Publications by authors named "Edward Bielejec"

Ion implantation is a key capability for the semiconductor industry. As devices shrink, novel materials enter the manufacturing line, and quantum technologies transition to being more mainstream. Traditional implantation methods fall short in terms of energy, ion species, and positional precision.

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Solid-state quantum emitters have emerged as a leading quantum memory for quantum networking applications. However, standard optical characterization techniques are neither efficient nor repeatable at scale. Here we introduce and demonstrate spectroscopic techniques that enable large-scale, automated characterization of colour centres.

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Local crystallographic features negatively affect quantum spin defects by changing the local electrostatic environment, often resulting in degraded or varied qubit optical and coherence properties. Few tools exist that enable the deterministic synthesis and study of such intricate systems on the nano-scale, making defect-to-defect strain environment quantification difficult. In this paper, we highlight state-of-the-art capabilities from the U.

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Understanding carrier trapping in solids has proven key to semiconductor technologies, but observations thus far have relied on ensembles of point defects, where the impact of neighboring traps or carrier screening is often important. Here, we investigate the capture of photogenerated holes by an individual negatively charged nitrogen-vacancy (NV) center in diamond at room temperature. Using an externally gated potential to minimize space-charge effects, we find the capture probability under electric fields of variable sign and amplitude shows an asymmetric-bell-shaped response with maximum at zero voltage.

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Article Synopsis
  • Focused ion beam implantation can precisely place defect centers in wide bandgap semiconductors but has low activation efficiency for creating single photon emitters.
  • A new scalable technique using multiple low-ion-implantation steps and in situ photoluminescence evaluation achieved a 70% yield of single defects in silicon carbide, significantly improving on typical methods.
  • This method shows promise for enhancing quantum information technologies and can be combined with techniques like annealing and cryogenic operations to work with other materials.
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  • - Diamond color centers, especially the negatively charged silicon vacancy (SiV) center, are important in quantum optics due to their narrow emission linewidth and favorable spin properties, making them suitable for various technologies.
  • - Nanodiamond (ND)-based SiV centers can be integrated into advanced structures for applications like biological imaging and sensing, and ion implantation is a key method for creating specific numbers of these color centers.
  • - The study successfully created single SiV centers in nanodiamonds, showing stable single-photon emission at room temperature, which opens new possibilities for advancements in quantum photonics, sensing, and biomedicine.
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We report tunable excitation-induced dipole-dipole interactions between silicon-vacancy color centers in diamond at cryogenic temperatures. These interactions couple centers into collective states, and excitation-induced shifts tag the excitation level of these collective states against the background of excited single centers. By characterizing the phase and amplitude of the spectrally resolved interaction-induced signal, we observe oscillations in the interaction strength and population state of the collective states as a function of excitation pulse area.

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An in situ counted ion implantation experiment improving the error on the number of ions required to form a single optically active silicon vacancy (SiV) defect in diamond 7-fold compared to timed implantation is presented. Traditional timed implantation relies on a beam current measurement followed by implantation with a preset pulse duration. It is dominated by Poisson statistics, resulting in large errors for low ion numbers.

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The application of color centers in wide-bandgap semiconductors to nanoscale sensing and quantum information processing largely rests on our knowledge of the surrounding crystalline lattice, often obscured by the countless classes of point defects the material can host. Here, we monitor the fluorescence from a negatively charged nitrogen-vacancy (NV) center in diamond as we illuminate its vicinity. Cyclic charge state conversion of neighboring point defects sensitive to the excitation beam leads to a position-dependent stream of photo-generated carriers whose capture by the probe NV leads to a fluorescence change.

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We characterize a high-density sample of negatively charged silicon-vacancy (SiV^{-}) centers in diamond using collinear optical multidimensional coherent spectroscopy. By comparing the results of complementary signal detection schemes, we identify a hidden population of SiV^{-} centers that is not typically observed in photoluminescence and which exhibits significant spectral inhomogeneity and extended electronic T_{2} times. The phenomenon is likely caused by strain, indicating a potential mechanism for controlling electric coherence in color-center-based quantum devices.

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Point defects in SiC are an attractive platform for quantum information and sensing applications because they provide relatively long spin coherence times, optical spin initialization, and spin-dependent fluorescence readout in a fabrication-friendly semiconductor. The ability to precisely place these defects at the optimal location in a host material with nano-scale accuracy is desirable for integration of these quantum systems with traditional electronic and photonic structures. Here, we demonstrate the precise spatial patterning of arrays of silicon vacancy ([Formula: see text]) emitters in an epitaxial 4H-SiC (0001) layer through mask-less focused ion beam implantation of Li.

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Article Synopsis
  • Developing quantum computers requires effectively distributing entanglement among many qubits, and diamond colour centres are promising candidates due to their remote entanglement and coherent control capabilities.
  • This research introduces a method to integrate high-yield "quantum microchiplets" made of diamond waveguide arrays into photonic integrated circuits, achieving a defect-free arrangement.
  • The study demonstrates that individual colour centre transitions can be finely tuned, allowing for consistent and stable optical performance, which is vital for advancing quantum repeaters and processors.
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By engineering atomic geometries composed of nearly 1000 atomic segments embedded in micro-resonators, we observe Bragg resonances induced by the atomic lattice at the telecommunication wavelength. The geometrical arrangement of erbium atoms into a lattice inside a silicon nitride (SiN) microring resonator reduces the scattering loss at a wavelength commensurate with the lattice. We confirm dependency of light emission to the atomic positions and lattice spacing and also observe Fano interference between resonant modes in the system.

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Article Synopsis
  • Quantum systems can lose their coherence when interacting with their environment, particularly due to thermal vibrations in solid-state systems, making it essential to lower operational temperatures to maintain performance.
  • A nano-electro-mechanical system was used to mitigate the effects of thermal phonons on a silicon-vacancy spin qubit in diamond, allowing for control of the strain environment without changing temperature.
  • This control improves optical transitions and spin coherence and suggests potential for strong coupling between the spin and single phonons, paving the way for advanced quantum technologies like phonon-mediated quantum gates.
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Article Synopsis
  • The research focuses on creating defect centre-nanocavity systems to enhance the connection between spin quantum memories and photons for quantum networks.
  • They successfully used a maskless method to create single silicon vacancy (SiV) centres in diamond with high precision through ion beam implantation.
  • The study shows a low conversion yield that increases significantly with additional electron irradiation, and it reveals promising characteristics for these quantum emitters that could aid in developing advanced quantum information processors.
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