Stretchable ionotronics have drawn increasing attention during the past decade, enabling myriad applications in engineering and biomedicine. However, existing ionotronic sensors suffer from limited sensing capabilities due to simple device structures and poor stability due to the leakage of ingredients. In this study, we rationally design and fabricate a plethora of architected leakage-free ionotronic sensors with multi-mode sensing capabilities, using DLP-based 3D printing and a polyelectrolyte elastomer.
View Article and Find Full Text PDFThe emergence of hydrophobic ionogels composed of hydrophobic polymer matrices and hydrophobic ionic liquids has drastically broadened the applications of ionic devices, especially for underwater explorations. Compared with traditional ionogels, hydrophobic ones are capable of achieving long-term stability in ambient and aqueous environments. In this review, the latest research developments of intrinsically hydrophobic ionogels are summarized, with particular emphases placed on the materials, mechanisms and applications.
View Article and Find Full Text PDFEutectogels are stretchable ionic conductors extensively developed in recent years, owing to their distinct advantages of low cost, non-volatility, non-toxicity, and outstanding biocompatibility. However, the susceptibility to humidity caused by the exchange of water molecules between the interiors of eutectogels and the external environment greatly restricts their practical applications. Here, a dip-coating strategy is proposed to fabricate a P(MEA--IBA) elastomer-coated P(AAC--AAM) eutectogel to achieve satisfactory humidity-resistant capability.
View Article and Find Full Text PDFDeveloping advanced materials for highly secure data-encryption is crucial but very challenging, as most data-encryption materials (the message area) are chemically different from the substrates (the background) on which they are being written, leading to high risks of data leakage by deciphering sophisticated instrumental analysis. Additionally, most materials require only one stimulus for decryption, resulting in a low-level of data-security. Here, a three configurational isomer-based data-encryption method is developed (, propylamine, isopropylamine, and cyclopropylamine).
View Article and Find Full Text PDFNumerous emerging applications in modern society require humidity sensors that are not only sensitive and specific but also durable and intelligent. However, conventional humidity sensors do not have all of these simultaneously because they require very different or even contradictory design principles. Here, inspired by camel noses, we develop a porous zwitterionic capacitive humidity sensor.
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