Towards shaping picosecond strain pulses via magnetostrictive transducers.

Using time-resolved x-ray diffraction, we demonstrate the manipulation of the picosecond strain response of a metallic heterostructure consisting of a dysprosium (Dy) transducer and a niobium (Nb) detection layer by an external magnetic field. We utilize the first-order ferromagnetic-antiferromagnetic phase transition of the Dy layer, which provides an additional large contractive stress upon laser excitation compared to its zero-field response. This enhances the laser-induced contraction of the transducer and changes the shape of the picosecond strain pulses driven in Dy and detected within the buried Nb layer.

Epitaxial growth of TbFe on piezoelectric LiNbO Z-cut.

The strongly magnetostrictive TbFe compound has been epitaxially grown on Z-cut Lithium Niobate (LiNbO) substrates after the deposition of various buffer layers (Mo, Ti and Ti/Mo). Detailed and combined RHEED and x-ray analysis permitted to unravel the in-plane and relative orientation relationships (OR) of the different materials in the system. Despite the use of different templates with different structural orders, similar final OR are eventually found between the piezoelectric substrate and the magnetic layer.

Epitaxial growth of magnetostrictive TbFe2 films on piezoelectric LiNbO3.

The TbFe compound has been deposited by molecular beam epitaxy on lithium niobate (LN) substrates with different orientations (LN Z-, 128 Y- and 41 Y-cuts). Despite the challenging growth on these unconventional substrates, crystalline TbFe films (as a single orientated domain or with a limited number of orientations) of reasonable structural quality could be obtained after the deposition of a Mo buffer layer. Detailed and combined RHEED and x-ray analysis permitted to unravel the complex Mo and TbFe crystal orientations and to reveal common 3D orientation relationships between the different lattices, whatever the initial LN cut.

Tracking picosecond strain pulses in heterostructures that exhibit giant magnetostriction.

We combine ultrafast X-ray diffraction (UXRD) and time-resolved Magneto-Optical Kerr Effect (MOKE) measurements to monitor the strain pulses in laser-excited TbFe/Nb heterostructures. Spatial separation of the Nb detection layer from the laser excitation region allows for a background-free characterization of the laser-generated strain pulses. We clearly observe symmetric bipolar strain pulses if the excited TbFe surface terminates the sample and a decomposition of the strain wavepacket into an asymmetric bipolar and a unipolar pulse, if a SiO glass capping layer covers the excited TbFe layer.

Spin-polarized resonant surface state in (1 1 1) Sm Gd Al, a zero-magnetization ferromagnet.

The electronic structure of (1 1 1) Sm Gd Al, a zero-magnetization ferromagnet, is investigated by angle- and spin- resolved photoemission spectroscopy. An intense electron pocket strongly localized around [Formula: see text] and close to the Fermi level is observed and analyzed in detail. Its various characteristics, combined with electronic structure calculations, reveal a resonant surface state of 5d character and Λ symmetry, likely built on bulk states developing around L points.

Ferroelectric Control of Organic/Ferromagnetic Spinterface.

Organic multiferroic tunnel junctions based on La Sr MnO /poly(vinylidene fluoride) (PVDF)/Co structures are fabricated. The tunneling magneto-resistance sign can be changed by electrically switching the ferroelectric polarization of PVDF barrier. It is demonstrated that the spin-polarization of the PVDF/Co spinterface can be actively controlled by tuning the ferroelectric polarization of PVDF.

Persistent nonequilibrium dynamics of the thermal energies in the spin and phonon systems of an antiferromagnet.

We present a temperature and fluence dependent Ultrafast X-Ray Diffraction study of a laser-heated antiferromagnetic dysprosium thin film. The loss of antiferromagnetic order is evidenced by a pronounced lattice contraction. We devise a method to determine the energy flow between the phonon and spin system from calibrated Bragg peak positions in thermal equilibrium.

Impact of buffer layer and Pt thickness on the interface structure and magnetic properties in (Co/Pt) multilayers.

The influence of Pt thickness on the interface structure (roughness / intermixing) and magnetic properties has been investigated for (Co / Pt) multilayers sputtered on a Pt or a thin oxide (MgO or AlO x ) buffer layer. When Pt thickness increases from 1.2 nm-2.

Jamming behavior of domains in a spiral antiferromagnetic system.

Using resonant magnetic x-ray photon correlation spectroscopy, we show that the domains of a spiral antiferromagnet enter a jammed state at the onset of long-range order. We find that the slow thermal fluctuations of the domain walls exhibit a compressed exponential relaxation with an exponent of 1.5 found in a wide variety of solidlike jammed systems and can be qualitatively explained in terms of stress release in a stressed network.

Magnetic and magnetoelastic properties of epitaxial SmFe2 thin film.

We report on magnetic and magnetoelastic measurements for a 5000 Å (110) SmFe(2) thin film, which was successfully analyzed by means of a point charge model for describing the effect of the epitaxial growth in this kind of system. Some of the main conclusions of the Mössbauer and magnetoelastic results and the new magnetization results up to 5 T allow us to get a full description of the crystal electric field, exchange, and magnetoelastic behavior in this compound. So, new single-ion parameters are obtained for the crystal field interaction of samarium ions, A(4)(r(4)) = +755 K/ion and A(6)(r(6)) = -180 K/ion, and new single-ion magnetoelastic coupling B(γ,2) is approximately equal -200 MPa and B(ε,2) is approximately equal MPa, which represent the tetragonal and the in-plane shear deformations, respectively.

Low temperature exchange bias in [DyFe(2)/YFe(2)] superlattices: effect of the thermo-magnetic preparation.

The effect of the thermo-magnetic preparation on exchange bias is investigated in an exchange-coupled [3 nm DyFe(2)/12 nmYFe(2)](22) superlattice. X-ray magnetic circular dichroism (XMCD) experiments at low temperature reveal that exchange bias originates from the quenched DyFe(2) magnetization, biasing the unpinned YFe(2) reversal. This quenched configuration can be tailored by changing the cooling field or the magnetic preparation at 300 K before zero-field cooling.

Long range spin ferromagnetic order with zero magnetization in (111)Sm(1-x)Gd(x)Al(2) films.

Bulk Sm(1-x)Gd(x)Al(2) (0.01 View Article and Find Full Text PDF

Propagation of Nd magnetic phases in Nd/Sm(001) superlattices.

The propagation of Nd long range magnetic order in the hexagonal and cubic sublattices has been investigated in double hexagonal compact Nd/Sm(001) superlattices by resonant x-ray magnetic scattering at the Nd L(2) absorption edge. For a superlattice with 3.7 nm thick Sm layers, the magnetic structure of the hexagonal sublattice propagates coherently through several bilayers, whereas the order in the cubic sublattice remains confined to single Nd blocks.