The coherent spin dynamics of electrons and holes in CsPbI perovskite nanocrystals in a glass matrix are studied by the time-resolved Faraday ellipticity technique in magnetic fields up to 430 mT across a temperature range from 6 K to 120 K. The Landé -factors and spin dephasing times are evaluated from the observed Larmor precession of electron and hole spins. The nanocrystal size in the three studied samples varies from about 8 to 16 nm, resulting in exciton transition varying from 1.
View Article and Find Full Text PDFNanomaterials (Basel)
December 2023
Coherent spin dynamics of electrons in CdSe colloidal nanoplatelets are investigated by time-resolved pump-probe Faraday rotation at room and cryogenic temperatures. We measure electron spin precession in a magnetic field and determine -factors of 1.83 and 1.
View Article and Find Full Text PDFCoherent spin dynamics of charge carriers in CsPbBr3 perovskite nanocrystals are studied in a temperature range of 4-300 K and in magnetic fields of up to 500 mT using time-resolved pump-probe Faraday rotation and differential transmission techniques. We detect electron spin Larmor precession in the entire temperature range. At temperatures below 50 K, hole spin precession is also observed.
View Article and Find Full Text PDFDouble-scroll attractors are one of the pillars of modern chaos theory. However, rigorous computer-free analysis of their existence and global structure is often elusive. Here, we address this fundamental problem by constructing an analytically tractable piecewise-smooth system with a double-scroll attractor.
View Article and Find Full Text PDFThe spin physics of perovskite nanocrystals with confined electrons or holes is attracting increasing attention, both for fundamental studies and spintronic applications. Here, stable [Formula: see text] lead halide perovskite nanocrystals embedded in a fluorophosphate glass matrix are studied by time-resolved optical spectroscopy to unravel the coherent spin dynamics of holes and their interaction with nuclear spins of the Pb isotope. We demonstrate the spin mode locking effect provided by the synchronization of the Larmor precession of single hole spins in each nanocrystal in the ensemble that are excited periodically by a laser in an external magnetic field.
View Article and Find Full Text PDFLead halide perovskite nanocrystals in a glass matrix are a promising platform for optoelectronic applications due to their excellent optical properties combined with outstanding stability against the environment. We reveal the potential of this system for spintronics by studying the electron spin properties of CsPb(Cl,Br) nanocrystals in a fluorophosphate glass matrix. Using optical spin orientation and spin depolarization with a radio frequency field, we measure longitudinal spin relaxation time, , reaching several hundreds of microseconds at low temperatures.
View Article and Find Full Text PDFPartial synchronization emerges in an oscillator network when the network splits into clusters of coherent and incoherent oscillators. Here, we analyze the stability of partial synchronization in the second-order finite-dimensional Kuramoto model of heterogeneous oscillators with inertia. Toward this goal, we develop an auxiliary system method that is based on the analysis of a two-dimensional piecewise-smooth system whose trajectories govern oscillating dynamics of phase differences between oscillators in the coherent cluster.
View Article and Find Full Text PDFThe inhomogeneity of an electron spin ensemble as well as fluctuating environment acting upon individual spins drastically shorten the spin coherence time T_{2} and hinder coherent spin manipulation. We show that this problem can be solved by the simultaneous application of a radio frequency (rf) field, which stimulates coherent spin precession decoupled from an inhomogeneous environment, and periodic optical pulses, which amplify this precession. The resulting resonance, taking place when the rf field frequency approaches the laser pulse repetition frequency, has a width determined by the spin coherence time T_{2} that is free from the effects of inhomogeneity and slow nuclear spin fluctuations.
View Article and Find Full Text PDFThe outstanding optical quality of lead halide perovskites inspires studies of their potential for the optical control of carrier spins as pursued in other materials. Entering largely uncharted territory, time-resolved pump-probe Kerr rotation is used to explore the coherent spin dynamics of electrons and holes in bulk formamidinium caesium lead iodine bromide (FA Cs PbI Br ) and to determine key parameters characterizing interactions of their spins, such as the g-factors and relaxation times. The demonstrated long spin dynamics and narrow g-factor distribution prove the perovskites as promising competitors for conventional semiconductors in spintronics.
View Article and Find Full Text PDFThe spin dynamics in CsPbBr lead halide perovskite nanocrystals are studied by picosecond pump-probe Faraday rotation in an external magnetic field. Coherent Larmor precession of electrons and holes with spin dephasing times of ∼600 ps is detected in a transversal magnetic field. The longitudinal spin relaxation time in weak magnetic fields reaches 80 ns at a temperature of 5 K.
View Article and Find Full Text PDFNon-smooth systems can generate dynamics and bifurcations that are drastically different from their smooth counterparts. In this paper, we study such homoclinic bifurcations in a piecewise-smooth analytically tractable Lorenz-type system that was recently introduced by Belykh et al. [Chaos 29, 103108 (2019)].
View Article and Find Full Text PDFNanomaterials (Basel)
November 2020
Van-der Waals heterostructures assembled from one or few atomic layer thickness crystals are becoming increasingly more popular in condensed matter physics. These structures are assembled using transfer machines, those are based on mask aligners, probe stations or are home-made. For many laboratories it is vital to build a simple, convenient and universal transfer machine.
