclosed in such a pattern is typically inaccessible, since the complete distribution can be visualized only after many detections. In fact this limitation is only true for delocalized patterns.
View Article and Find Full Text PDFMore than thirty years ago Glauber suggested that the link between the reversible microscopic and the irreversible macroscopic world can be formulated in physical terms through an inverted harmonic oscillator describing quantum amplifiers. Further theoretical studies have shown that the paradigm for irreversibility is indeed the reversed harmonic oscillator. As outlined by Glauber, providing experimental evidence of these idealized physical systems could open the way to a variety of fundamental studies, for example to simulate irreversible quantum dynamics and explain the arrow of time.
View Article and Find Full Text PDFUsing the history dependence of a dipolar glass hosted in a compositionally disordered lithium-enriched potassium tantalate niobate (KTN:Li) crystal, we demonstrate scale-free optical propagation at tunable temperatures. The operating equilibration temperature is determined by previous crystal spiralling in the temperature/cooling-rate phase space.
View Article and Find Full Text PDFWe report the observation of Gaussian beam fragmentation into Airy-like waveforms during nonlinear propagation. The effect is supported by the high-intensity photovoltaic nonlinearity arising in unbiased pure congruent lithium niobate. The process is found to occur when the nonlinear response is dominated by the nonlocal effects associated with the charge-displacement process.
View Article and Find Full Text PDFWe consider optical propagation through a centrosymmetric photorefractive crystal with the externally applied bias voltage modulated along the optical propagation direction. We analytically prove that, if the modulation scale is smaller than the optical diffraction length, the resulting effective nonlinearity has an even parity in the transverse plane for an even-symmetric intensity profile and supports bending-free solitons down to few-micrometer beam widths. Numerical integration of the full photorefractive model for light-matter interaction allows us to confirm the feasibility of these miniaturized solitons and, for longer modulation periods, to investigate the excitation of self-trapped wiggling optical beams.
View Article and Find Full Text PDFWe demonstrate electro-optic spatial two-dimensional mode switching in a bulk sample of potassium lithium tantalate niobate. Spatial confinement, mode coupling, and electro-optic functionality are mediated by two photorefractive needle solitons of opposite electroholographic charges embedded together in their anisotropic lobular structure.
View Article and Find Full Text PDFTransverse instabilities are shown to accompany counterpropagation of optical beams through reflection gratings in Kerr media. The instability threshold of continuous waves is analytically derived, and it is shown that the presence of the grating broadens and narrows the stability region of plane waves in focusing and defocusing media, respectively. Furthermore, counterpropagating soliton stability is numerically investigated and compared with the transverse modulation instability analysis, revealing an underlying physical link.
View Article and Find Full Text PDFWe investigate (1+1D) spatial optical solitons embedded in a fixed-volume grating in centrosymmetric photorefractive crystals. We numerically identify a two-parameter soliton family and deduce both its existence surface and soliton profiles. For shallow gratings, the soliton Fourier spectrum exhibits three lobes located at the reciprocal lattice points -K, 0, and K.
View Article and Find Full Text PDFWe analytically predict the existence of both spatial bright and dark counterpropagating solitons in a reflection grating in the presence of the Kerr nonlinearity. The basic trapping mechanism consists of a twofold balance where diffraction is compensated by self-focusing and reflection is altered by the nonlinear-induced interferometric grating. We find that, whenever the spectral soliton profile lies within the grating stop band, bright and dark solitons exist only if the mutual phase of the counterpropagating solitons is pi or 0, respectively.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
March 2005
We extend investigation of one-dimensional solitons in biased photorefractive crystals to long propagation regimes, where self-trapping over a large number of linear diffraction lengths combines with the progressive growth of generally distortive spatially nonlocal components. Results indicate that saturation halts the radiative misshaping of the soliton, which follows that specific bending trajectory along which its evolution is governed by the same local screening nonlinearity that intervenes in short propagation conditions, where spatial nonlocality has a negligible effect. This finding not only allows the prediction of the curvature and of the relative role of charge displacement and diffusion, but implies a set of interesting observable effects, such as boomerangs, counterpropagating and cavity geometries, quasirectilinear and anomalous collisions, along with specific consequences on soliton arrays and on coupling to bulk gratings.
View Article and Find Full Text PDFThe observation of initial time dynamics of self-trapping in photorefractive media indicates that optical spatial solitons supported by intense cumulative nonlinearities manifest temporally nonlocal signatures in the form of stretched exponential behavior. This general result, supported also by numerical predictions, is triggered by wave shaping in a time-constant buildup map, a consequence of the spatially resolved inertial response intrinsic to the geometrical transition from a diffracting to a self-focused beam, inherent to soliton appearance.
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