Interfacial solar vapor generation (ISVG) is an emerging technology to alleviate the global freshwater crisis. However, high-cost, low freshwater collection rate, and salt-blockage issues significantly hinder the practical application of solar-driven desalination devices based on ISVG. Herein, with a low-cost copper plate (CP), nonwoven fabric (NWF), and insulating ethylene-vinyl acetate foam (EVA foam), a multistage device is elaborately fabricated for highly efficient simultaneous freshwater and salt collection.
View Article and Find Full Text PDFThe dyeing wastewater contains amounts of refractory organic compounds, and severely endangers the ecosystem and human health. To alleviate this problem, in this study, the low-cost broad-spectrum nano-adsorbent (denoted as CD/CA-g-CS) with strong antibacterial activity has been synthesized by chemical binding of β-cyclodextrin (β-CD) with chitosan (CS) and citric acid (CA) for high-efficient dyes scavenger. Taking advantage of the extraordinary water insolubility, porous nature and abundant surface groups, the synthesized CD/CA-g-CS outperforms the previously reported adsorbents in terms of adsorption performance.
View Article and Find Full Text PDFDuring the course of a review of our publication, we found two errors in Figure 4b and Figure 9 [...
View Article and Find Full Text PDFMaterials (Basel)
August 2022
The dilemma of diminishing freshwater resources caused by water pollution has always impacted human life. Solar-driven interfacial evaporation technology has the potential for freshwater production via solar-driven distillation. However, in solar-driven interfacial evaporation technology, it is difficult to overcome the problem of wastewater containing various contaminants.
View Article and Find Full Text PDFTo meticulously establish an efficient photothermal multifunctional hydrogel dressing is a prospective strategy for the treatment of diabetic chronic wounds. Herein, glucose oxidase (GO) was added to polydopamine/acrylamide (PDA/AM) hydrogels to reduce hyperglycemia to a normal level (3.9-6.
View Article and Find Full Text PDFBacterial biofilms on wounds can lead to ongoing inflammation and delayed reepithelialization, which brings a heavy burden to the medical systems. Nitric oxide based treatment has attracted attention because it is a promising strategy to eliminate biofilms and heal infected wounds. Herein, a series of tryptophan-based poly(ester urea)s with good biodegradation and biocompatibility were developed for the preparation of composite mats by electrospinning.
View Article and Find Full Text PDFJ Colloid Interface Sci
July 2022
Flame retardant and antibacterial investigation of cellulose has attracted more and more attention. In order to improve the modification efficiency, inspired by multiple hydrogen bonding in spider silk, flame retardant and antibacterial dual function modified cellulose was achieved by multi structure hydrogen bonding in this research. A novel nano SiO based Schiff base flame retardant (SiAPH) and dodecyl quaternary ammonium salt (HDAC) were synthesized.
View Article and Find Full Text PDFDiabetic wound treatment remains a major challenge due to the difficulties of eliminating bacterial biofilm and relieving wound hypoxia. To address these issues simultaneously, a multifunctional Dex-SA-AEMA/MnO/PDA (DSAMP) hydrogel platform was developed with excellent biocompatibility and porous structure. The hydrogel could absorb the exudate, maintain humidity and permeate oxygen, which was prepared by encapsulating polydopamine (PDA) and manganese dioxide (MnO) into Dex-SA-AEMA (DSA) hydrogel by UV irradiation.
View Article and Find Full Text PDFScope: Royal jelly (RJ) has a wide range of biological functions, its effect on hyperplasia of the mammary gland (HMG) in mammals is unclear. This study aims to investigate the effect of RJ on HMG and the dose-response relationship of RJ in the treatment of HMG.
Methods And Results: HMG rats are induced by intramuscular injection of estrogen (E2) and progesterone, and are treated with different doses of RJ (100, 200, 400, and 800 mg kg d ).
Infected wounds show delayed and incomplete healing processes and even render patients at a high risk of death due to the formed bacterial biofilms in the wound site, which protect bacteria against antimicrobial treatments and immune response. Nitric oxide based therapy is considered a promising strategy for eliminating biofilms and enhancing wound healing, which encounters a significant challenge of controlling the NO release behavior at the wound site. Herein, a kind of phenylalanine based poly(ester urea)s with high thermal stability are synthesized and fabricated to electrospun films as NO loading vehicle for infected wound treatment.
View Article and Find Full Text PDFThe chronic wounds often hinder wound healing resulting from infection; thus, an ideal wound dressing should be able to maintain a healthy wound microenvironment. Herein, peptide modified nanofibers reinforced hydrogel has been designed by Schiff base dynamic crosslinking. The incorporation of the nanofibers into the hydrogel extremely enhances the stability and mechanical strength of the hydrogel.
View Article and Find Full Text PDFCoating a cationic antibacterial layer on the surface of cotton fabric is an effective strategy to provide it with excellent antibacterial properties and to protect humans from bacterial cross-infection. However, washing with anionic detergent will inactivate the cationic antibacterial coating. Although this problem can be solved by increasing the amount of cationic antibacterial coating, excessive cationic antibacterial coating reduces the drapability of cotton fabric and affects the comfort of wearing it.
