Publications by authors named "Brendan Faeth"

Moiré superlattices constructed from transition metal dichalcogenides have demonstrated a series of emergent phenomena, including moiré excitons, flat bands, and correlated insulating states. All of these phenomena depend crucially on the presence of strong moiré potentials, yet the properties of these moiré potentials, and the mechanisms by which they can be generated, remain largely open questions. Here, we use angle-resolved photoemission spectroscopy with submicron spatial resolution to investigate an aligned WS/WSe moiré superlattice and graphene/WS/WSe trilayer heterostructure.

View Article and Find Full Text PDF

Interface quantum materials have yielded a plethora of previously unknown phenomena, including unconventional superconductivity, topological phases, and possible Majorana fermions. Typically, such states are detected at the interface between two insulating constituents by electrical transport, but whether either material is conducting, transport techniques become insensitive to interfacial properties. To overcome these limitations, we use angle-resolved photoemission spectroscopy and molecular beam epitaxy to reveal the electronic structure, charge transfer, doping profile, and carrier effective masses in a layer-by-layer fashion for the interface between the Dirac nodal-line semimetal SrIrO and the correlated metallic Weyl ferromagnet SrRuO.

View Article and Find Full Text PDF

The observation of replica bands by angle-resolved photoemission spectroscopy has ignited interest in the study of electron-phonon coupling at low carrier densities, particularly in monolayer FeSe/SrTiO_{3}, where the appearance of replica bands has motivated theoretical work suggesting that the interfacial coupling of electrons in the FeSe layer to optical phonons in the SrTiO_{3} substrate might contribute to the enhanced superconducting pairing temperature. Alternatively, it has also been recently proposed that such replica bands might instead originate from extrinsic final state losses associated with the photoemission process. Here, we perform a quantitative examination of replica bands in monolayer FeSe/SrTiO_{3}, where we are able to conclusively demonstrate that the replica bands are indeed signatures of intrinsic electron-boson coupling, and not associated with final state effects.

View Article and Find Full Text PDF

Topological materials are derived from the interplay between symmetry and topology. Advances in topological band theories have led to the prediction that the antiperovskite oxide Sr SnO is a topological crystalline insulator, a new electronic phase of matter where the conductivity in its (001) crystallographic planes is protected by crystallographic point group symmetries. Realization of this material, however, is challenging.

View Article and Find Full Text PDF
Article Synopsis
  • The study investigates the electroadsorption free energies of hydroxide (OH) and oxide (O) on the RuO(110) surface and their relationship to the oxygen evolution reaction (OER) electrocatalysis, considering pH effects.
  • Using the Sabatier principle, which suggests moderate stabilization of intermediates for optimal catalytic activity, the authors compare oxygen electroadsorption energies to OER activity.
  • The findings reveal that while electroadsorption energies on RuO(110) vary with pH and follow certain scaling relations, there is no direct correlation with OER activity, prompting questions about the applicability of the Sabatier principle in predicting performance for highly active electrocatalysts where kinetics might play a bigger
View Article and Find Full Text PDF