Publications by authors named "Denise L Mauzerall"

Severe PM pollution threatens public health in India. Atmospheric stagnation traps emitted pollutants, worsening their health impacts. Global warming is anticipated to alter future stagnation patterns, impacting the effectiveness of air quality policies.

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Secondary inorganic aerosols play an important role in air pollution and climate change, and their formation modulates the atmospheric deposition of reactive nitrogen (including oxidized and reduced nitrogen), thus impacting the nitrogen cycle. Large-scale and long-term analyses of secondary inorganic aerosol formation based on model simulations have substantial uncertainties. Here we improve constraints on secondary inorganic aerosol formation using decade-long in situ observations of aerosol composition and gaseous precursors from multiple monitoring networks across the United States.

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Clean hydrogen has the potential to serve as an energy carrier and feedstock in decarbonizing energy systems, especially in "hard-to-abate" sectors. Although many countries have implemented policies to promote electrolytic hydrogen development, the impact of these measures on costs of production and greenhouse gas emissions remains unclear. Our study conducts an integrated analysis of provincial levelized costs and life cycle greenhouse gas emissions for all hydrogen production types in China.

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China's coal chemical sector uses coal as both a fuel and feedstock and its increasing greenhouse gas (GHG) emissions are hard to abate by electrification alone. Here we explore the GHG mitigation potential and costs for onsite deployment of green H and O in China's coal chemical sector, using a life-cycle assessment and techno-economic analyses. We estimate that China's coal chemical production resulted in GHG emissions of 1.

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Battery storage is critical for integrating variable renewable generation, yet how the location, scale, and timing of storage deployment affect system costs and carbon dioxide (CO) emissions is uncertain. We improve a power system model, SWITCH-China, to examine three nationally uniform battery deployment strategies (Renewable-connected, Grid-connected, and Demand-side) and a heterogeneous battery deployment strategy where each province is allowed to utilize any of the three battery strategies. Here, we find that the heterogeneous strategy always provides the lowest system costs among all four strategies, where provinces with abundant renewable resources dominantly adopt Renewable-connected batteries while those with limited renewables dominantly adopt Demand-side batteries.

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Industrial parks are emerging priorities for carbon mitigation. Here we analyze air quality, human health, and freshwater conservation co-benefits of decarbonizing the energy supply of 850 China's industrial parks. We examine a clean energy transition including early retirement of coal-fired facilities and subsequent replacement with grid electricity and onsite energy alternatives (municipal solid waste-to-energy, rooftop photovoltaic, and distributed wind power).

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In 2017, the Chinese government launched a clean heating campaign that replaced millions of rural coal stoves with various clean heaters. The clean heating program contributed to remarkable improvements in air quality. However, the benefits of reducing heating demand by improving building envelope efficiency were not sufficiently considered.

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Worldwide efforts to switch away from coal have increased the reliance on natural gas imports for countries with inadequate domestic production. In preparing for potential gas import disruptions, there have been limited attempts to quantify the environmental and human health impacts of different options and incorporate them into decision-making. Here, we analyze the air pollution, human health, carbon emissions, and water consumption impacts under a set of planning strategies to prepare for potentially fully disrupted natural gas imports in China.

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Large-scale carbon capture, utilization, and storage (CCUS) requires development of critical infrastructure to connect capture locations to geological storage sites. Here, we investigate what government policies would be required to make the development of CO pipelines and large-scale CCUS in the power sector economically viable. We focus on the transition from conventional coal to non-CO-emitting natural gas-fired Allam-cycle power with CCUS and study a system in which 156 Allam-cycle power generators representing 100 GW of capacity send their captured CO emissions to three geological storage locations in the central United States through 7500 miles of new pipeline.

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Background: Modeling suggests that climate change mitigation actions can have substantial human health benefits that accrue quickly and locally. Documenting the benefits can help drive more ambitious and health-protective climate change mitigation actions; however, documenting the adverse health effects can help to avoid them. Estimating the health effects of mitigation (HEM) actions can help policy makers prioritize investments based not only on mitigation potential but also on expected health benefits.

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China's gains in food production over the past four decades have been associated with substantial agricultural nitrogen losses, which contribute to air and water pollution, greenhouse gas emissions and damage to human health. Here, we explore the potential to improve agricultural production practices that simultaneously increase yields while addressing these environmental challenges. We link agronomic research with air quality modelling for an integrated assessment of four improved nitrogen management strategies: improved farm management practices with nitrogen use reductions; machine deep placement of fertilizer; enhanced-efficiency fertilizer use; and improved manure management.

