Resource efficient single photon source based on active frequency multiplexing.

We propose a new, to the best of our knowledge, single photon source based on the principle of active multiplexing of heralded single photons, which, unlike previously reported architecture, requires a limited amount of physical resources. We discuss both its feasibility and the purity and indistinguishability of single photons as a function of the key parameters of a possible implementation.

Gold-induced photothermal background in on-chip surface enhanced stimulated Raman spectroscopy.

Surface enhanced Raman spectroscopy (SERS) and stimulated Raman spectroscopy (SRS) are well established techniques capable of boosting the strength of Raman scattering. The combination of both techniques (surface enhanced stimulated Raman spectroscopy, or SE-SRS) has been reported using plasmonic nanoparticles. In parallel, waveguide enhanced Raman spectroscopy has been developed using nanophotonic and nanoplasmonic waveguides.

Mitigation of photon background in nanoplasmonic all-on-chip Raman sensors.

In the quest for a more compact and cheaper Raman sensor, photonic integration and plasmonic enhancement are central. Nanoplasmonic slot waveguides exhibit the benefits of SERS substrates while being compatible with photonic integration and mass-scale (CMOS) fabrication. A difficulty in pursuing further integration of the Raman sensor with lasers, spectral filters, spectrometers and interconnecting waveguides lies in the presence of a photon background generated by the excitation laser field in any dielectric waveguide constituting those elements.

Plasma-Enhanced Atomic Layer Deposition of Nanostructured Gold Near Room Temperature.

A plasma-enhanced atomic layer deposition (PE-ALD) process to deposit metallic gold is reported, using the previously reported MeAu(PMe) precursor with H plasma as the reactant. The process has a deposition window from 50 to 120 °C with a growth rate of 0.030 ± 0.

High index contrast photonic platforms for on-chip Raman spectroscopy.

Nanophotonic waveguide enhanced Raman spectroscopy (NWERS) is a sensing technique that uses a highly confined waveguide mode to excite and collect the Raman scattered signal from molecules in close vicinity of the waveguide. The most important parameters defining the figure of merit of an NWERS sensor include its ability to collect the Raman signal from an analyte, i.e.

Strong Nonlinear Coupling in a Si_{3}N_{4} Ring Resonator.

We demonstrate that nondegenerate four-wave mixing in a Si_{3}N_{4} microring resonator can result in a nonlinear coupling rate between two optical fields exceeding their energy dissipation rate in the resonator, corresponding to strong nonlinear coupling. We demonstrate that this leads to a Rabi-like splitting, for which we provide a theoretical description in agreement with our experimental results. This yields new insight into the dynamics of nonlinear optical interactions in microresonators and access to novel phenomena.

Integrated silicon nitride electro-optic modulators with atomic layer deposited overlays.

Silicon nitride (SiN) is currently the most prominent CMOS-compatible platform for photonics at wavelengths <1  μm. However, realizing fast electro-optic (EO) modulators, the key components of any integrated optics platform, remains challenging in SiN. Modulators based on the plasma dispersion effect, as in silicon, are not available.

All-optically tunable buffer for single photons.

We demonstrate a photon buffer for quantum communication systems via a quantum frequency conversion-dispersion technique based on Bragg scattering four-wave mixing. The all-fiber setup is capable of imparting all-optical and continuously tunable delays onto single photons with minimal photon noise and absorption. Tunable delays up to 23 times the photon duration are demonstrated with on/off efficiencies as high as 55%.

Stimulated Raman spectroscopy of analytes evanescently probed by a silicon nitride photonic integrated waveguide.

We report, to the best of our knowledge, the first demonstration of stimulated Raman spectroscopy enhanced by a nanophotonic integrated circuit. The Raman response of low-concentration dimethyl sulfoxide is evanescently probed via centimeter-long wire waveguides. A signal enhancement of close to five orders of magnitude, as compared to the case of on-chip spontaneous Raman scattering, is demonstrated.

Frequency multiplexing for quasi-deterministic heralded single-photon sources.

Parametric single-photon sources are well suited for large-scale quantum networks due to their potential for photonic integration. Active multiplexing of photons can overcome the intrinsically probabilistic nature of these sources, resulting in near-deterministic operation. However, previous implementations using spatial and temporal multiplexing scale unfavorably due to rapidly increasing switching losses.

On the determination of χ in thin films: a comparison of one-beam second-harmonic generation measurement methodologies.

The determination of the second-order susceptibility (χ) of thin film samples can be a delicate matter since well-established χ measurement methodologies such as the Maker fringe technique are best suited for nonlinear materials with large thicknesses typically ranging from tens of microns to several millimeters. Here we compare two different second-harmonic generation setups and the corresponding measurement methodologies that are especially advantageous for thin film χ characterization. This exercise allows for cross-checking the χ obtained for identical samples and identifying the main sources of error for the respective techniques.

Ramsey Interference with Single Photons.

Interferometry using discrete energy levels of nuclear, atomic, or molecular systems is the foundation for a wide range of physical phenomena and enables powerful techniques such as nuclear magnetic resonance, electron spin resonance, Ramsey-based spectroscopy, and laser or maser technology. It also plays a unique role in quantum information processing as qubits may be implemented as energy superposition states of simple quantum systems. Here, we demonstrate quantum interference involving energy states of single quanta of light.

Single mode waveguide platform for spontaneous and surface-enhanced on-chip Raman spectroscopy.