View Article and Find Full Text PDFThe current water treatment technology is still based on low energy efficient processes due to the complex composition of wastewater. To achieve high energy efficiency, many micro-porous materials with complex functional groups have been fabricated because of their high pollutant adsorption capabilities. In this work, antibacterial β-cyclodextrin-based nanoparticles (E-β-CDN) were prepared via one-pot method to explore their adsorption performance to pollutants in wastewater.
View Article and Find Full Text PDFAlthough traditional alkaline (TAL) process for ramie degumming is commonly used in the industry, it causes severe environmental concerns. In this work, an emerging organic solvent degumming process utilizing FeCl catalyst (FeCl-OS) was developed in one step. The influences of FeCl-OS system on fiber properties (e.
View Article and Find Full Text PDFA polyester hernia patch has received extensive attention in mesh hernia repair. However, it is still a challenge to develop polyester-based implants with inherent antibacterial properties due to the lack of active functional groups. In this study, poly(butylene succinate-co-butylene aspartate) (PBSA) was constructed by introducing aspartic acid on a polybutylene succinate (PBS) polyester chain (PBSA).
View Article and Find Full Text PDFACS Appl Mater Interfaces
November 2019
One of the fundamental properties of natural systems is their water transport ability, and living systems have efficient moisture management features. Here, a unique structure, inspired by the water transfer behavior in trees, was designed for one-dimensional (1D) fiber assemblies. In this 1D fiber assembly structure, a differential capillary effect enabling rapid water transfer at the interface between traditional cotton fibers and electrospun nanofibers was explored.
View Article and Find Full Text PDFIn this work, β-cyclodextrin (β-CD) based hollow nanoparticles (denoted as β-CDHN) with abundant active sites and high specific surface area were first fabricated via a facile one-step method. The β-CDHN presented a maximum adsorption capacity of 2080.35, 427.
View Article and Find Full Text PDFA facile route of 'copolymerization/blending' was proposed to fabricate silicon/nitrogen synergistically reinforced flame-retardant PA6 nanocomposites with simultaneously improved anti-dripping and mechanical properties. Firstly, a persistently inherent flame-retardant PA6 (FR-PA6), with 1,3-bis(3-aminopropyl)tetramethyl disiloxane (MSDS), was synthesized controllable amidation and a polycondensation reaction. Melamine cyanurate (MCA) nanoparticles as a 'gas phase' synergistic agent were then added into FR-PA6 to further improve its flame retardancy.
View Article and Find Full Text PDFBacterial infection is one of the most significant complications worldwide and has been one of the main factors of morbidity and mortality for the chronic wounds. Considering the negative charged feature of bacterial pathogens, a positive charged poly(ester amide) (PEA) micellar system based on lysine, arginine and phenylalanine is developed. In this study, a serials of PEA random copolymers can be obtained by altering the sorts of amino acids and feed ratio, and the self-assembled PEA micelles with an average diameter ranging from 150 to 200 nm exhibit the integrated properties of excellent biocompatibility and enzymatic biodegradation.
View Article and Find Full Text PDFThe stimuli-sensitive and biodegradable hydrogels are promising biomaterials as controlled drug delivery systems for diverse biomedical applications. In this study, we construct hybrid hydrogels combined with peptide-based bis-acrylate and acrylic acid (AAc). The peptide-based bis-acrylate/AAc hybrid hydrogel displays an interconnected and porous structure by scanning electron microscopy (SEM) observation and exhibits pH-dependent swelling property.
View Article and Find Full Text PDFConsidering the excellent thermo-mechanical properties, chemical stability and low cost of biodegradable aliphatic-aromatic copolyesters, they are an ideal matrix when functionalized for capturing pollutants in wastewater. In this work, biodegradable poly((butylene succinate--terephthalate)--serinol terephthalate) (PBSST) copolyesters with amino side group (-NH) were first synthesized through copolymerization, followed by grafting carboxymethyl-β-cyclodextrin (CM-β-CD) into PBSST molecular chains amidation reaction to prepare PBSST--β-CD. The corresponding nanofibrous membranes were then fabricated by electrospinning as adsorbents for efficiently removing cationic dye methyl blue (MB) from aqueous solutions.
View Article and Find Full Text PDFHere, charge-storage nonvolatile organic field-effect transistor (OFET) memory devices based on interfacial self-assembled molecules are proposed. The functional molecules contain various aromatic amino moieties (N-phenyl-N-pyridyl amino- (PyPN), N-phenyl amino- (PN), and N,N-diphenyl amino- (DPN)) which are linked by a propyl chain to a triethoxysilyl anchor group and act as the interface modifiers and the charge-storage elements. The PyPN-containing pentacene-based memory device (denoted as PyPN device) presents the memory window of 48.
View Article and Find Full Text PDFImmediate hemorrhage control and anti-infection play important roles in the wound management. Besides, a moist environment is also beneficial for wound healing. Hydrogels are promising materials in urgent hemostasis and drug release.
View Article and Find Full Text PDF