Electrochemical CO reduction reaction (CO-RR) in non-aqueous electrolytes offers significant advantages over aqueous systems, as it boosts CO solubility and limits the formation of HCO and CO anions. Metal-organic frameworks (MOFs) in non-aqueous CO-RR makes an attractive system for CO capture and conversion. However, the predominantly organic composition of MOFs limits their electrical conductivity and stability in electrocatalysis, where they suffer from electrolytic decomposition.
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