Publications by authors named "Basko D"

We study a quantum interacting spin system subject to an external drive and coupled to a thermal bath of vibrational modes, uncorrelated for different spins, serving as a model for dynamic nuclear polarization protocols. We show that even when the many-body eigenstates of the system are ergodic, a sufficiently strong coupling to the bath may effectively localize the spins due to many-body quantum Zeno effect. Our results provide an explanation of the breakdown of the thermal mixing regime experimentally observed above 4-5 K in these protocols.

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We develop a theory of cavity quantum electrodynamics for a 2D electron gas in the presence of Rashba spin-orbit coupling and perpendicular static magnetic field, coupled to spatially nonuniform multimode quantum cavity photon field. We demonstrate that the lowest polaritonic frequency of the full Hamiltonian can vanish for realistic parameters, achieving the Dicke superradiant quantum phase transition. This singular behavior originates from soft spin-flip transitions possessing a nonvanishing dipole moment at nonzero wave vectors and can be viewed as a static paramagnetic instability.

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Monolayers of semiconducting transition metal dichalcogenides are two-dimensional direct-gap systems which host tightly bound excitons with an internal degree of freedom corresponding to the valley of the constituting carriers. Strong spin-orbit interaction and the resulting ordering of the spin-split subbands in the valence and conduction bands makes the lowest-lying excitons in WX_{2} (X being S or Se) spin forbidden and optically dark. With polarization-resolved photoluminescence experiments performed on a WSe_{2} monolayer encapsulated in a hexagonal boron nitride, we show how the intrinsic exchange interaction in combination with the applied in-plane and/or out-of-plane magnetic fields enables one to probe and manipulate the valley degree of freedom of the dark excitons.

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This Letter addresses the dynamical quantum problem of a driven discrete energy level coupled to a semi-infinite continuum whose density of states has a square-root-type singularity, such as states of a free particle in one dimension or quasiparticle states in a BCS superconductor. The system dynamics is strongly affected by the quantum-mechanical repulsion between the discrete level and the singularity, which gives rise to a bound state, suppresses the decay into the continuum, and can produce Stueckelberg oscillations. This quantum coherence effect may limit the performance of mesoscopic superconducting devices, such as the quantum electron turnstile.

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The Coulomb interaction among massless Dirac fermions in graphene is unscreened around the isotropic Dirac points, causing a logarithmic velocity renormalization and a cone reshaping. In less symmetric Dirac materials possessing anisotropic cones with tilted axes, the Coulomb interaction can provide still more exotic phenomena, which have not been experimentally unveiled yet. Here, using site-selective nuclear magnetic resonance, we find a non-uniform cone reshaping accompanied by a bandwidth reduction and an emergent ferrimagnetism in tilted Dirac cones that appear on the verge of charge ordering in an organic compound.

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We report on the realization of a single-electron source, where current is transported through a single-level quantum dot (Q) tunnel coupled to two superconducting leads (S). When driven with an ac gate voltage, the experiment demonstrates electron turnstile operation. Compared to the more conventional superconductor-normal-metal-superconductor turnstile, our superconductor-quantum-dot-superconductor device presents a number of novel properties, including higher immunity to the unavoidable presence of nonequilibrium quasiparticles in superconducting leads.

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We report a theoretical study of electron spin resonance in bulk topological insulators, such as Bi2Se3, Bi2Te3 and Sb2Te3. Using the effective four-band model, we find the electron energy spectrum in a static magnetic field and determine the response to electric and magnetic dipole perturbations, represented by oscillating electric and magnetic fields perpendicular to the static field. We determine the associated selection rules and calculate the absorption spectra.

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We present magneto-Raman scattering studies of electronic inter-Landau level excitations in quasineutral graphene samples with different strengths of Coulomb interaction. The band velocity associated with these excitations is found to depend on the dielectric environment, on the index of Landau level involved, and to vary as a function of the magnetic field. This contradicts the single-particle picture of noninteracting massless Dirac electrons but is accounted for by theory when the effect of electron-electron interaction is taken into account.

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We study the discrete nonlinear Schröinger equation with weak disorder, focusing on the regime when the nonlinearity is, on the one hand, weak enough for the normal modes of the linear problem to remain well resolved but, on the other, strong enough for the dynamics of the normal mode amplitudes to be chaotic for almost all modes. We show that in this regime and in the limit of high temperature, the macroscopic density ρ satisfies the nonlinear diffusion equation with a density-dependent diffusion coefficient, D(ρ) = D(0)ρ(2). An explicit expression for D(0) is obtained in terms of the eigenfunctions and eigenvalues of the linear problem, which is then evaluated numerically.

