This study investigated transport pathways and photochemical formation responsible for ozone exceedances during the September 2021 deployment of the Tracking Aerosol Convection Interactions ExpeRiment/Air Quality (TRACER-AQ) campaign in Houston, Texas. We focused on two ozone episodes, September 6th-September 11th ("Episode 1") and September 23rd-September 26th ("Episode 2"), when the maximum daily eight-hour average (MDA8) ozone at surface monitors exceeded 70 ppbv. Long-range transport patterns of air masses during these episodes were from the central/northern US.
View Article and Find Full Text PDFThis study investigated the long-term variations in ambient levels of surface ozone, volatile organic compounds (VOCs), and nitrogen oxides (NO) within the Houston-Galveston-Brazoria (HGB) region. Analysis of ozone levels revealed an overall reduction in the maximum daily 8-h average ozone (MDA8 O) from 2000 to 2019 (April-October) with an average rate of ∼ -0.48 ppb/yr across HGB.
View Article and Find Full Text PDFEpidemiological studies have linked exposure to ambient particulate matter (PM) with gastrointestinal (GI) diseases. Ambient ultrafine particles (UFP) are the redox-active sub-fraction of PM2.5, harboring elemental and polycyclic aromatic hydrocarbons from urban environmental sources including diesel and gasoline exhausts.
View Article and Find Full Text PDFThe goal of this study was to characterize changes in components and toxicological properties of PM during the nationwide 2019-Coronavirus (COVID-19) lockdown restrictions in Milan, Italy. Time-integrated PM filters were collected at a residential site in Milan metropolitan area from April 11th to June 3rd at 2020, encompassing full-lockdown (FL), the followed partial-lockdown (PL2), and full-relaxation (FR) periods of COVID-19 restrictions. The collected filters were analyzed for elemental and organic carbon (EC/OC), water-soluble organic carbon (WSOC), individual organic species (e.
View Article and Find Full Text PDFIn this study, we investigated aerosol chemical composition, spectral properties of aerosol extracts, and source contributions to the aerosol light-absorbing brown carbon (BrC) in central Los Angeles from July 2018 to March 2019, during warm and cold seasons. Spectrophotometric measurements (water and methanol extracts; 200 < λ < 1100) and chemical analyses were performed on collected particulate matter (PM), and relationships of BrC light absorption (Abs) to source tracer chemical species were evaluated. Mass absorption efficiency (MAE) of both water and methanol extracted solutions exhibited an increasing trend from warm period to cold season, with an annual average value of 0.
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