This study aims to understand the fate and transport of per- and polyfluoroalkyl substances (PFAS) and inorganic fluoride (IF) at an undisclosed municipal wastewater treatment plant (WWTP) operating a sewage sludge incinerator (SSI). A robust statistical analysis characterized concentrations and mass flows at all WWTP and SSI primary influents/effluents, including thermal-treatment derived airborne emissions. WWTP-level net mass flows (NMFs) of total PFAS were not statistically different from zero.
View Article and Find Full Text PDFA review of published literature was conducted to present the concentrations and composition profiles of per- and polyfluoroalkyl substances (PFAS) from significant sources to the environment. The major sources of PFAS to the environment are categorized under direct and indirect sources. The characteristic compounds and concentrations are summarized as found from direct sources such as manufacturing facilities, aqueous film-forming foam (AFFF) applications, metal coating operations, and textile and paper coating operations; and from indirect sources such as landfills and wastewater treatment plants (WWTPs).
View Article and Find Full Text PDFThe brick kiln industrial sector in South Asia accounts for large amounts of short-lived climate forcer (SLCF) emissions, namely black carbon (BC), organic carbon (OC), and sulfur dioxide (SO; the precursor to atmospheric sulfate [SO]). These SLCFs are air pollutants and have important impacts on both human health and the Arctic, a region currently experiencing more than double the rate of warming relative to the global average. Using previously derived Arctic equilibrium temperature response factors, we estimate the contribution to Arctic temperature impacts from previously reported emissions of BC, OC, and SO from four prevalent South Asian brick kiln types (Bull's Trench [BTK], Down Draught [DDK], Vertical Shaft [VSBK], and Zig-zag).
View Article and Find Full Text PDFThe use of residential heating devices is a key source of black carbon and other short-lived climate forcer emissions in Arctic and other high latitude regions, with important impacts to the Arctic climate and human health. The types of combustion technologies and fuels used varies by region, which impacts the emission profiles of these pollutants and thus the magnitude of Arctic climate responses. Using emission inventory data from 14 European countries, we derive wood-fueled residential heating emissions of black carbon, organic carbon, and sulfate from six appliance types in 2016.
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