Publications by authors named "Buchun Si"

Roughly 10 % of the world's arable land is affected by salinization, which significantly reducing crop yields, degrading soil health, and posing a serious threat to food security and ecological stability. High-efficient water-saving irrigation (HEI) technologies have showed positive effects on crop yield, especially with long-term application in salinized soil fields. However, the microbial mechanisms and influential pathways that promote crop yield and reduce salinity under consecutive HEI remain unclear.

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This study developed a comprehensive nitrogen (N) flow model utilizing localized data in 2000-2019. Enhancements were conducted upon previous models: (1) variations in feed N intake of cows across different production phases was considered; (2) N emission in the Intergovernmental Panel on Climate Change (IPCC) and the European Monitoring and Evaluation Program and the European Environment Agency (EMEP/EEA) was incorporated; (3) emission factor (EF) of NH was corrected based on local climate; and (4) field application of manure was excluded from the system boundary to accommodate China's production status. The effects of farm scale (LF, ≥100 heads; SF, <100 heads) and manure management strategies (dry-cleaning and slurry) were considered.

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The global shift toward net-zero emissions necessitates resource recovery from wet waste. In this study, we demonstrate the first feasibility of combining pilot-scale microbial electrolytic cells (MECs) with hydrothermal liquefaction (HTL) for simultaneous post-hydrothermal liquefaction wastewater (PHW) treatment and efficient hydrogen (H₂) production to meet biocrude upgrading requirements. Long-term single reactor operation revealed that fixed anode potential enabled rapid startup, and low catholyte pH and high salinity were effective in suppression of cathodic methanogenesis and acetogenesis - resulting in high current density of 16.

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The co-occurrence of nutrients and pharmaceuticals and personal care products (PPCPs) in sewage effluent can degrade water quality of the receiving watersheds. This study investigated the simultaneous removal of excess nutrients and PPCP contaminants by developing a novel woodchip bioreactor and biochar (B) treatment system. The result revealed that woodchip bioreactors could effectively remove nitrate via a denitrification process and adsorb some PPCPs.

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To overcome the global water shortage, the treated wastewater is increasingly utilized in agricultural irrigation, and thus reducing freshwater consumption and increasing the water sustainability. Drip irrigation technology is the most appropriate irrigation method to utilize these water sources. However, its operating performance is negatively affected by calcium carbonate (CaCO) scaling, which is one of the most dominant precipitations and also closely related to dissolved ions and the hydraulic characteristics inside irrigation systems.

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Article Synopsis
  • - This study evaluates the environmental impacts of pig farm buildings, focusing on their carbon and water footprints through building information modeling (BIM) and operational simulations.
  • - The findings revealed that the operational stage is the primary contributor to carbon (49.3-84.9%) and water footprints (65.5-92.5%), while material production and farm maintenance follow as smaller contributors.
  • - Using aerated concrete for construction could significantly lower both carbon and water footprints, highlighting the potential for sustainable designs in agricultural buildings.
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Substantial levels of antibiotics remain in liquid digestate, posing a significant threat to human safety and the environment. A comprehensive assessment of residual antibiotics in liquid digestate and related removal technologies is required. To this end, this review first evaluates the potential risks of the residual antibiotics in liquid digestate by describing various anaerobic digestion processes and their half-lives in the environment.

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Hydrothermal liquefaction (HTL) is a cost-effective and environment-friendly technology for using biomass to produce bio-crude oil. The critical challenge of HTL is its complicated aqueous product containing high concentrations of organics and diverse toxicants. This paper reports the continuous anaerobic digestion of raw and zeolite-adsorbed Chlorella HTL wastewater using up-flow anaerobic sludge bed reactors.

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Although the world is gradually moving towards renewable energy resources, the coal industry will continue to be a major energy supply sector in the foreseeable future. However, by-products such as coal fly ash (CFA), coal bottom ash (CBA), and boiler slag are generated during coal combustion, and have become a significant environmental concern. There is an urgent need for transdisciplinary efforts in research, policy, and practice to reduce these by-products substantially.

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Microbial stability and evolution are a critical aspect for biosensors, especially in detecting dynamic and emerging anaerobic biohythane production. In this study, two upflow air-cathode chamber microbial fuel cells (UMFCs) were developed for in situ monitoring of the biohydrogen and biomethane reactors under a COD range of 1000-6000 mg/L and 150-1000 mg/L, respectively. Illumina MiSeq sequencing evidenced the dramatic shift of dominant microbial communities in UMFCs from hydrolytic and acidification bacteria (Clostridiaceae_1, Ruminococcaceae, Peptostreptococcaceae) to acetate-oxidizing bacteria (Synergistaceae, Dysgonomonadaceae, Spirochaetaceae).

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Algal bloom microalgae are abundant in polluted water systems, but their biocrude oil production potential via hydrothermal liquefaction (HTL) is limited. This study proposed a novel process that combined biological (dark fermentation) and thermochemical (HTL) techniques aimed at changing the feedstock characteristics to be more suitable for thermochemical conversion, herein named integrated dark fermentation-hydrothermal liquefaction (DF-HTL). DF-HTL conversion of algae significantly enhanced the biocrude oil yield (wt %), carbon content (mol), energy content (MJ), and energy conversion ratios by 9.

