X-ray Thomson scattering experiments in the soft and hard x-ray regime yield information on fundamental parameters of high-density systems. Pump-probe experiments with variable time delay provide insight into the excitation and relaxation dynamics in dense plasmas. On short time scales, a local thermodynamic equilibrium description might not be sufficient.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
July 2015
The spectrum of x-ray Thomson scattering is proportional to the dynamic structure factor. An important contribution is the ion feature which describes elastic scattering of x rays off electrons. We apply an ab initio method for the calculation of the form factor of bound electrons, the slope of the screening cloud of free electrons, and the ion-ion structure factor in warm dense beryllium.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
July 2014
We investigate subpicosecond dynamics of warm dense hydrogen at the XUV free-electron laser facility (FLASH) at DESY (Hamburg). Ultrafast impulsive electron heating is initiated by a ≤ 300-fs short x-ray burst of 92-eV photon energy. A second pulse probes the sample via x-ray scattering at jitter-free variable time delay.
View Article and Find Full Text PDFThe introduction of brilliant free-electron lasers enables new pump-probe experiments to characterize warm dense matter states. For instance, a short-pulse optical laser irradiates a liquid hydrogen jet that is subsequently probed with brilliant soft x-ray radiation. The strongly inhomogeneous plasma prepared by the optical laser is characterized with particle-in-cell simulations.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
April 2010
A quantum kinetic approach for the energy relaxation in strongly coupled plasmas with different electron and ion temperatures is presented. Based on the density operator formalism, we derive a balance equation for the energies of electrons and ions connecting kinetic, correlation, and exchange energies with a quite general expression for the electron-ion energy-transfer rate. The latter is given in terms of the correlation function of density fluctuations which allows for a derivation of increasingly realistic approximation schemes including a coupled-mode expression.
View Article and Find Full Text PDFWe investigate ultrafast (fs) electron dynamics in a liquid hydrogen sample, isochorically and volumetrically heated to a moderately coupled plasma state. Thomson scattering measurements using 91.8 eV photons from the free-electron laser in Hamburg (FLASH at DESY) show that the hydrogen plasma has been driven to a nonthermal state with an electron temperature of 13 eV and an ion temperature below 0.
View Article and Find Full Text PDFCollective Thomson scattering with extreme ultraviolet light or x rays is shown to allow for a robust measurement of the free electron density in dense plasmas. Collective excitations like plasmons appear as maxima in the scattering signal. Their frequency position can directly be related to the free electron density.
View Article and Find Full Text PDFWe present the first collective x-ray scattering measurements of plasmons in solid-density plasmas. The forward scattering spectra of a laser-produced narrow-band x-ray line from isochorically heated beryllium show that the plasmon frequency is a sensitive measure of the electron density. Dynamic structure calculations that include collisions and detailed balance match the measured plasmon spectrum indicating that this technique will enable new applications to determine the equation of state and compressibility of dense matter.
View Article and Find Full Text PDFThe interaction of ultrashort laser pulses with matter is a topic of growing interest. In particular, recent developments on free-electron lasers have opened an unexplored field in which many interesting physical phenomena are to be expected. Since hydrodynamic descriptions of the interaction process need a microscopic "input," a quantum statistical theory of energy absorption by matter is required.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
May 2005
Collisional absorption of dense fully ionized plasmas in strong laser fields is investigated using quantum statistical methods as well as molecular dynamics simulations. For high-frequency fields, quantum statistical expressions for the electrical current density and the electron-ion collision frequency are presented. Strong correlations are taken into account and their influence on the absorption rate is discussed.
View Article and Find Full Text PDFPhys Rev E Stat Phys Plasmas Fluids Relat Interdiscip Topics
December 1999
The two-particle problem within a nonequilibrium many-particle system is investigated in the framework of real-time Green's functions. Starting from the nonequilibrium Bethe-Salpeter equation on the Keldysh contour, a Dyson equation is given for two-time two-particle Green's functions. Thereby the well-known Kadanoff-Baym equations are generalized to the case of two-particle functions.
View Article and Find Full Text PDFPhys Rev E Stat Phys Plasmas Fluids Relat Interdiscip Topics
October 1999
A kinetic theory for quantum many-particle systems in time-dependent electromagnetic fields is developed based on a gauge-invariant formulation. The resulting kinetic equation generalizes previous results to quantum systems and includes many-body effects. It is, in particular, applicable to the interaction of strong laser fields with dense correlated plasmas.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
March 2002
The stopping power of strongly coupled, partially ionized plasmas is investigated for charged beam particles with arbitrary velocities. Our approach is based on kinetic equations of the Boltzmann type that are suitably generalized to describe three-particle collisions. In this way, we consider elastic collisions between the beam and free plasma particles as well as the ionization and excitation of composite plasma particles by beam particle impact.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
August 2001
Collisional absorption of dense, fully ionized plasmas in strong laser fields is investigated starting from a quantum kinetic equation with non-Markovian and field-dependent collision integrals in dynamically screened Born approximation. This allows to find rather general balance equations for the energy and the current. For high-frequency laser fields, quantum statistical expressions for the electrical current density and the cycle-averaged electron-ion collision frequency in terms of the Lindhard dielectric function are derived.
View Article and Find Full Text PDFPhys Rev E Stat Phys Plasmas Fluids Relat Interdiscip Topics
October 1996
Phys Rev E Stat Phys Plasmas Fluids Relat Interdiscip Topics
March 1996