Translatory and rotatory motion of exchange-bias capped Janus particles controlled by dynamic magnetic field landscapes.

Magnetic Janus particles (MJPs), fabricated by covering a non-magnetic spherical particle with a hemispherical magnetic in-plane exchange-bias layer system cap, display an onion magnetization state for comparably large diameters of a few microns. In this work, the motion characteristics of these MJPs will be investigated when they are steered by a magnetic field landscape over prototypical parallel-stripe domains, dynamically varied by superposed external magnetic field pulse sequences, in an aqueous medium. We demonstrate, that due to the engineered magnetization state in the hemispherical cap, a comparably fast, directed particle transport and particle rotation can be induced.

Transport Efficiency of Biofunctionalized Magnetic Particles Tailored by Surfactant Concentration.

Controlled transport of surface-functionalized magnetic beads in a liquid medium is a central requirement for the handling of captured biomolecular targets in microfluidic lab-on-chip biosensors. Here, the influence of the physiological liquid medium on the transport characteristics of functionalized magnetic particles and on the functionality of the coupled protein is studied. These aspects are theoretically modeled and experimentally investigated for prototype superparamagnetic beads, surface-functionalized with green fluorescent protein immersed in buffer solution with different concentrations of a surfactant.

Gauge invariant and gauge dependent aspects of topological walking colloidal bipeds.

Paramagnetic colloidal spheres assemble to colloidal bipeds of various length in an external magnetic field. When the bipeds reside above a magnetic pattern and we modulate the direction of the external magnetic field, the rods perform topologically distinct classes of protected motion above the pattern. The topological protection allows each class to be robust against small continuous deformations of the driving loop of the external field.

Colloidal trains.

Single and double paramagnetic colloidal particles are placed above a magnetic square pattern and are driven with an external magnetic field processing around a high symmetry direction of the pattern. The external magnetic field and that of the pattern confine the colloids into lanes parallel to a lattice vector of the pattern. The precession of the external field causes traveling minima of the magnetic potential along the direction of the lanes.

Edge transport at the boundary between topologically equivalent lattices.

Edge currents of paramagnetic colloidal particles propagate at the edge between two topologically equivalent magnetic lattices of different lattice constant when the system is driven with periodic modulation loops of an external magnetic field. The number of topologically protected particle edge transport modes is not determined by a bulk-boundary correspondence. Instead, we find a rich variety of edge transport modes that depend on the symmetry of both the edge and the modulation loop.

Size limits of magnetic-domain engineering in continuous in-plane exchange-bias prototype films.

The application of superparamagnetic particles as biomolecular transporters in microfluidic systems for lab-on-a-chip applications crucially depends on the ability to control their motion. One approach for magnetic-particle motion control is the superposition of static magnetic stray field landscapes (MFLs) with dynamically varying external fields. These MFLs may emerge from magnetic domains engineered both in shape and in their local anisotropies.

Magnetophoretic lensing by concentric topographic cylinders of perpendicular magnetic anisotropy multilayers.

Colloidal magnetophoretic lensing of water suspended micrometer-sized superparamagnetic beads (SPBs) above a topographically patterned magnetic thin film system with perpendicular magnetic anisotropy is demonstrated. The magnetic pattern consisting of concentric annuli of micron-sized widths has been superimposed with a rotating external magnetic field, and it is shown that the trajectories of the SPBs above this structure are similar to light rays in an optical focusing lens. SPB trajectories converge towards the central region and have divergent trajectories while passing the center.

Lattice symmetries and the topologically protected transport of colloidal particles.

The topologically protected transport of colloidal particles on top of periodic magnetic patterns is studied experimentally, theoretically, and with computer simulations. To uncover the interplay between topology and symmetry we use patterns of all possible two dimensional magnetic point group symmetries with equal lengths lattice vectors. Transport of colloids is achieved by modulating the potential with external, homogeneous but time dependent magnetic fields.

Modification of the saturation magnetization of exchange bias thin film systems upon light-ion bombardment.

The magnetic modification of exchange bias materials by 'ion bombardment induced magnetic patterning' has been established more than a decade ago. To understand these experimental findings several theoretical models were introduced. Few investigations, however, did focus on magnetic property modifications caused by effects of ion bombardment in the ferromagnetic layer.

Manipulation of Superparamagnetic Beads on Patterned Exchange-Bias Layer Systems for Biosensing Applications.

A technology platform based on a remotely controlled and stepwise transport of an array arrangement of superparamagnetic beads (SPB) for efficient molecular uptake, delivery and accumulation in the context of highly specific and sensitive analyte molecule detection for the application in lab-on-a-chip devices is presented. The near-surface transport of SPBs is realized via the dynamic transformation of the SPBs' magnetic potential energy landscape above a magnetically stripe patterned Exchange-Bias (EB) thin film layer systems due to the application of sub-mT external magnetic field pulses. In this concept, the SPB velocity is dramatically influenced by the magnitude and gradient of the magnetic field landscape (MFL) above the magnetically stripe patterned EB substrate, the SPB to substrate distance, the magnetic properties of both the SPBs and the EB layer system, respectively, as well as by the properties of the external magnetic field pulses and the surrounding fluid.

Directed Magnetic Particle Transport above Artificial Magnetic Domains Due to Dynamic Magnetic Potential Energy Landscape Transformation.

An approach for a remotely controllable transport of magnetic micro- and/or nanoparticles above a topographically flat exchange-bias (EB) thin film system, magnetically patterned into parallel stripe domains, is presented where the particle manipulation is achieved by sub-mT external magnetic field pulses. Superparamagnetic core-shell particles are moved stepwise by the dynamic transformation of the particles' magnetic potential energy landscape due to the external magnetic field pulses without affecting the magnetic state of the thin film system. The magnetic particle velocity is adjustable in the range of 1-100 μm/s by the design of the substrate's magnetic field landscape (MFL), the particle-substrate distance, and the magnitude of the applied external magnetic field pulses.