Strong confinement, in all dimensions, and high mechanical frequencies are highly desirable for quantum optomechanical applications. We show that GaAs/AlAs micropillar cavities fully confine not only photons but also extremely high frequency (19-95 GHz) acoustic phonons. A strong increase of the optomechanical coupling upon reducing the pillar size is observed, together with record room-temperature Q-frequency products of 10^{14}.
View Article and Find Full Text PDFPolariton-mediated light-sound interaction is investigated through resonant Brillouin scattering experiments in GaAs/AlAs multiple-quantum wells. Photoelastic coupling enhancement at exciton-polariton resonance reaches 10(5) at 30 K as compared to a typical bulk solid room temperature transparency value. When applied to GaAs based cavity optomechanical nanodevices, this result opens the path to huge displacement sensitivities and to ultrastrong coupling regimes in cavity optomechanics with couplings g(0) in the range of 100 GHz.
View Article and Find Full Text PDFResonators based on acoustic distributed Bragg reflectors (DBRs) were optimized to work in the GHz-THz regime, and grown by molecular beam epitaxy. We show that in structures made of GaAlAs alloys a simultaneous optimal confinement of light in the visible range and phonons in the tens of GHz range can be achieved. We report time resolved differential optical reflectivity experiments performed with fs-ps laser pulses.
View Article and Find Full Text PDFTopological insulators (Bi2Se3) of single- and few-quintuple-layer (few-QLs) films were investigated by Raman spectroscopy and epitaxied on a GaAs substrate. At a measurement temperature of 80 K, we observed the emergence of additional A2u and Eu modes (Raman inactive in the bulk crystal) below 9-QLs film thicknesses, assigned to the crystal-symmetry breakdown in ultrathin films. Furthermore, the out-of-plane A1g modes changed in width, frequency, and intensity for decreasing numbers of QL, while the in-plane Eg mode split into three Raman lines, not resolved in previous room temperature experiments.
View Article and Find Full Text PDFWe present a novel ultra-high resolution Raman spectroscopy technique based in a Fabry-Pérot/triple spectrometer tandem with multichannel acquisition. We describe the system, detail the calibration process, and experimentally test the technique, showing that effective finesses in excess of 1000 are possible. The technique is specifically tailored for low intensity, complex and spectrally extended Raman spectra, providing shorter acquisition times with respect to similar tandem systems with monochannel detectors.
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