Sewage sludge is recognized as both a source and a reservoir for antibiotic resistance genes (ARGs). Within an anaerobic digestion (AD) system, the presence of microplastics (MPs) has been observed to potentially facilitate the proliferation of these ARGs. Understanding the influence of MPs on microbial behavior and horizontal gene transfer (HGT) within the AD system is crucial for effectively managing the dissemination of ARGs in the environment.
View Article and Find Full Text PDFThe pervasive occurrence of emerging contaminants (ECs) in sewage sludge (SWS) poses significant safety challenges concerning the processing, disposal, and secure application, ultimately jeopardizing both human health and the ecological environment. To comprehensively comprehend the evolutionary trajectories, present state, and research advancements in the field of ECs in SWS, a systematic was conducted, scrutinizing the annual publication quantity, disciplinary distribution, core authors, involved nations/regions, pertinent keywords, and citation status of 2082 research publications related to ECs in SWS from 1990 to 2023. The results indicate a substantial upward trajectory in the research literature pertaining to ECs in SWS.
View Article and Find Full Text PDFObjective: The objective of the study was to systemically evaluate the clinical efficacy of minimally invasive stereotactic puncture for intracranial hematoma evacuation in patients with cerebral hemorrhage.
Materials And Methods: Relevant studies in PubMed, Web of Science, MEDLINE, China National Knowledge Infrastructure, Wanfang, and VIP databases were searched. A meta-analysis was performed following the inclusion and exclusion criteria screening, data extraction, and literature quality evaluation.
Erythromycin (ERY), as a common macrolides antibiotic, is widely used for sterilisation and disinfection of humans or livestock whose migration and transformation in the surface water environment are significantly related to dissolved organic matter (DOM). The characteristics of DOM can be greatly influenced by the complexation between ERY with itself in soil infiltration system. Using spectroscopic techniques (excitation-emission matrices, parallel factor analysis, Fourier infrared spectroscopy, and synchronous fluorescence spectroscopies) to explore the complexation properties of each DOM component with ERY in the system.
View Article and Find Full Text PDFSulfadiazine (SD) is a common antibiotic administered to treat bacterial infections in livestock, and its fate and migration are greatly affected by dissolved organic matter (DOM). The soil infiltration system [a typical low-impact development (LID) facility] can significantly alter DOM properties during runoff pollution, thus affecting the complexation of SD with DOM. Here, the binding characteristics of different DOM components and SD in the soil infiltration system were explored using spectroscopic techniques (excitation-emission matrices, parallel factor analysis, and synchronous fluorescence spectroscopy).
View Article and Find Full Text PDFThe emergence and persistence of antibiotic resistance genes (ARGs) in wastewater treatment plants (WWTPs) has aroused growing public concern for its risk to human health and ecological safety. Moreover, heavy metals concentrated in sewage and sludge could potentially favour co-selection of ARGs and heavy metal resistance genes (HMRGs). In this study, the profile and abundance of antibiotic and metal resistance genes in influent, sludge and effluent were characterized based on the Structured ARG Datebase (SARG) and Antibacterial Biocide and Metal Resistance Gene Datebase (BacMet) by metagenomic analysis.
View Article and Find Full Text PDFA storm-drain inlet is an important link in the transport of microplastic pollutants in urban rainwater runoff. In three functional districts (agricultural, commercial, and residential) from Beijing South 2nd Ring Road to South 6th Ring Road, microplastics in storm-drain inlet sediments were analyzed for abundance and characteristics. The abundance of microplastics in the collected samples ranged from 1121 ± 247 items kg to 7393 ± 491 items kg.
View Article and Find Full Text PDFJ Environ Sci (China)
March 2023
Citrate (Ct) was chosen as a typical chelator used in the Fe-peroxydisulfate (PDS) process to improve sludge dewaterability. The PDS-Fe-Ct process exhibited better performance in sludge dewatering than PDS-Fe. Specifically, with a PDS dosage of 1.
