Persistent Ground-State Planar Alignment of Iodine Molecule through Resonant Excitation.

We demonstrate the generation of a persistent planar molecular alignment by subjecting a relatively warm gas sample to a resonant femtosecond laser pulse. By optically probing I_{2} molecules in their vibronic ground states, we observe a persistent delocalization of their axes near the plane orthogonal to the field direction. This phenomenon is attributed to the one-photon resonant excitation, primarily removing molecules from the thermal ground-state distribution that are initially aligned along the field, i.

High-gain far-detuned nonlinear frequency conversion in a few-mode graded-index optical fiber.

We present theoretical and experimental evidence of high-gain far-detuned nonlinear frequency conversion, extending towards both the visible and the mid-infrared, in a few-mode graded-index silica fiber pumped at 1.064  , and more specifically achieving gains of hundreds of dB per meter below 0.65  and beyond 3.

Phase-matching-free ultrashort laser pulse characterization from a transient plasma lens.

A phase-matching-free ultrashort pulse retrieval based on the defocusing of a laser-induced plasma is presented. In this technique, a pump pulse ionizes a rare gas providing a plasma lens whose creation time is ultrafast. A probe pulse propagating through this gas lens experiences a switch of its divergence.

Multi-octave mid-infrared supercontinuum generation in tapered chalcogenide-glass rods.

We report on the experimental development of short-tapered chalcogenide-glass rods for mid-infrared supercontinuum generation. Multi-octave spectral broadening of femtosecond laser pulses is demonstrated from 1.6 to 15.

Discretized Conical Waves in Multimode Optical Fibers.

Multimode optical fibers are essential in bridging the gap between nonlinear optics in bulk media and single-mode fibers. The understanding of the transition between the two fields remains complex due to intermodal nonlinear processes and spatiotemporal couplings, e.g.

Doppler effect as a tool for ultrashort electric field reconstruction.

We present a new, to the best of our knowledge, variant of the spectral-shearing interferometry method for characterizing ultrashort laser pulses. This original approach, called Doppler effect e-field replication (DEER), exploits the rotational Doppler effect for producing frequency shear and provides spectral shearing in the absence of frequency conversion, enabling operation in the ultraviolet spectral range. Evaluation of the DEER-spectral phase interferometry for direct electric field reconstruction setup reveals a phase reconstruction of great reliability.

BOAR: Biprism based optical autocorrelation with retrieval.

A simple and compact single-shot autocorrelator is presented and analyzed in detail. The autocorrelator is composed of two elements only: a Fresnel biprism used to create two temporally delayed replicas of the pulse to characterize and a camera in which two-photon absorption takes place. The two-photon absorption signal obtained in the camera can be used to retrieve the pulse duration, the frequency chirp, and the pulse spectrum, provided that a Gaussian temporal shape is assumed.

Multimodal unidirectional pulse propagation equation.

In this paper, after a brief recall of the derivation of the unidirectional pulse propagation equation generalized to structured media, a fast modal transform linking the spatiotemporal representation of the field and its modal distribution is presented. This transform is used for solving the propagation equation by using a split-step algorithm in an efficient way. As an example, we present, to the best of our knowledge, the first numerical evidence of the generation of conical waves in highly multimodes waveguides.

Polarized all-normal dispersion supercontinuum reaching 2.5 µm generated in a birefringent microstructured silica fiber.

We demonstrate a polarized all-normal dispersion supercontinuum generated in a birefringent silica microstructured fiber spanning beyond 2.5 µm. To our knowledge, this is the spectra reaching the furthest in mid-infrared ever generated in normal dispersion silica fibers.

Shaping of ultraviolet femtosecond laser pulses by Fourier domain harmonic generation.

We present a method to finely tailor ultraviolet femtosecond laser pulses using a pulse shaper with ability in the infrared/visible spectral range. We have developed to that end a frequency doubling module in which the up-conversion mechanism is carried out in the Fourier plane of a 4 f -line. The pulse shaper is used to imprint a spectral phase and/or amplitude onto the fundamental pulse.

Mid-infrared laser filamentation in molecular gases.

We observed the filamentation of mid-infrared ultrashort laser pulses (3.9 μm, 80 fs) in molecular gases. It efficiently generates a broadband supercontinuum over two octaves in the 2.

White light generation over three octaves by femtosecond filament at 3.9 µm in argon.

We report the first (to our knowledge) experimental results and numerical simulations on mid-IR femtosecond pulse filamentation in argon using 0.1 TW peak-power, 80 fs, 3.9 μm pulses.

High-field quantum calculation reveals time-dependent negative Kerr contribution.

The exact quantum time-dependent optical response of hydrogen under strong-field near-infrared excitation is investigated and compared to the perturbative model widely used for describing the effective atomic polarization induced by intense laser fields. By solving the full 3D time-dependent Schrödinger equation, we exhibit a supplementary, quasi-instantaneous defocusing contribution missing in the weak-field model of polarization. We show that this effect is far from being negligible, in particular when closures of ionization channels occur and stems from the interaction of electrons with their parent ions.

