This paper theoretically investigates the generation of isolated elliptically polarized attosecond pulses with a tunable ellipticity from the interaction of Cl molecule and a polarization-gating laser pulse. A three-dimensional calculation based on the time-dependent density functional theory is done. Two different methods are proposed for generating elliptically polarized single attosecond pulses.
View Article and Find Full Text PDFEnhanced high harmonics are generated by local and global optimization approaches to achieve a supercontinuum spectrum. Based on time-dependent density functional theory calculations, the optimum convolution of a two-color chirped pulse from an N2O molecule implements a significant enhancement of cutoff frequency and high harmonic yield. The optimization is done by controlling the effective chirp parameters and the carrier-envelope phase of the designed laser field.
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