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The influence of persulfate assisted hydrothermal carbonization (HTC) (160 °C-220 °C) of spirulina and hydrochar properties was assessed. The elementary composition and proximate analysis of hydrochar were investigated on the carbonization degree and basic fuel properties, and the surface functional groups and morphological characteristics of hydrochar were analyzed as well as thermal stability. Results suggested that persulfate assisted process enhanced the carbonization degree of hydrochar by oxygen reduction (1.

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The influence of co-hydrothermal carbonization (co-HTC) on the hydrochar properties and nutrients distribution derived from food waste (FW) and woody sawdust (WS) blend was assessed. The carbon retention, surface functional groups and morphology features involved in hydrochar were evaluated to study the interaction effects. Results suggested that hydrochar yield consistently decreased with increase of both FW ratio and HTC temperature.

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Bamboo shoot shell (BSS), a major byproduct from bamboo shoot industries with a high amount of output annually, needs to be sustainably management due to its impact on environment and human health. Anaerobic digestion is an eco-friendly and sustainable option, but its efficiency is limited by recalcitrance of lignocellulose structure. A cascade pretreatment (CP) using microwave irradiation and fungus metabolism was developed in this work to reduce the recalcitrance of BSS and enhance its methane production.

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Biohythane production from wastewater via anaerobic fermentation currently relies on two-stage physically separated biohydrogen and biomethane reactors, which requires closed monitoring, the implementation of a control system, and cost-intensive, complex operation. Herein, an innovative multistage anaerobic hythane reactor (MAHR) was reported via integrating two-stage fermentation into one reactor. MAHR was constructed using an internal down-flow packed bed reactor and an external up-flow sludge blanket to enhance microbial enrichment and thermodynamic feasibility of the associated bioreactions.

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Excessive food waste presents an opportunity to simultaneously alleviate waste and produce renewable resources. The present work uses hydrothermal liquefaction (HTL) with elevated temperatures (280-380 °C) and times (10-60 min) to convert categorized food residues collected from a university campus dining hall into biocrude oil. Analysis of distinct feedstocks presented different biochemical compositions (protein, carbohydrate, and lipid) and yielded between 2 and 79% biocrude oil for the respective optimized HTL temperatures and times.

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Hydrothermal pretreatment (HTP) using an acidic catalyst is known to be effective for reducing lignocellulosic biomass recalcitrance. Post-hydrothermal liquefaction wastewater (PHW) from hydrothermal liquefaction of swine manure contains a large fraction of organic acids and thus was introduced to improve the HTP of cornstalk in this study. The response surface methodology was performed to optimize operating parameters of HTP for preserving structural polysaccharides while removing the barrier substances.

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Developing efficient methods to recover energy from post-hydrothermal liquefaction wastewater (PHW) is critical for scaling up hydrothermal liquefaction (HTL) technology. Here we evaluated two-stage fermentation (TF) and catalytic hydrothermal gasification (CHG) for biohythane production using PHW. A hydrogen yield of 29 mL·g COD and methane yield of 254 mL·g COD were achieved via TF.

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Post-hydrothermal liquefaction wastewater (PHWW), which contains approximately 80% of original feedstock resources, shows great potential to achieve sustainable development of an environment-enhancing energy system. A combination of anaerobic digestion and algae cultivation was proposed for methane recovery and nutrient supply from PHWW. Granular activated carbon (GAC) and ozone were used to enhance energy recovery from the PHWW.

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Hydrothermal liquefaction is a promising technology to convert wet biomass into bio-oil. However, post-hydrothermal liquefaction wastewater (PHWW) is also produced during the process. This wastewater contains a high concentration of organic compounds, including phenols and N-heterocyclic compounds which are two main inhibitors for biological treatment.

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One critical challenge of hydrothermal liquefaction (HTL) is its complex aqueous product, which has a high concentration of organic pollutants (up to 100gCOD/L) and diverse fermentation inhibitors, such as furfural, phenolics and N-heterocyclic compounds. Here we report continuous anaerobic digestion of HTL wastewater via an up-flow anaerobic sludge bed reactor (UASB) and packed bed reactor (PBR). Specifically, we investigated the transformation of fermentation inhibitors and microbial response.

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A concept of biohythane production by combining biohydrogen and biomethane together via two-stage anaerobic fermentation (TSAF) has been recently proposed and considered as a promising approach for sustainable hythane generation from waste biomass. The advantage of biohythane over traditional biogas are more environmentally benign, higher energy recovery and shorter fermentation time. However, many of current efforts to convert waste biomass into biohythane are still at the bench scale.

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Biofuel production from lignocellulosic biomass through hydrothermal liquefaction (HTL) is a promising direction. This study characterized the products and investigated the elemental migration during the HTL of cornstalk at seven different operation temperatures (210-375°C). The biocrude oil yield significantly increased from 7.

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Article Synopsis
  • The study explores a method for producing biohythane from cornstalk using hydrothermal liquefaction (HTL) followed by two-stage fermentation, addressing the challenges of utilizing lignocellulosic biomass.
  • Results show that while biohydrogen production decreased at high organic loading rates (OLR), methane production rates in both UASB and PBR systems remained stable, achieving efficient energy and carbon recovery of 79.0% and 67.7% respectively.
  • The process effectively degraded fermentation inhibitors like 5-hydroxymethyl furfural and furfural, highlighting the advantages of two-stage fermentation over single-stage for superior methane production.
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