Open-aperture Z-scan study for absorption saturation: accurate measurement of saturation intensity in YLF:Yb for optical refrigeration.

Knowledge of saturation intensity of gain or absorption plays a fundamental role in a variety of applications ranging from lasers to many nonlinear optical processes. Here, we present an analytical expression for open-aperture Z-scan transmission for accurately measuring the saturation intensity in the low absorbance samples but at arbitrary pump intensities. We exploit this formalism to investigate the absorption saturation of : (YLF:Yb) in the anti-Stokes excitation region for optical refrigeration at high pump intensities.

Optical refrigeration: the role of parasitic absorption at cryogenic temperatures.

Optical cooling of a YLF:Yb single crystal to 87 K, well below the minimum achievable temperature predicted from existing theory, has been observed. This discrepancy between theory and data has motivated us to revisit the current model of optical refrigeration, in particular the critical role of parasitic background absorption. Challenging experiments that measured the cooling efficiency as a function of temperature reveal that the background absorption coefficient decreases with temperature, resulting in a significant enhancement of the cooling efficiency at cryogenic temperatures.

Tm-doped crystals for mid-IR optical cryocoolers and radiation balanced lasers.

We report the complete characterization of various cooling-grade Tm-doped crystals including, to the best of our knowledge, the first demonstration of optical refrigeration in Tm:YLF crystals. Room temperature laser cooling efficiencies of 1% and 2% (mol) Tm:YLF and 1% Tm:BYF crystals at different excitation polarizations are measured, and their external quantum efficiency and background absorption are extracted. By performing detailed low-temperature spectroscopic analysis of the samples, global minimum achievable temperatures of 160 to 110 K are estimated.

87 fs pulse generation in a diode-pumped semiconductor saturable absorber mirror mode-locked Yb:YLF laser.

A Yb:YLF crystal has been investigated in a femtosecond oscillator pumped by two 400 mW single-mode fiber-coupled diodes emitting at 976 nm and mode locked with a semiconductor saturable absorber mirror. Almost Fourier transform-limited pulses with durations of 87 and 107 fs were demonstrated for extraordinary and ordinary polarizations, respectively. This is, to the best of our knowledge, the first demonstration of sub-100 fs pulses with Yb:YLF, and it proves the potential for ultrashort pulse generation and amplification with this material.

Novel approach for solid state cryocoolers.

Laser cooling in solids is based on anti-Stokes luminescence, via the annihilation of lattice phonons needed to compensate the energy of emitted photons, higher than absorbed ones. Usually the anti-Stokes process is obtained using a rare-earth active ion, like Yb. In this work we demonstrate a novel approach for optical cooling based not only to Yb anti-Stokes cycle but also to virtuous energy-transfer processes from the active ion, obtaining an increase of the cooling efficiency of a single crystal LiYF(4) (YLF) doped Yb at 5at.

Influence of other rare earth ions on the optical refrigeration efficiency in Yb:YLF crystals.

We investigated the effect of rare earth impurities on the cooling efficiency of Yb³⁺:LiYF₄ (Yb:YLF). The refrigeration performance of two single crystals, doped with 5%-at. Yb and with identical history but with different amount of contaminations, have been compared by measuring the cooling efficiency curves.