We review an on-chip approach for spontaneous Raman spectroscopy and surface-enhanced Raman spectroscopy based on evanescent excitation of the analyte as well as evanescent collection of the Raman signal using complementary metal oxide semiconductor (CMOS)-compatible single mode waveguides. The signal is either directly collected from the analyte molecules or via plasmonic nanoantennas integrated on top of the waveguides. Flexibility in the design of the geometry of the waveguide, and/or the geometry of the antennas, enables optimization of the collection efficiency.

Continuous generation of rubidium vapor in hollow-core photonic bandgap fibers.

We demonstrate high optical depths (50±5) that last for hours in rubidium-filled hollow-core photonic bandgap fibers, which represent a 1000× improvement over the operation times previously reported. We investigate the vapor generation mechanism using both a continuous wave and a pulsed light source, and find that the mechanism for generating the rubidium atoms is primarily due to thermal vaporization. The continuous generation of large vapor densities should enable measurements at the single-photon level by averaging over longer time scales.

Atomic layer deposited second-order nonlinear optical metamaterial for back-end integration with CMOS-compatible nanophotonic circuitry.

We report the fabrication of artificial unidimensional crystals exhibiting an effective bulk second-order nonlinearity. The crystals are created by cycling atomic layer deposition of three dielectric materials such that the resulting metamaterial is noncentrosymmetric in the direction of the deposition. Characterization of the structures by second-harmonic generation Maker-fringe measurements shows that the main component of their nonlinear susceptibility tensor is about 5 pm/V, which is comparable to well-established materials and more than an order of magnitude greater than reported for a similar crystal [Appl.

Efficiency of evanescent excitation and collection of spontaneous Raman scattering near high index contrast channel waveguides.

We develop and experimentally verify a theoretical model for the total efficiency η0 of evanescent excitation and subsequent collection of spontaneous Raman signals by the fundamental quasi-TE and quasi-TM modes of a generic photonic channel waveguide. Single-mode silicon nitride (Si3N4) slot and strip waveguides of different dimensions are used in the experimental study. Our theoretical model is validated by the correspondence between the experimental and theoretical absolute values within the experimental errors.

Visible-to-near-infrared octave spanning supercontinuum generation in a silicon nitride waveguide.

The generation of an octave spanning supercontinuum covering 488-978 nm (at -30  dB) is demonstrated for the first time on-chip. This result is achieved by dispersion engineering a 1-cm-long Si3N4 waveguide and pumping it with an 100-fs Ti:Sapphire laser emitting at 795 nm. This work offers a bright broadband source for biophotonic applications and frequency metrology.

Strong polarization mode coupling in microresonators.

We observe strong modal coupling between the TE00 and TM00 modes in Si3N4 ring resonators revealed by avoided crossings of the corresponding resonances. Such couplings result in significant shifts of the resonance frequencies over a wide range around the crossing points. This leads to an effective dispersion that is one order of magnitude larger than the intrinsic dispersion and creates broad windows of anomalous dispersion.

Frequency translation via four-wave mixing Bragg scattering in Rb filled photonic bandgap fibers.

We demonstrate frequency translation at microwatt pump power levels in Rubidium vapor confined to a hollow-core photonic bandgap fiber using four-wave mixing Bragg scattering. The 5S(1/2)→5D(3/2) two-photon transition in 85Rb is employed for the four-wave mixing process. Using continuous-wave pump beams at 780 and 795 nm, a weak signal beam at 776 nm is translated to a wavelength of 762 nm with a 21% conversion efficiency at pump powers of 300 μW.

Silicon-on-insulator integrated source of polarization-entangled photons.

We report the experimental generation of polarization-entangled photons at telecommunication wavelengths using spontaneous four-wave mixing in silicon-on-insulator wire waveguides. The key component is a 2D coupler that transforms path entanglement into polarization entanglement at the output of the device. Using quantum state tomography we find that the produced state has fidelity 88% with a pure nonmaximally entangled state.

Nonlinear properties of and nonlinear processing in hydrogenated amorphous silicon waveguides.

We propose hydrogenated amorphous silicon nanowires as a platform for nonlinear optics in the telecommunication wavelength range. Extraction of the nonlinear parameter of these photonic nanowires reveals a figure of merit larger than 2. It is observed that the nonlinear optical properties of these waveguides degrade with time, but that this degradation can be reversed by annealing the samples.

On-chip parametric amplification with 26.5 dB gain at telecommunication wavelengths using CMOS-compatible hydrogenated amorphous silicon waveguides.

We present what we believe to be the first study of parametric amplification in hydrogenated amorphous silicon waveguides. Broadband on/off amplification up to 26.5 dB at telecom wavelength is reported.

Generation of correlated photons in hydrogenated amorphous-silicon waveguides.

We report the first (to our knowledge) observation of correlated photon emission in hydrogenated amorphous-silicon waveguides. We compare this to photon generation in crystalline silicon waveguides with the same geometry. In particular, we show that amorphous silicon has a higher nonlinearity and competes with crystalline silicon in spite of higher loss.

Continuous wave photon pair generation in silicon-on-insulator waveguides and ring resonators.

Silicon waveguides are promising chi(3)-based photon pair sources. Demonstrations so far have been based on picosecond pulsed lasers. Here, we present the first investigation of photon pair generation in silicon waveguides in a continuous regime.