Active road noise control (ARNC) systems have been widely investigated for low-frequency road noise attenuation in vehicle cabins. Multiple reference and error sensors are usually required to ensure noticeable noise reduction. However, this tends to slow down the convergence speed of adaptive algorithms due to the coupling of secondary paths and the cross correlation of reference signals.
View Article and Find Full Text PDFNumerous advanced and lightweight signal processing methods have been presented for single-channel speech enhancement (SE). It is imperative to carefully explore how to efficiently combine, integrate, and balance these methods. This paper proposes a more effective and less resource-intensive SE system, focused on the integration and adaptation of several approaches, especially the temporal cepstrum smoothing (TCS).
View Article and Find Full Text PDFThe recently proposed semi-blind source separation (SBSS) method for nonlinear acoustic echo cancellation (NAEC) outperforms adaptive NAEC in attenuating the nonlinear acoustic echo. However, the multiplicative transfer function (MTF) approximation makes it unsuitable for real-time applications, especially in highly reverberant environments, and the natural gradient makes it hard to balance well between fast convergence speed and stability. In this paper, two more effective SBSS methods based on auxiliary-function-based independent vector analysis (AuxIVA) and independent low-rank matrix analysis (ILRMA) are proposed.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2021
The dramatic growth of the sodium-ion battery market evokes a high demand for high-performance cathodes. In this work, a nanosized amorphous FePO@rGO composite is developed using coprecipitation combined with low-temperature hydrothermal synthesis, which registered a surface area of 179.43 m g.
View Article and Find Full Text PDFTransition metal phosphides (TMPs) have received considerable attention owing to their great potential in energy conversion and storage technologies. Elaborate design and synthesis of various TMPs with abundant structures in order to meet the requirements of various applications is one of the major goals and challenges of sustainable chemistry. In this work, an electrostatic spray deposition (ESD) approach has been developed and has been demonstrated to be a general strategy to fabricate TMPs for the first time.
View Article and Find Full Text PDFDeveloping high power-high energy electrochemical energy storage systems is an ultimate goal in the energy storage field, which is even more difficult but significant for low-cost sodium ion batteries. Here, fluoride is successfully prepared by the electrostatic spray deposition (ESD) technique, which greatly expands the application scope of ESD. A two-step strategy (solvothermal plus ESD method) is proposed to construct a bicontinuous ordered network of 3D porous Na (VO) (PO ) F/reduced graphene oxide (NVOPF/rGO).
View Article and Find Full Text PDFNiobium-based oxides including Nb O , TiNb O compounds, M-Nb-O (M = Cr, Ga, Fe, Zr, Mg, etc.) family, etc., as the unique structural merit (e.
View Article and Find Full Text PDFThe development of advanced electrode materials for various energy-storage systems, especially the fabrication of designed structures and morphologies of electrode materials, has attracted intense interest in both the academic and industrial fields. Among the various synthesis methods, electrostatic spray deposition (ESD) is a simple but versatile approach, by which materials can be fabricated with various morphologies, such as granular, dense, and porous, in an easily controllable manner. Herein, motivated by the rapid advancements of the given technology, a comprehensive introduction of ESD is provided, with emphasis on the kinds of materials and the types of morphology that can be obtained, along with the important control parameters.
View Article and Find Full Text PDFDeveloping high-performance, affordable, and durable batteries is one of the decisive technological tasks of our generation. Here, we review recent progress in understanding how to optimally arrange the various necessary phases to form the nanoscale structure of a battery electrode. The discussion begins with design principles for optimizing electrode kinetics based on the transport parameters and dimensionality of the phases involved.
View Article and Find Full Text PDFAim: ) play important roles in occurrence and development of osteosarcoma. Previous studies had verified the role of ) in various diseases, especially in cancers. Our purpose in this study was to investigate the values of in development and prognosis of osteosarcoma.
