Controlled oligomerization of [1.1.1]propellane through radical polarity matching: selective synthesis of SF- and CFSF-containing [2]staffanes.

Selectivity in radical chain oligomerizations involving [1.1.1]propellane - i.

Overcoming a Radical Polarity Mismatch in Strain-Release Pentafluorosulfanylation of [1.1.0]Bicyclobutanes: An Entryway to Sulfone- and Carbonyl-Containing SF-Cyclobutanes.

The first assortment of achiral pentafluorosulfanylated cyclobutanes (SF-CBs) are now synthetically accessible through strain-release functionalization of [1.1.0]bicyclobutanes (BCBs) using SFCl.

High-power two-color plasma-based THz generation driven by a Tm-doped fiber laser.

We report on the efficient generation of broadband THz radiation based on a two-color gas-plasma scheme. Broadband THz pulses covering the whole THz spectral region, from 0.1-35 THz, are generated.

Pulses of 32 mJ and 158 fs at 20-kHz repetition rate from a spatiotemporally combined fiber laser system.

A high-energy, high-power ultrafast fiber laser system based on spatiotemporal coherent combination is presented. Bursts of eight subsequent chirped-pulse amplification (CPA)-stretched pulses are amplified simultaneously in 16 parallel ytterbium-doped rod-type amplifiers. After spatial and temporal coherent combination of the total 128 amplified pulse replicas into a single pulse, it is compressed in a partially protective-gas-filled CPA compressor.

Continuously tunable high photon flux high harmonic source.

In this work, a continuously tunable extreme ultraviolet source delivering a state-of-the-art photon flux of >10 ph/s/eV spanning from 50 eV to 70 eV is presented. The setup consists of a high-power fiber laser with a subsequent multipass cell followed by a waveguide-based high harmonic generation setup. Spectral tuning over the full line spacing is achieved by slightly adjusting the lasers driving pulse energy, utilizing nonlinear propagation effects and pulse chirping.

Nonlinear pulse compression to 51-W average power GW-class 35-fs pulses at 2-µm wavelength in a gas-filled multi-pass cell.

We report on the generation of GW-class peak power, 35-fs pulses at 2-µm wavelength with an average power of 51 W at 300-kHz repetition rate. A compact, krypton-filled Herriott-type cavity employing metallic mirrors is used for spectral broadening. This multi-pass compression stage enables the efficient post compression of the pulses emitted by an ultrafast coherently combined thulium-doped fiber laser system.

Ultrafast Tm-doped fiber laser system delivering 1.65-mJ, sub-100-fs pulses at a 100-kHz repetition rate.

High-energy, ultrafast, short-wavelength infrared laser sources with high average power are important tools for industrial and scientific applications. Through the coherent combination of four ultrafast thulium-doped rod-type fiber amplifiers, we demonstrate a Tm-doped chirped pulse amplification system with a compressed pulse energy of 1.65 mJ and 167 W of average output power at a repetition rate of 101 kHz.

Gas-plasma-based generation of broadband terahertz radiation with 640 mW average power.

We present a high-power source of broadband terahertz (THz) radiation covering the whole THz spectral region (0.1-30 THz). The two-color gas plasma generation process is driven by a state-of-the-art ytterbium fiber chirped pulse amplification system based on coherent combination of 16 rod-type amplifiers.

Scaling potential of beam-splitter-based coherent beam combination.

The impact of nonlinear refraction and residual absorption on the achievable peak- and average power in beam-splitter-based coherent beam combination is analyzed theoretically. While the peak power remains limited only by the aperture size, a fundamental average power limit is given by the thermo-optical and thermo-mechanical properties of the beam splitter material and its coatings. Based on our analysis, 100 kW average power can be obtained with state-of-the-art optics at maintained high beam quality (M ≤ 1.

Multipass cell for high-power few-cycle compression.

A multipass cell for nonlinear compression to few-cycle pulse duration is introduced composing dielectrically enhanced silver mirrors on silicon substrates. Spectral broadening with 388 W output average power and 776 µJ pulse energy is obtained at 82% cell transmission. A high output beam quality (${{\rm{M}}^2} \lt {1.

Investigation of spatiotemporal output beam profile instabilities from differentially pumped capillaries.

Differentially pumped capillaries, i.e., capillaries operated in a pressure gradient environment, are widely used for nonlinear pulse compression.

1 kW, 10 mJ, 120 fs coherently combined fiber CPA laser system.

An ultrafast fiber chirped-pulse amplification laser system based on a coherent combination of 16 ytterbium-doped rod-type amplifiers is presented. It generates 10 mJ pulse energy at 1 kW average power and 120 fs pulse duration. A partially helium-protected, two-staged chirped-pulse amplification grating compressor is implemented to maintain the close to diffraction-limited beam quality by avoiding nonlinear absorption in air.

Kilowatt-average-power compression of millijoule pulses in a gas-filled multi-pass cell.

We demonstrate the reliable generation of 1-mJ, 31-fs pulses with an average power of 1 kW by post-compression of 200-fs pulses from a coherently combined Yb:fiber laser system in an argon-filled Herriott-type multi-pass cell with an overall compression efficiency of 96%. We also analyze the output beam, revealing essentially no spatiospectral couplings or beam quality loss.

Fiber laser-driven gas plasma-based generation of THz radiation with 50-mW average power.

We present on THz generation in the two-color gas plasma scheme driven by a high-power, ultrafast fiber laser system. The applied scheme is a promising approach for scaling the THz average power but it has been limited so far by the driving lasers to repetition rates up to 1 kHz. Here, we demonstrate recent results of THz generation operating at a two orders of magnitude higher repetition rate.

23 mJ high-power fiber CPA system using electro-optically controlled divided-pulse amplification.

The pulse-energy scaling technique electro-optically controlled divided-pulse amplification is implemented in a high-power ultrafast fiber laser system based on coherent beam combination. A fiber-integrated front end and a multipass-cell-based back end allow for a small footprint and a modular implementation. Bursts of eight pulses are amplified parallel in up to 12 ytterbium-doped large-pitch fiber amplifiers.

Temporal contrast enhancement of energetic laser pulses by filtered self-phase-modulation-broadened spectra.

We present a novel approach for temporal contrast enhancement of energetic laser pulses by filtered self-phase-modulation-broadened spectra. A measured temporal contrast enhancement by at least seven orders of magnitude in a simple setup has been achieved. This technique is applicable to a wide range of laser parameters and poses a highly efficient alternative to existing contrast-enhancement methods.