Phase separation has important implications for the mechanical, thermal, and electrical properties of materials. Weightless conditions prevent buoyancy and sedimentation from affecting the dynamics of phase separation and the morphology of the domains. In our experiments, sulfur hexafluoride (SF6) was initially heated about 1K above its critical temperature under microgravity conditions and then repeatedly quenched using temperature steps, the last one being of 3.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
December 2012
Large density fluctuations were observed by illuminating a cylindrical cell filled with sulfur hexafluoride (SF(6)), very near its liquid-gas critical point (|T-T(c)|< 300 μK) and recorded using a microscope with 3 μm spatial resolution. Using a dynamic structure factor algorithm, we determined from the recorded images the structure factor (SF), which measures the spatial distribution of fluctuations at different moments, and the correlation time of fluctuations. This method authorizes local measurements in contrast to the classical scattering techniques that average fluctuations over the illuminating beam.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
May 2008
We present both the experimental and computational methods and results of phase-separating experiments performed with sulfur hexafluoride (SF6) close to its critical density. These experiments were performed in microgravity to suppress buoyancy and convection-driven effects. Phase separation under reduced gravity is analyzed for both 0.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
September 2005
By performing near-critical fluid experiments in the weightlessness of an orbiting space vehicle, we have suppressed buoyancy-driven flows and gravitational constraints on the liquid-gas interface of a large gas bubble. At equilibrium, the liquid completely wets the walls of a cylindrical cell, and the bubble is pushed to the sidewall. In these experiments the system's temperature T is increased at a constant rate past the critical temperature T(C), pushing it slightly out of equilibrium.
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