View Article and Find Full Text PDFIn this paper, we consider blinking systems, i.e., non-autonomous systems generated by randomly switching between several autonomous continuous time subsystems in each sequential fixed period of time.
View Article and Find Full Text PDFWe develop a simple method for measuring the electron spin relaxation times [Formula: see text], [Formula: see text] and [Formula: see text] in semiconductors and demonstrate its exemplary application to n-type GaAs. Using an abrupt variation of the magnetic field acting on electron spins, we detect the spin evolution by measuring the Faraday rotation of a short laser pulse. Depending on the magnetic field orientation, this allows us to measure either the longitudinal spin relaxation time [Formula: see text] or the inhomogeneous transverse spin dephasing time [Formula: see text].
View Article and Find Full Text PDFModeling cooperative dynamics using networks of phase oscillators is common practice for a wide spectrum of biological and technological networks, ranging from neuronal populations to power grids. In this paper we study the emergence of stable clusters of synchrony with complex intercluster dynamics in a three-population network of identical Kuramoto oscillators with inertia. The populations have different sizes and can split into clusters where the oscillators synchronize within a cluster, but notably, there is a phase shift between the dynamics of the clusters.
View Article and Find Full Text PDFThe low-temperature emission spectrum of CdSe colloidal nanoplatelets (NPLs) consists of two narrow lines. The high-energy line stems from the recombination of neutral excitons. The origin of the low-energy line is currently debated.
View Article and Find Full Text PDFChaotic attractors appear in various physical and biological models; however, rigorous proofs of their existence and bifurcations are rare. In this paper, we construct a simple piecewise-smooth model which switches between three three-dimensional linear systems that yield a singular hyperbolic attractor whose structure and bifurcations are similar to those of the celebrated Lorenz attractor. Due to integrability of the linear systems composing the model, we derive a Poincaré return map to rigorously prove the existence of the Lorenz-type attractor and explicitly characterize bifurcations that lead to its birth, structural changes, and disappearance.
View Article and Find Full Text PDFThe original version of this Article contained an error in Fig. 2c, in which the numbers on the y-axis were given in the wrong order: '800' at the bottom through to '0' at the top. This has been corrected in both the PDF and HTML versions of the Article.
View Article and Find Full Text PDFThe lead halide perovskites demonstrate huge potential for optoelectronic applications, high energy radiation detectors, light emitting devices and solar energy harvesting. Those materials exhibit strong spin-orbit coupling enabling efficient optical orientation of carrier spins in perovskite-based devices with performance controlled by a magnetic field. Here we show that elaborated time-resolved spectroscopy involving strong magnetic fields can be successfully used for perovskites.
View Article and Find Full Text PDFModern pedestrian and suspension bridges are designed using industry standard packages, yet disastrous resonant vibrations are observed, necessitating multimillion dollar repairs. Recent examples include pedestrian-induced vibrations during the opening of the Solférino Bridge in Paris in 1999 and the increased bouncing of the Squibb Park Bridge in Brooklyn in 2014. The most prominent example of an unstable lively bridge is the London Millennium Bridge, which started wobbling as a result of pedestrian-bridge interactions.
View Article and Find Full Text PDFWe study the band-edge exciton fine structure and in particular its bright-dark splitting in colloidal semiconductor nanocrystals by four different optical methods based on fluorescence line narrowing and time-resolved measurements at various temperatures down to 2 K. We demonstrate that all these methods provide consistent splitting values and discuss their advances and limitations. Colloidal CdSe nanoplatelets with thicknesses of 3, 4 and 5 monolayers are chosen for experimental demonstrations.
View Article and Find Full Text PDFSeveral modern footbridges around the world have experienced large lateral vibrations during crowd loading events. The onset of large-amplitude bridge wobbling has generally been attributed to crowd synchrony; although, its role in the initiation of wobbling has been challenged. To study the contribution of a single pedestrian into overall, possibly unsynchronized, crowd dynamics, we use a bio-mechanically inspired inverted pendulum model of human balance and analyze its bi-directional interaction with a lively bridge.
View Article and Find Full Text PDFWe study the co-existence of stable patterns of synchrony in two coupled populations of identical Kuramoto oscillators with inertia. The two populations have different sizes and can split into two clusters where the oscillators synchronize within a cluster while there is a phase shift between the dynamics of the two clusters. Due to the presence of inertia, which increases the dimensionality of the oscillator dynamics, this phase shift can oscillate, inducing a breathing cluster pattern.
View Article and Find Full Text PDFThe dynamics of the expansion of the first order spatial coherence g(1) for a polariton system in a high-Q GaAs microcavity was investigated on the basis of Young's double slit experiment under 3 ps pulse excitation at the conditions of polariton Bose-Einstein condensation. It was found that in the process of condensate formation the coherence expands with a constant velocity of about 10(8) cm/s. The measured coherence is smaller than that in a thermal equilibrium system during the growth of condensate density and well exceeds it at the end of condensate decay.
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