View Article and Find Full Text PDFTransition metal sulfides have a great potential for energy storage due to the pronouncedly higher capacity (owing to conversion to metal or even alloy) than traditional insertion electrode materials. However, the poor cycling stability still limits the development and application in lithium and sodium ion batteries. Here, taking SnS as a model material, a novel general strategy is proposed to fabricate a 3D porous interconnected metal sulfide/carbon nanocomposite by the electrostatic spray deposition technique without adding any expensive carbonaceous materials such as graphene or carbon nanotube.
View Article and Find Full Text PDFA 3D tricontinuous Na3 V2 (PO4 )3 :reduced graphene oxide-carbon nanotube cathode is directly deposited on the current collector without any conductive additives or binders by a facile electrostatic spray deposition (ESD) technique. Such an electrode displays excellent rate capability and long cycling stability, which is rather typical of supercapacitors but is connected here with the much higher energy density of an efficient battery electrode.
View Article and Find Full Text PDFMuch attention has been paid to metastable materials in the lithium battery field, especially to nanocrystalline and amorphous materials. Nonetheless, fundamental issues such as lithium potential variations have not been pertinently addressed. Using LiFePO4 as a model system, we inspect such lithium potential variations for various lithium storage modes and evaluate them thermodynamically.
View Article and Find Full Text PDFGermanium-based materials (Ge and GeOx) have recently demonstrated excellent lithium-ion storage ability and are being considered as the most promising candidates to substitute commercial carbon-based anodes of lithium-ion batteries. Nevertheless, practical implementation of Ge-based materials to lithium-ion batteries is greatly hampered by the poor cyclability that resulted from the huge volume variation during lithiation/delithiation processes. Herein, uniform carbon-encapsulated Ge and GeOx nanowires were synthesized by a one-step controlled pyrolysis of organic-inorganic hybrid GeOx/ethylenediamine (GeOx/EDA) nanowires in H2/Ar and Ar atmospheres, respectively.
View Article and Find Full Text PDFWe report on a new ultrafast solid electrolyte of the composition Li11Si2PS12, which exhibits a higher room-temperature Li ion diffusivity than the present record holder Li10GeP2S12. We discuss the high-pressure synthesis and ion dynamics of tetragonal Li11Si2PS12, and comparison is made with our investigations of related members of the LMePS family, i.e.
View Article and Find Full Text PDFSodium ion batteries are one of the realistic promising alternatives to the lithium analogues. However, neither theoretical energy/power density nor the practical values reach the values of Li cathodes. Poorer performance is expected owing to larger size, larger mass, and lower cell voltage.
View Article and Find Full Text PDFThe preparation and electrochemical storage behavior of MoS2 nanodots--more precisely single-layered ultrasmall nanoplates--embedded in carbon nanowires has been studied. The preparation is achieved by an electrospinning process that can be easily scaled up. The rate performance and cycling stability of both lithium and sodium storage were found to be outstanding.
View Article and Find Full Text PDFComp Biochem Physiol Part D Genomics Proteomics
September 2012
Next-generation sequencing (NGS) has proven a valuable platform for fast and easy obtaining of large numbers of sequences at relatively low cost. In this study we use shot-gun sequencing method on Illumina HiSeq 2000, to obtain enough sequences for the assembly of the bryozoan Membranipora grandicella (Bryozoa: Cheilostomatida) mitochondrial genome, which is the first representative of the suborder Malacostegina. The complete mitochondrial genome is 15,861 bp in length, which is relatively larger than other studied bryozoans.
View Article and Find Full Text PDFLarge single crystals of LiFePO(4) have been chemically delithiated. The relevance of chemical oxidation in comparison with electrochemical delithiation is discussed. Analyses of the Li content and profiles were done by electron energy loss spectroscopy and secondary ion mass spectrometry.
View Article and Find Full Text PDFLithium ions in LiFePO(4) were observed directly at atomic resolution by an aberration-corrected annular-bright-field scanning transmission electron microscopy technique. In addition, it was found in partially delithiated LiFePO(4) that the remaining lithium ions preferably occupy every second layer, along the b axis, analogously to the staging phenomenon observed in some layered intercalation compounds. This new finding challenges previously proposed LiFePO(4)/FePO(4) two-phase separation mechanisms.
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