Higher-order Kerr improve quantitative modeling of laser filamentation.

We test numerical filamentation models against experimental data about the peak intensity and electron density in laser filaments. We show that the consideration of the higher-order Kerr effect improves the quantitative agreement without the need of adjustable parameters.

Conical emission from laser filaments and higher-order Kerr effect in air.

We numerically investigate the conical emission (CE) from ultrashort laser filaments, both considering and disregarding the higher-order Kerr effect (HOKE). While the consideration of HOKE has almost no influence on the predicted CE from collimated beams, differences arise for tightly focused beams. This difference is attributed to the different relative contributions of the nonlinear focus and of the modulational instability over the whole filament length.

Transition from plasma-driven to Kerr-driven laser filamentation.

While filaments are generally interpreted as a dynamic balance between Kerr focusing and plasma defocusing, the role of the higher-order Kerr effect (HOKE) is actively debated as a potentially dominant defocusing contribution to filament stabilization. In a pump-probe experiment supported by numerical simulations, we demonstrate the transition between two distinct filamentation regimes at 800 nm. For long pulses (1.

From higher-order Kerr nonlinearities to quantitative modeling of third and fifth harmonic generation in argon.

The recent measurement of negative higher-order Kerr effect (HOKE) terms in gases has given rise to a controversial debate, fed by its impact on short laser pulse propagation. By comparing the experimentally measured yield of the third and fifth harmonics, with both an analytical and a full comprehensive numerical propagation model, we confirm the absolute and relative values of the reported HOKE indices.

Arbitrary-order nonlinear contribution to self-steepening.

On the basis of the recently published generalized Miller formulas, we derive the spectral dependence of the contribution of arbitrary-order nonlinear indices to the group-velocity index. We show that in the context of laser filamentation in gases, all experimentally accessible orders (up to the ninth-order nonlinear susceptibility chi((9)) in air and chi((11)) in argon) have contributions of alternative signs and similar magnitudes. Moreover, we show both analytically and numerically that the dispersion term of the nonlinear indices must be considered when computing the intensity-dependent group velocity.

Higher-order Kerr terms allow ionization-free filamentation in gases.

We show that higher-order nonlinear indices (n(4), n(6), n(8), n(10)) provide the main defocusing contribution to self-channeling of ultrashort laser pulses in air and argon at 800 nm, in contrast with the previously accepted mechanism of filamentation where plasma was considered as the dominant defocusing process. Their consideration allows us to reproduce experimentally observed intensities and plasma densities in self-guided filaments.

Optical rogue wave statistics in laser filamentation.

We experimentally observed optical rogue wave statistics during high power femtosecond pulse filamentation in air. We characterized wavelength-dependent intensity fluctuations across 300 nm broadband filament spectra generated by pulses with several times the critical power for filamentation. We show how the statistics vary from a near-Gaussian distribution in the vicinity of the pump to a long tailed "L-shaped" distribution at the short wavelength and long wavelength edges.

Ultraviolet-visible conical emission by multiple laser filaments.

We characterized the angular distribution of the supercontinuum emission from multiple infrared laser filaments propagating in air over long distances, from the infrared (1080 nm) to ultraviolet (225 nm). These experimental data suggest that the X-Waves modeling or Cerenkov emission, rather than phase matching of four-wave mixing, could explain the conical emission. We also estimate the total light conversion efficiency from the original laser wavelength into the white-light continuum.

Dual-color co-filamentation in Argon.

We investigate both experimentally and theoretically the mechanisms driving the co-filamentation of two ultrashort laser pulses at 800 and 400 nm in Argon. The cross-Kerr lens and cross-phase modulation between the two filaments of different colors bridging both the continuum spectra and the plasma channels induced by the individual pulses. This dual-color filamentation also results in the simultaneous generation of two few-cycle pulses at both 800 and 400 nm, providing a potential way to generate attosecond pulses.

Ultrafast gaseous "half-wave plate".

We demonstrate that filaments generated by ultrashort laser pulses can induce a remarkably large birefringence in Argon over its whole length, resulting in an ultrafast "half-wave plate" for a copropagating probe beam. This birefringence originates from the difference between the nonlinear refractive indices induced by the filament on the axes parallel and orthogonal to its polarization. An angle of 45 degrees between the filament and the probe polarizations allows the realization of ultrafast Kerr-gates, with a switching time ultimately limited by the duration of the filamenting pulse.

Laser noise compression by filamentation at 400 nm in argon.

Filamentation is an efficient way to produce an intense and spectrally broad, but poorly stable, source for coherent control spectroscopy. We first described both theoretically and experimentally the filamentation and broadening of a 410 nm ultrashort laser pulse in Argon. By observing the theoretical and experimental spectral cross-correlation in the filament, we then show that the stability of the source can be improved.