High-order above-threshold ionisation of diatomic molecules by few-cycle bicircular and orthogonally polarised two-colour pulses.

Improved molecular strong-field approximation theory is used to calculate the ionisation probability for the high-order above-threshold ionisation process induced by a few-cycle pulse with two carrier frequencies and one envelope. The asymmetry in the photoelectron momentum distribution is due to the ultrashort nature of the driving pulse and due to the relative orientation of the molecule with respect to the laser field. We introduce the generalised asymmetry parameter, which can be used to quantitatively measure the asymmetry between the photoelectron spectra along arbitrarily many selected directions.

High-order harmonic generation by aligned homonuclear diatomic cations.

We introduce the theory of high-order harmonic generation by aligned homonuclear diatomic cations using a strong-field approximation. The target cation is represented as a system which consists of two atomic (ionic) centres and one active electron, while the driving field is either a monochromatic or bichromatic field. For a linearly polarised driving field, we investigate the differences between the harmonic spectra obtained with a neutral molecule and the corresponding molecular cation.

Elliptic Dichroism in the Above-Threshold Ionization of Molecules Induced by a Strong Laser Field.

Using a strong-field-approximation theory, we investigate the high-order above-threshold ionization of diatomic molecules exposed to the monochromatic and bichromatic elliptically polarized fields. We devote particular attention to the difference between the photoelectron momentum distributions obtained with fields with opposite helicity. This difference is quantified using the elliptic-dichroism parameter, which represents the normalized difference between the differential ionization rates calculated with driving fields with opposite helicity.

Nondipole effects in terahetz-pulse-assisted strong-field ionization.

Nondipole effects in processes assisted by a THz field having the strength of a few MV/cm can be significant due to its long wavelength. We illustrate this for strong-laser-field-induced ionization assisted by a THz field. To this end, we generalize our strong-field-approximation theory so that it includes the first-order term in a 1/c expansion of the vector potential.