Publications by authors named "C Diddens"

A uniform solidification front undergoes nontrivial deformations when encountering an insoluble dispersed particle in a melt. For solid particles, the overall deformation characteristics are primarily dictated by heat transfer between the particle and the surrounding, remaining unaffected by the rate of approach of the solidification front. In this Letter we show that, conversely, when interacting with a droplet or a bubble, the deformation behavior exhibits entirely different and unexpected behavior.

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Correction for 'Evaporation-driven liquid flow in sessile droplets' by Hanneke Gelderblom , , 2022, , 8535-8553, https://doi.org/10.1039/D2SM00931E.

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The evaporation of a sessile droplet spontaneously induces an internal capillary liquid flow. The surface-tension driven minimisation of surface area and/or surface-tension differences at the liquid-gas interface caused by evaporation-induced temperature or chemical gradients set the liquid into motion. This flow drags along suspended material and is one of the keys to control the material deposition in the stain that is left behind by a drying droplet.

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The transport and aggregation of particles in suspensions is an important process in many physicochemical and industrial processes. In this work, we study the transport of particles in an evaporating binary droplet. Surprisingly, the accumulation of particles occurs not only at the contact line (due to the coffee-stain effect) or at the solid substrate (due to sedimentation) but also at a particular radial position near the liquid-air interface, forming a "ring", which we term as the .

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Hypothesis: Thermal Marangoni flow in evaporating sessile water droplets is much weaker in experiments than predicted theoretically. Often this is attributed to surfactant contamination, but there have not been any in-depth analyses that consider the full fluid and surfactant dynamics. It is expected that more insight into this problem can be gained by using numerical models to analyze the interplay between thermal Marangoni flow and surfactant dynamics in terms of dimensionless parameters.

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