View Article and Find Full Text PDFCr(VI) has drawn growing concern because of its acute toxicity and strong carcinogenic properties to most organisms. Metal-organic frameworks (MOFs) have attracted broad interest in removing Cr(VI) as a novel porous adsorbent. In this work, a novel modified Cu@MIL-53(Fe) material and its derivatives have been successfully synthesized via solvothermal and calcination methods and applied for Cr(VI) removal.
View Article and Find Full Text PDFJ Environ Manage
October 2022
Mixtures of N, N-bis(carboxymethyl)-L-glutamic acid tetrasodium salt (GLDA) with citric acid (CA), glutamic acid (GLU), and aspartic acid (ASP) at the optimal proportion of 1:1, 1:2, and 2:1, respectively. They were employed for heavy metal removal from the sludge. The removal rate of common heavy metals (Cu, Pb, Zn, Ni, Cr, and Cd) and the retention degree of nutrients (total nitrogen, total phosphorus, available-N, Olsen-P, and organic matter) in the treated sludge were analyzed.
View Article and Find Full Text PDFIn order to investigate the photocatalytic degradation of dissolved organic matter (DOM) in landfill leachate, TiO/ZnO heterostructural composite powders were fabricated combining with hydrothermal synthesis and solid-state reaction method. The prepared TiO/ZnO composite powders consist of anatase TiO nanoparticles distributing on the surface of wurtzite ZnO particles. The optical band gap of TiO/ZnO powder is less than that of pure ZnO or TiO powder.
View Article and Find Full Text PDFEffluent organic matter (EfOM) contains a large number of substances that are harmful to both the environment and human health. To avoid the negative effects of organic matter in EfOM, advanced treatment of organic matter is an urgent task. Four typical oxidants (HO, PS, PMS, NaClO) and UV-combined treatments were used to treat micro-contaminants in the presence or absence of EfOM, because the active radical species produced in these UV-AOPs are highly reactive with organic contaminants.
View Article and Find Full Text PDFResource recovery from wastewater is a promising and challenging topic. Herein, a well-designed ion exchange membrane optimized light-driven photoelectrochemical unit (MPECS) was constructed to reduce the effect of inorganic salt on the photoelectrochemical performance of the photoanode. TiO/carbon dots/WO (TCDW) photoanode with the indirect Z-scheme heterojunction structure was successfully fabricated, achieving a strong light harvest performance (10.
View Article and Find Full Text PDFIn this present study, an advection ecological permeable dam (AEPD) based on a biofilm reactor was established to investigate pollution control performance and dissolved organic matter (DOM) bio-degradation. The AEPD achieved optimal efficiency-chemical oxygen demand, 6-53 mg/L; total nitrogen concentration, 1.47-6.
View Article and Find Full Text PDFEnviron Technol
January 2023
Stormwater wetlands play a crucial role in the urban environment, providing many ecosystem services. In this work, a stormwater wetland was developed to study the effects on the removal of pollutants and the characteristics of dissolved organic matter (DOM) under different operating conditions, such as hydraulic retention time (HRT) and water depth. The results showed that the stormwater wetland exhibited excellent pollutant-removal performance, such as NHN, TN, TP, COD, and suspended solids (SS).
View Article and Find Full Text PDFEcotoxicol Environ Saf
September 2021
Biochar-derived water-extractable organic matter (WEOM) was obtained under low-temperature pyrolysis (300 °C) using corncob as raw material. WEOM may affect the mobility and bioavailability of soil heavy metals (HMs) through complexation when biochar was used for soil HM remediation. Herein, the characteristics of complexation between HMs (Cr(III) and Cu(II)) and biochar-derived WEOM were investigated by using spectroscopic techniques in conjunction with parallel factor (PARAFAC) analysis and two-dimensional correlation spectroscopy (2D-COS).
View Article and Find Full Text PDFHydrophyte decomposition caused large amounts of dissolved organic matter (DOM) to enter aquatic environment that influence the migration and transformation of heavy metals (HMs). Six hydrophytes with five dry weight gradients (DWG) were used for the decomposition experiments. The results showed that protein-like materials occupy relatively high content in the hydrophyte-derived DOM.
