ACS Appl Mater Interfaces
October 2024
A smart window that dynamically regulates light transmittance is crucial for modern life end-users and promising for on-demand optical devices. The advent of three-dimensional (3D) photonic crystal microspheres has enriched the functions of a smart window. However, the smart window formed by polymer microspheres encounters poor mechanical strength and microstructural defects.
View Article and Find Full Text PDFWe propose a type of reflectionless graphene perfect absorber (GPA) in which the reflection channel is forbidden, while the transmission channel is open. Peak absorption of 99.97% in the near-infrared is numerically demonstrated for monolayer graphene loaded on a one-dimensional silicon photonic crystal slab with rhomboid cross sections that supports parity symmetric unidirectional guided resonances (UGRs).
View Article and Find Full Text PDFA typical optomechanical system is a cavity with one movable mirror and one fixed mirror. However, this configuration has been considered incapable of integrating sensitive mechanical elements while maintaining high cavity finesse. Although the membrane-in-the-middle solution seems to be able to overcome this contradiction, it introduces additional components that will lead to unexpected insertion loss, resulting in reduced cavity quality.
View Article and Find Full Text PDFWe theoretically propose a broadband transverse unidirectional scattering scheme based on the interaction between a tightly focused azimuthally polarized beam (APB) and a silicon hollow nanostructure. When the nanostructure is located at a specific position in the focal plane of the APB, the transverse scattering fields can be decomposed into contributions from transverse components of the electric dipoles, longitudinal components of magnetic dipoles and magnetic quadrupole components. In order to satisfy the transverse Kerker conditions for these multipoles within a wide infrared spectrum, we design a novel nanostructure with hollow parallelepiped shape.
View Article and Find Full Text PDFA kind of graphene-based perfect absorber which can generate low-threshold and high-extinction-ratio optical bistability in the near-IR band is proposed and simulated with numerical methods. The interaction between input light and monolayer graphene in the absorber can be greatly enhanced due to the perfect absorption. The large nonlinear coefficient of graphene and the strong light-graphene interaction contribute to the nonlinear response of the structure, leading to relatively low switching thresholds of less than 2.
View Article and Find Full Text PDFIn the paper, a type of phase change metamaterial for tunable infrared stealth and camouflage is proposed and numerically studied. The metamaterial combines high temperature resistant metal Mo with phase-changing material GST and can be switched between the infrared "stealthy" and "non-stealthy" states through the phase change process of the GST. At the amorphous state of GST, there is a high absorption peak at the atmospheric absorption spectral range, which can achieve infrared stealth in the atmospheric window together with good radiative heat dissipation in the non-atmospheric window.
View Article and Find Full Text PDFThe high saturation current density and ultrafast heating modulation of graphene makes it a competitive candidate for future thermal emission source. However, the low emissivity and easy oxidation under high temperature in air limit graphene application in the spectral range from the visible to near infrared. Here, we report a visible graphene thermal emitter based on the metal Fabry-Pérot (FP) cavity, which can greatly enhance the emissivity of graphene at wavelength around 637 nm and protect graphene from oxidation.
View Article and Find Full Text PDFSince the discovery of the quantum Hall effect in 1980, it has attracted intense interest in condensed matter physics and has led to a new type of metrological standard by utilizing the resistance quantum. Graphene, a true two-dimensional electron gas material, has demonstrated the half-integer quantum Hall effect and composite-fermion fractional quantum Hall effect due to its unique massless Dirac fermions and ultra-high carrier mobility. Here, we use a monolayer graphene encapsulated with hexagonal boron nitride and few-layer graphite to fabricate micrometer-scale graphene Hall devices.
View Article and Find Full Text PDFA very attractive advantage of graphene is that its Fermi level can be regulated by electrostatic bias doping. It is of great significance to investigate and control the spatial location of graphene emission for graphene thermal emitters, in addition to tuning the emission intensity and emission spectrum. Here, we present a detailed theoretical model to describe the graphene emission characteristics versus gate voltages.
View Article and Find Full Text PDFTwo-dimensional (2D) materials have got extensive attention for multifunctional device applications in advanced nanoelectronics and optoelectronics, such as field-effect transistors, photodiodes, and solar cells. In our work, we fabricated MoTe-MoS van der Waals heterostructure photodetectors with great performance using the mechanical exfoliation method and restack technique. It is demonstrated that our MoTe-MoS heterostructure photodetector device can operate without bias voltage, possessing a low dark current (10 pA) and high photocurrent on/off ratio (>10).
View Article and Find Full Text PDFA key process in electrochemical energy technology is hydrogen evolution reaction (HER). However, its electrochemical properties mainly depend on the catalytic activity of the material itself. Therefore, it is important to find efficient electrocatalysts to realize clean hydrogen production.
