Taming Friedrich-Wintgen Interference in a Resonant Metasurface: Vortex Laser Emitting at an On-Demand Tilted Angle.

Friedrich-Wintgen (FW) interference is an atypical coupling mechanism that grants loss exchange between leaky resonances in non-Hermitian classical and quantum systems. Intriguingly, such a mechanism makes destructive interference possible for scenarios in which a radiating wave becomes a bound state in the continuum (BIC) by giving away all of its losses. Here we propose and demonstrate experimentally an original concept to tailor FW-BICs with polarization singularity at on-demand wavevectors in an optical metasurface.

Exploring the benefits of surface analysis techniques to develop double multilayer transfer printing of J-Aggregates cyanine dyes by integrating L-b-L and μCp processes.

Layer-by-layer self-assembly (L-b-L assembly) makes possible to obtain polyelectrolyte multilayers (PEMs) and one of the polyelectrolytes could be replaced by a dye molecule to obtain multilayers which may exhibit optical properties of great interest. On the other hand, μCp has become a routine technique for the preparation of micro- and nanostructured surfaces. In our development in progress of a surface engineering strategy to transfer J-Agg cyanine dyes onto surfaces by integrating L-b-L process and μCp, this contribution highlights how surface analysis imaging techniques can bring valuable information for the development of the process involving a double Multilayers Transfer Printing (MTP) with a Moiré effect.

Tamm plasmons in metal/nanoporous GaN distributed Bragg reflector cavities for active and passive optoelectronics.

We theoretically and experimentally investigate Tamm plasmon (TP) modes in a metal/semiconductor distributed Bragg reflector (DBR) interface. A thin Ag (silver) layer with a thickness (55 nm from simulation) that is optimized to guarantee a low reflectivity at the resonance was deposited on nanoporous GaN DBRs fabricated using electrochemical (EC) etching on freestanding semipolar (2021¯) GaN substrates. The reflectivity spectra of the DBRs are compared before and after the Ag deposition and with that of a blanket Ag layer deposited on GaN.

Selective grating obtained by dye microstructuration based on local photobleaching using a laser writer.

We propose a method to pattern organic optically active materials based on local photobleaching for creating a wavelength-selective grating. Usually, photobleaching is considered a limitation for an organic emitter. Here, this property is exploited to locally suppress dye emission and absorption at the microscale with an abrupt interface and no changes in layer thickness.

Anisotropy and Controllable Band Structure in Suprawavelength Polaritonic Metasurfaces.

In this Letter, we exploit the extended coherence length of mixed plasmon-exciton states to generate active metasurfaces. For this purpose, periodic stripes of organic dye are deposited on a continuous silver film. Typical metasurface effects, such as effective behavior and geometry sensitivity, are measured for periods exceeding the polaritonic wavelength by more than one order of magnitude.

Enhancement of spontaneous emission in Tamm plasmon structures.

It was theoretically and experimentally demonstrated that in metal/semiconductor Tamm plasmon structures the probability of spontaneous emission can be increased despite losses in metal, and theoretical analysis of experimental results suggested that the enhancement could be as high as one order of magnitude. Tamm plasmon structure with quantum dots has been fabricated and the emission pattern has been measured. Electromagnetic modes of the structure have been analyzed and modification of spontaneous emission rates has been calculated showing a good agreement with experimentally observed emission pattern.

High quality factor confined Tamm modes.

We demonstrate that quality factors up to 5000 can be obtained in Tamm-like hybrid metal/semiconductor structures. To do this, a Bragg mirror is covered by a thin transparent layer and a metallic film. The reduced losses of these modes are related to an intermediate behavior between conventional Tamm plasmon and Bragg modes lying deeper in the semiconductor medium.

Highly efficient singular surface plasmon generation by achiral apertures.

We report a highly efficient generation of singular surface plasmon (SP) fields by an achiral plasmonic structure consisting of Λ-shaped apertures. Our quantitative analysis, based on leakage radiation microscopy (LRM), demonstrates that the induced spin-orbit coupling can be tuned by adjusting the apex angle of the Λ-shaped aperture. Specifically, the array of Λ-shaped apertures with the apex angle 60° is shown to give rise to the directional coupling efficiency.

Coherence and aberration effects in surface plasmon polariton imaging.

We study theoretically and experimentally coherent imaging of surface plasmon polaritons using either leakage radiation microscopy through a thin metal film or interference microscopy through a thick metal film. Using a rigorous modal formalism based on scalar Whittaker potentials, we develop a systematic analytical and vectorial method adapted to the analysis of coherent imaging involving surface plasmon polaritons. The study includes geometrical aberrations due index mismatch which played an important role in the interpretation of recent experiments using leakage radiation microscopy.

Leakage interferences applied to surface plasmon analysis.

We report the experimental combination of leakage radiation microscopy with a Young slit experiment to address the spatial coherence properties of surface waves. We applied this method to measurements of surface plasmon polaritons (SPPs). The relationship between the spatial decay and interference contrast allows us to extract the degree of coherence.

Confined Tamm plasmon lasers.

We demonstrate that confined Tamm plasmon modes can be advantageously exploited for the realization of new kind of metal/semiconductor lasers. Laser emission is demonstrated for Tamm structures with various diameters of the metallic disks which provide the confinement. A reduction of the threshold with the size is observed.

Spatial coherence properties of surface plasmon investigated by Young's slit experiment.

In this Letter, we present an original method to extract the optical properties of surface plasmon polaritons (SPPs) on silver surfaces. A two Young's slit experiment combined with a leakage radiation microscope has been built. By correlating both imagery and coherence measurements on the same area, we are able to address the evolution of the SPP spatial coherence along its propagation.

Coherent emission from a disordered organic semiconductor induced by strong coupling with surface plasmons.

In this Letter, we show that the strong coupling between a disordered set of molecular emitters and surface plasmons leads to the formation of spatially coherent hybrid states extended on macroscopic distances. Young-type interferometric experiments performed on a system of J-aggregated dyes spread on a silver layer evidence the coherent emission from different molecular emitters separated by several microns. The coherence is absent in systems in the weak-coupling regime demonstrating the key role of the hybridization of the molecules with the plasmon.

Evidence for confined tamm plasmon modes under metallic microdisks and application to the control of spontaneous optical emission.

We demonstrate strong confinement of the optical field by depositing a micron sized metallic disk on a planar distributed Bragg reflector. Confined Tamm plasmon modes are evidenced both experimentally and theoretically, with a lateral confinement limited to the disk area and strong coupling to TE polarized fields. Single quantum dots controllably coupled to these modes are shown to experience acceleration of their spontaneous emission when spectrally resonant with the mode.

Strong coupling between surface plasmons and excitons in an organic semiconductor.

We report on the observation of a strong coupling between a surface plasmon and an exciton. Reflectometry experiments are performed on an organic semiconductor, namely, cyanide dye J aggregates, deposited on a silver film. The dispersion lines present an anticrossing that is the signature of a strong plasmon-exciton coupling.