Tensile Strain-Dependent Ultrafast Electron Transfer and Relaxation Dynamics in Flexible WSe/MoS Heterostructures.

Understanding and controlling carrier dynamics in two-dimensional (2D) van der Waals heterostructures through strain are crucial for their flexible applications. Here, femtosecond transient absorption spectroscopy is employed to elucidate the interlayer electron transfer and relaxation dynamics under external tensile strains in a WSe/MoS heterostructure. The results show that a modest ∼1% tensile strain can significantly alter the lifetimes of electron transfer and nonradiative electron-hole recombination by >30%.

Ag microlabyrinth/nanoparticles coated large-area thin PDMS films as flexible and transparent SERS substrates for in situ detection.

Flexible and transparent surface-enhanced Raman scattering (SERS) substrates haveattractedmuchattention as a fast, sensitive and in situ detection platform for practical applications. However, the large-area fabrication of flexible and transparent SERS substrates with high performance is still challenging. Here, a flexible and transparent SERS substrate based on large-area thin PDMS film decorated with Ag microlabyrinth/nanoparticles hierarchical structures (denoted as ALNHS@PDMS) is fabricated by using the floating-on-water method and magnetron sputtering technology.

3D Flexible SERS Substrates Integrated with a Portable Raman Analyzer and Wireless Communication for Point-of-Care Application.

With the development of flexible surface-enhanced Raman spectroscopy (SERS) substrates that can realize rapid detection, the SERS technique accompanied by miniaturized Raman spectrometers holds great promise for point-of-care testing (POCT). For an detection strategy, constructing high-performance flexible and transparent SERS substrates through a facile and cost-effective fabrication method is critically important. Herein, we present a simple method for fabricating a large-area flexible and transparent SERS substrate consisting of a silver-nanoparticle-grafted wrinkled polydimethylsiloxane (Ag NPs@W-PDMS) film, using a surface-wrinkling technique and magnetron sputtering technology.

Multicomponent gas detection technology of FDM and TDM based on photoacoustic spectroscopy.

In this paper, a multicomponent gas detection system based on photoacoustic spectroscopy (PAS) is proposed with a combination of frequency division multiplexing (FDM) and time division multiplexing (TDM), combining a resonance photoacoustic cell and broadband microphone. A PAS gas cell with a wide frequency response bandwidth was used to achieve the FDM by selecting a specific modulation frequency of each component gas. The sawtooth wave driver current of each laser was output at a constant time interval for achieving the TDM.

Two-component gas quartz-enhanced photoacoustic spectroscopy sensor based on time-division multiplexing of distributed-feedback laser driver current.

A two-component gas sensor in quartz-enhanced photoacoustic spectroscopy based on time-division multiplexing (TDM) technology of a distributed-feedback (DFB) laser driver current was proposed and experimentally demonstrated. The quartz tuning-fork-based photoacoustic spectroscopy (PAS) cell configuration with two optical collimators and two acoustic microresonators was designed to detect the second-harmonic (${2}f$2f) PAS signal. The two optical collimators guaranteed that the two laser beams would inject the PAS cell conveniently, providing higher power input than a 3 dB optical fiber coupler.

3D aluminum/silver hierarchical nanostructure with large areas of dense hot spots for surface-enhanced raman scattering.

Plasmonic nanomaterials possessing large-volume, high-density hot spots with high field enhancement are highly desirable for ultrasensitive surface-enhanced Raman scattering (SERS) sensing. However, many as-prepared plasmonic nanomaterials are limited in available dense hot spots and in sample size, which greatly hinder their wide applications in SERS devices. Here, we develop a two-step physical deposition protocol and successfully fabricate 3D hierarchical nanostructures with highly dense hot spots across a large scale (6 × 6 cm ).

Bioscaffold arrays decorated with Ag nanoparticles as a SERS substrate for direct detection of melamine in infant formula.

Three-dimensional (3D) plasmonic structures have been intensively investigated as high performance surface enhanced Raman scattering (SERS) substrates. Here, we demonstrate a 3D biomimetic SERS substrate prepared by deposition of silver nanoparticles (Ag NPs) on the bioscaffold arrays of cicada wings using laser molecular beam epitaxy. This deposition method can offer a large number of nanoparticles with average diameter of ∼10 nm and nanogaps of sub-10 nm on the surface of chitin nanopillars to generate a high density of hotspots.

Combined study of the ground and excited states in the transformation of nanodiamonds into carbon onions by electron energy-loss spectroscopy.

The electron momentum density and sp/sp ratio of carbon materials in the thermal transformation of detonation nanodiamonds (ND) into carbon nano-onions are systematically studied by electron energy-loss spectroscopy (EELS). Electron energy-loss near-edge structures of the carbon K-ionization in the electron energy-loss spectroscopy are measured to determine the sp content of the ND-derived samples. We use the method developed by Titantah and Lamoen, which is based on the ability to isolate the π spectrum and has been shown to give reliable and accurate results.