View Article and Find Full Text PDFMagnetic phosphorylated chitosan composite (P-MCS), an excellent adsorbent for Co(II), was synthesized in this experiment via a facile fabrication. Its removal efficiency was improved by optimizing pH, contact time, and initial concentration. The adsorption isotherms and kinetic models of Co(II) by P-MCS followed the Langmuir model and the pseudo-second-order model, respectively.
View Article and Find Full Text PDFIn this study, an efficient adsorption and reusable magnetic ligand material (FeO@Chitosan-EDTA) was synthesized by binding EDTA dianhydride onto magnetic chitosan, and it was employed in removal of Co(II) from aqueous solution. The maximum adsorption capacity of Co(II) onto FeO@CS-EDTA was 48.78 mg/g at pH = 5 (303 K), which is much higher than that of FeO@Chitosan as well as chitosan.
View Article and Find Full Text PDFIn this study, the performance of LaCoO (LCO) catalytic ozonation was evaluated comprehensively, including the degradation efficiency of benzotriazole (BZA) as a typical emerging pollutant, toxic bromate reduction and the disinfection by-products (DBPs) precursors removal ability in effluent organic matter (EfOM), as well as EfOM reactive activity in catalytic ozonation. Additionally, the reduction of toxic halogenated by-products in (catalytic) ozonation was reported, which was not focused on previous researches before. Results showed that LCO catalytic ozonation improved the removal efficiency of BZA, UV and SUVA via enhanced HO· formation.
View Article and Find Full Text PDFBackground: Netrin-1 exhibits anti-inflammatory properties. Netrin-1 could alleviate brain injury of subarachnoid hemorrhage (SAH) rat. This study was designed to discern the utility of serum netrin-1 as a biomarker for assessing the severity and prognosis of patients with aneurysmal SAH.
View Article and Find Full Text PDFCarbamazepine (CBZ) is a worldwide anti-epileptic drug, whose fate and migration can be greatly influenced by contact with dissolved organic matter (DOM). The properties of DOM in road runoff can be greatly changed by grassy swale (GS) treatment, which influences the complexation of CBZ with DOM. Spectroscopic techniques were employed to explore the different binding properties between CBZ and DOM, and to understand the migration and biogeochemistry of CBZ.
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
December 2018
Characteristics of physicochemical parameters, dissolved-phase heavy metals, and polycyclic aromatic hydrocarbons (PAHs) were investigated for 68 urban snowmelt surface runoff and snowpack samples collected from five different functional areas in Beijing, including a business area (BA), a cultural and educational area (CEA), a garden area (GA), a residential area (RA), and a roadside area (RSA). Both snowmelt surface runoff and snowpack were significantly polluted by organic matter, as indicated by their high concentrations of chemical oxygen demand (COD) and total organic carbon (TOC). Among the 11 heavy metals analyzed, Zn was the most enriched in all samples, followed by Mn, Fe, and Cu, whereas the concentrations of Pb, Cr, Cd, As, Ni, Sb, and Co were comparatively low.
View Article and Find Full Text PDFIn this research, the adsorptive removal of diclofenac sodium, one of the representative pharmaceuticals and personal care products, from aqueous solution using FeO@MOF-100(Fe) magnetic microspheres was studied for the first time. The FeO@MOF-100(Fe) microspheres exhibit strong magnetism and stability, which were observed as a core-shell structure. The maximum adsorption capacity of FeO@MOF-100(Fe) for diclofenac sodium can reach 377.
View Article and Find Full Text PDFComposting leachates were collected to investigate the fluorescent characteristic and compositional change of dissolved organic matter (DOM) and the effects of the DOM and nutrients on heavy metal distribution during a leachate combination treatment process. Excitation-emission matrix (EEM) fluorescence spectra showed that, with the progress of the treatment units, the content of fulvic-like, humic-like, and protein-like substances gradually decreased. One fulvic-like component (C1), three humic-like components (C2, C3, and C4), and three protein-like components (C5, C6, and C7) were identified in the leachate DOM by parallel factor analysis.
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