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We report a comprehensive study of the tuning with electric fields of the resonant magneto-exciton optical phonon coupling in gated graphene. For magnetic fields around B ∼ 25 T that correspond to the range of the fundamental magneto-phonon resonance, the electron-phonon coupling can be switched on and off by tuning the position of the Fermi level in order to Pauli block the two fundamental inter-Landau level excitations. The effects of such a profound change in the electronic excitation spectrum are traced through investigations of the optical phonon response in polarization resolved magneto-Raman scattering experiments.

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Raman spectroscopy is an integral part of graphene research. It is used to determine the number and orientation of layers, the quality and types of edge, and the effects of perturbations, such as electric and magnetic fields, strain, doping, disorder and functional groups. This, in turn, provides insight into all sp(2)-bonded carbon allotropes, because graphene is their fundamental building block.

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Local nature and scaling of chaos in weakly nonlinear disordered chains.

Phys Rev E Stat Nonlin Soft Matter Phys

September 2012

The dynamics of a disordered nonlinear chain can be either regular or chaotic with a certain probability. The chaotic behavior is often associated with the destruction of Anderson localization by the nonlinearity. In the present work it is argued that at weak nonlinearity chaos is nucleated locally on rare resonant segments of the chain.

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Graphite, a model (semi)metal with trigonally warped bands, is investigated with a magnetoabsorption experiment and viewed as an electronic system in the vicinity of the Lifshitz transition. A characteristic pattern of up to 20 cyclotron resonance harmonics has been observed. This large number of resonances, their relative strengths and characteristic shapes trace the universal properties of the electronic states near a separatrix in momentum space.

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Graphene is at the center of a significant research effort. Near-ballistic transport at room temperature and high mobility make it a potential material for nanoelectronics. Its electronic and mechanical properties are also ideal for micro- and nanomechanical systems, thin-film transistors, and transparent and conductive composites and electrodes.

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Graphene edges are of particular interest since their orientation determines the electronic properties. Here we present a detailed Raman investigation of graphene flakes with edges oriented at different crystallographic directions. We also develop a real space theory for Raman scattering to analyze the general case of disordered edges.

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In earlier work we calculated the wavefunction and energy of the solvated polaron in DNA with a simple model in which the charge was taken to be on a single chain of bases at the center of the double helix. To better approximate the actual situation, we have now extended the calculations to the case in which the charge is distributed on two chains of bases, complementary to each other, one on each side of the center. The binding energy of the resulting polaron is somewhat larger than that obtained for the single-chain polaron, the result of each chain of the polaron being closer to some of the polarization charge it induces.

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It has been shown, theoretically and experimentally, that a hole or an excess electron on a DNA molecule in solution forms a delocalized wave function, a polaron. For an all-adenine (A) sequence or a mixed sequence of guanines (G's) and A's, calculations taking into account the polarization of the solution give the wave function spread over approximately four bases, which appears to be in agreement with experiment. The polaron may move by hopping or by drift.

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We study conductance through a quantum dot under Coulomb blockade conditions in the presence of an external periodic perturbation. The stationary state is determined by the balance between the heating of the dot electrons by the perturbation and cooling by electron exchange with the cold contacts. We show that the Coulomb blockade peak can have a peculiar shape if heating is affected by dynamic localization, which can be an experimental signature of this effect.

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The dynamic localization in energy space, suppression of the absorption of energy from an external microwave field due to quantum interference, was analyzed recently for a closed quantum dot in the absence of electron-electron interactions. Here a weak interaction is shown to lead to a finite absorption and heating, which may be viewed as hopping between localized Floquet states. The heating rate grows together with the electronic temperature, eventually destroying the localization.

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We analyze the response of a complex quantum-mechanical system (e.g., a quantum dot) to a time-dependent perturbation phi(t).

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We address the problem of interplay between self-trapping effects and effects of an external potential, which may be relevant for many physical systems, such as polarons in solids or a Bose-Einstein condensate with attraction. If the potential consists of two different wells, the system initially localized in the shallower well may relax into the deeper well, or may not if stabilized by the self-trapping effect. We show how this picture can be applied to interpret results of recent experiments on electron transfer in the DNA molecule [Giese et al.

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An excess charge on a DNA chain in solution interacts with polar solvent molecules and mobile counterions. We give the first theoretical estimate of the resulting hole self-localization energy and calculate the corresponding contribution to hole mobility on a DNA stack consisting of a single base pair repeated.

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We study the stationary motion of a polaron in a conducting polymer in the presence of a high electric field. Using the Su-Schrieffer-Heeger model plus an electric field, we find that at polaron velocities not exceeding the sound velocity, the dissipation of the electronic energy into the lattice occurs via emission of phonons with single selected wave vector. For this case the corresponding contribution to the polaron mobility can be calculated analytically.

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Hole traps in DNA.

J Am Chem Soc

November 2001

Sequences of guanines, GG and GGG, are known to be readily oxidized, forming radical cations, i.e., hole traps, on DNA.

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