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Natural gas vehicles (NGVs) have been promoted in China to mitigate air pollution, yet our measurements and analyses show that NGV growth in China may have significant negative impacts on climate change. We conducted real-world vehicle emission measurements in China and found high methane emissions from heavy-duty NGVs (90% higher than current emission limits). These emissions have been ignored in previous emission estimates, leading to biased results.

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Urban air pollution features large spatial and temporal variations due to the high heterogeneity in emissions and ventilation conditions, which render the pollutant distributions in complex urban terrains difficult to measure. Current urban air pollution models are not able to simulate pollutant dispersion and distribution at a low computational cost and high resolution. To address this limitation, we have developed the urban terrain air pollution (UTAP) dispersion model to investigate, at a spatial resolution of 5 m and a temporal resolution of 1 h, the distribution of the local traffic-related NO concentration at the pedestrian level in a 1 × 1 km area in Baoding, Hebei, China.

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Recent studies have reported methane (CH) emissions from abandoned and active oil and gas infrastructure across the United States, where measured emissions show regional variability. To investigate similar phenomena in West Virginia, we measure and characterize emissions from abandoned and active conventional oil and gas wells. In addition, we reconcile divergent regional CH emissions estimates by comparing our West Virginia emissions estimates with those from other states in the United States.

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Solar photovoltaic (PV) electricity generation is expanding rapidly in China, with total capacity projected to be 400 GW by 2030. However, severe aerosol pollution over China reduces solar radiation reaching the surface. We estimate the aerosol impact on solar PV electricity generation at the provincial and regional grid levels in China.

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China is the world's top carbon emitter and suffers from severe air pollution. We examine near-term air quality and CO co-benefits of various current sector-based policies in China. Using a 2015 base case, we evaluate the potential benefits of four sectoral mitigation strategies.

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Facing severe air pollution and growing dependence on natural gas imports, the Chinese government plans to increase coal-based synthetic natural gas (SNG) production. Although displacement of coal with SNG benefits air quality, it increases CO emissions. Due to variations in air pollutant and CO emission factors and energy efficiencies across sectors, coal replacement with SNG results in varying degrees of air quality benefits and climate penalties.

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Ground-level ozone (O), harmful to most living things, is produced from both domestic and foreign emissions of anthropogenic precursors. Previous estimates of the linkage from distant sources rely on the sensitivity approach (i.e.

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Black carbon (BC) aerosol strongly absorbs solar radiation, which warms climate. However, accurate estimation of BC's climate effect is limited by the uncertainties of its spatiotemporal distribution, especially over remote oceanic areas. The HIAPER Pole-to-Pole Observation (HIPPO) program from 2009 to 2011 intercepted multiple snapshots of BC profiles over Pacific in various seasons, and revealed a 2 to 5 times overestimate of BC by current global models.

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To increase energy security and reduce emissions of air pollutants and CO from coal use, China is attempting to duplicate the rapid development of shale gas that has taken place in the United States. This work builds a framework to estimate the lifecycle greenhouse gas (GHG) emissions from China's shale gas system and compares them with GHG emissions from coal used in the power, residential, and industrial sectors. We find the mean lifecycle carbon footprint of shale gas is about 30-50% lower than that of coal in all sectors under both 20 year and 100 year global warming potentials (GWP and GWP).

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Ammoniated aerosols are important for urban air quality, but emissions of the key precursor NH are not well quantified. Mobile laboratory observations are used to characterize fleet-integrated NH emissions in six cities in the U.S.

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Recent measurements of methane emissions from abandoned oil/gas wells show that these wells can be a substantial source of methane to the atmosphere, particularly from a small proportion of high-emitting wells. However, identifying high emitters remains a challenge. We couple 163 well measurements of methane flow rates; ethane, propane, and n-butane concentrations; isotopes of methane; and noble gas concentrations from 88 wells in Pennsylvania with synthesized data from historical documents, field investigations, and state databases.

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As part of the 12th Five-Year Plan, the Chinese government has developed air pollution prevention and control plans for key regions with a focus on the power, transport, and industrial sectors. Here, we investigate the contribution of residential emissions to regional air pollution in highly polluted eastern China during the heating season, and find that dramatic improvements in air quality would also result from reduction in residential emissions. We use the Weather Research and Forecasting model coupled with Chemistry to evaluate potential residential emission controls in Beijing and in the Beijing, Tianjin, and Hebei (BTH) region.

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Improvements in nitrogen use efficiency in crop production are critical for addressing the triple challenges of food security, environmental degradation and climate change. Such improvements are conditional not only on technological innovation, but also on socio-economic factors that are at present poorly understood. Here we examine historical patterns of agricultural nitrogen-use efficiency and find a broad range of national approaches to agricultural development and related pollution.

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