Self-assembly of two-dimensional, amorphous materials on a liquid substrate.

Recent experimental utilization of liquid substrate in the production of two-dimensional crystals, such as graphene, together with a general interest in amorphous materials, raises the following question: is it beneficial to use a liquid substrate to optimize amorphous material production? Inspired by epitaxial growth, we use a two-dimensional coarse-grained model of interacting particles to show that introducing a motion for the substrate atoms improves the self-assembly process of particles that move on top of the substrate. We find that a specific amount of substrate liquidity (for a given sample temperature) is needed to achieve optimal self-assembly. Our results illustrate the opportunities that the combination of different degrees of freedom provides to the self-assembly processes.

The effect of disordered substrate on crystallization in 2D.

In this work, the effect of amorphous substrate on crystallization is addressed. By performing Monte-Carlo simulations of solid on solid models, we explore the effect of the disorder on crystal growth. The disorder is introduced via local geometry of the lattice, where local connectivity and transition rates are varied from site to site.