ACS Appl Mater Interfaces
February 2025
Flexible bioelectronic devices, which can directly detect various external stimuli or biosignals and communicate the information to the users, have been broadly investigated due to the increasing demand for wearable devices. Among them, alternating-current electroluminescence (ACEL) devices are proposed as sensitive sensing systems for various targets, such as fingerprints. Herein, we propose a method for preparing high-performance ACEL devices by using an Ag electrode, polyethylene terephthalate (PET) substrate, FKM/EMI ionogel, and ZnS:Cu/BaTiO/Ecoflex emissive layer.
View Article and Find Full Text PDFConformable, sensitive, long-lasting, external power supplies-free multifunctional electronics are highly desired for personal healthcare monitoring and artificial intelligence. Herein, we report a series of stretchable, skin-like, self-powered tactile and motion sensors based on single-electrode mode triboelectric nanogenerators. The triboelectric sensors were composed of ultraelastic polyacrylamide (PAAm)/(polyvinyl pyrrolidone) PVP/(calcium chloride) CaCl conductive hydrogels and surface-modified silicon rubber thin films.
View Article and Find Full Text PDFConductive hydrogels are widely used in sports monitoring, healthcare, energy storage, and other fields, due to their excellent physical and chemical properties. However, synthesizing a hydrogel with synergistically good mechanical and electrical properties is still challenging. Current fabrication strategies are mainly focused on the polymerization of hydrogels with a single component, with less emphasis on combining and matching different conductive hydrogels.
View Article and Find Full Text PDFRobust conductive hydrogels are in great demand for the practical applications of smart soft robots, epidermal electronics, and human-machine interactions. We successfully prepared nanoparticles enhanced polyacrylamide/hydroxypropyl guar gum/acryloyl-grafted chitosan quaternary ammonium salt/calcium ions/SiO nanoparticles (PHC/Ca/SiO NPs) conductive hydrogels. Owing to the stable chemical and physical hybrid crosslinking networks and reversible non-covalent interactions, the PHC/Ca/SiO NPs conductive hydrogel showed good conductivity (~3.
View Article and Find Full Text PDFTransparent, conductive hydrogels with good mechanical strength and toughness are in great demand of the fields of biomedical and future wearable smart electronics. We reported a carboxymethyl chitosan (CMCS)-calcium chloride (CaCl)/polyacrylamide (PAAm)/poly(N-methylol acrylamide (PNMA) transparent, tough and conductive hydrogel containing a bi-physical crosslinking network through in situ free radical polymerization. It showed excellent light transmittance (>90%), excellent toughness (10.
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