View Article and Find Full Text PDFThe number of active sites and stability of the structure of electrocatalysts are the key factors in the process of overall water splitting. In this paper, cobalt-sulfide-selenium (Se:CoS) core-shell nanostructures are prepared by a simple two-step method, including hydrothermal reaction and chemical vapor deposition. The resulting product exhibits excellent electrochemical performance, owing to the synergistic effects between CoS and CoSe, as well as the plentiful active sites in the electrode structure.
View Article and Find Full Text PDFWe theoretically present a high-efficiency switchable reflective terahertz polarization converter composed of a periodic array of rectangular-shaped metal-dielectric-graphene sandwich structure on a dielectric substrate supported by a thick metallic film. Graphene sheet together with the rectangular-shaped metal patch provides tunable anisotropic hybrid magnetic plasmon resonance to obtain tunable phase delay of 90° and 180°, corresponding to a quarter-wave plate (QWP) and half-wave plate (HWP), respectively. Results of numerical simulations indicate that the proposed structure can switch functions between a QWP and HWP at a certain frequency simply by adjusting the Fermi energy of graphene.
View Article and Find Full Text PDFIn general, the functions of most metalenses cannot be adjusted dynamically after being fabricated. Here, we theoretically propose an electrically tunable metalens composed of single-layered and non-structured doped graphene loaded with ribbon-shaped metallic strip arrays with varied widths and gaps. The combination of the different widths and gaps can provide full phase coverage from 0 to 2π, which is necessary for a plane wave to be focused.
View Article and Find Full Text PDFConsiderably subtle vibrations can be detected by light signals. Commonly, this is achieved based on the phase change of light that can be attributed to the vibration of a movable mirror, which has been used in gravitational wave detection. For a homogeneous dielectric membrane, the thinner the membrane, the greater the membrane vibration amplitude will be with respect to the sound pressure.
View Article and Find Full Text PDFElectromagnetically induced transparency (EIT) arises from the coherent coupling and interference between a superradiant (bright) mode in one resonator and a subradiant (dark) mode in an adjacent resonator. Generally, the two adjacent resonators are structurally or spatially asymmetric. Here, by numerical simulation, we demonstrate that tunable EIT can be induced by graphene ribbon pairs without structurally or spatially asymmetry.
View Article and Find Full Text PDFGraphene has unique properties which make it an ideal material for photonic and optoelectronic devices. However, the low light absorption in monolayer graphene seriously limits its practical applications. In order to greatly enhance the light absorption of graphene, many graphene-based structures have been developed to achieve perfect absorption of incident waves.
View Article and Find Full Text PDFBroadband optical absorption structures in the near infrared by coupling monolayer-graphene with periodical metal structures are proposed and demonstrated numerically. Optical absorption of graphene with over-50%-absorption bandwidth up to hundreds of nanometer caused by magnetic dipole resonances and magnetic coupling effect are investigated in detail, and the demonstrated bandwidths are one order higher than those caused by dielectric guiding mode resonances. In addition, the influences of geometrical parameters of structures are fully analyzed and these demonstrated structures show angular-insensitive absorption for oblique incidence in a large angular range.
View Article and Find Full Text PDFIn general, there is a fundamental trade-off between the operational bandwidth and the attainable absorption. So, obtaining broadband wave absorption of a low reference standard such as 90% is not very difficult. However, when trying to obtain higher absorption such as 99%, the bandwidth will drop dramatically.
View Article and Find Full Text PDFWe propose a broadband terahertz absorber consisting of nonstructured graphene loaded with arrays of elliptic dielectric cylinders. The relative bandwidth for the absorption above 90% reaches about 65%. The working mechanism of broad bandwidth mainly comes from two aspects.
View Article and Find Full Text PDFWe present a wave absorption design consisting of periodical arrays of dielectric bricks on the dielectric substrate, which is coated with single-layered and nonstructured graphene, supported by a thick piece of metal. The design is demonstrated to broadband near-perfect absorption with 0.82 terahertz (THz) bandwidth of over 90% absorption and with central frequency of 1.
View Article and Find Full Text PDFWe show numerically that both coherent perfect absorption and transparency can be realized in a monolayer graphene. The graphene film, doped and patterned with a periodical array of holes, can support plasmonic resonances in the Mid-infrared range. Under the illumination of two counter-propagating coherent optical beams, resonant optical absorption may be tuned continuously from 99.
View Article and Find Full Text PDFWe achieve a broadband unidirectional transmission or One-way diffraction grating by cascading two parallel gratings made of isotropic material with different periods. In order to significantly reduce the reciprocal transmission of the zero order, one of them is chosen to be a subwavelength grating and designed as a wideband reflector for the incident-wave. It is demonstrated that more than 65 percent of the incident-wave energy can be transmitted unidirectionally with less than 0.
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