Superanomalous skin-effect and enhanced absorption of light scattered on conductive media.

Light scattering spectroscopy is a powerful tool for studying various media, but interpretation of its results requires a detailed knowledge of how media excitations are coupled to electromagnetic waves. In electrically conducting media, an accurate description of propagating electromagnetic waves is a non-trivial problem because of non-local light-matter interactions. Among other consequences, the non-locality gives rise to the anomalous (ASE) and superanomalous (SASE) skin effects.

Beyond the Four-Level Model: Dark and Hot States in Quantum Dots Degrade Photonic Entanglement.

Entangled photon pairs are essential for a multitude of quantum photonic applications. To date, the best performing solid-state quantum emitters of entangled photons are semiconductor quantum dots operated around liquid-helium temperatures. To favor the widespread deployment of these sources, it is important to explore and understand their behavior at temperatures accessible with compact Stirling coolers.

Two-Photon Excitation Sets Limit to Entangled Photon Pair Generation from Quantum Emitters.

Entangled photon pairs are key to many novel applications in quantum technologies. Semiconductor quantum dots can be used as sources of on-demand, highly entangled photons. The fidelity to a fixed maximally entangled state is limited by the excitonic fine-structure splitting.

Erratum: Accuracy of the Quantum Regression Theorem for Photon Emission from a Quantum Dot [Phys. Rev. Lett. 127, 100402 (2021)].

This corrects the article DOI: 10.1103/PhysRevLett.127.

Accuracy of the Quantum Regression Theorem for Photon Emission from a Quantum Dot.

The quantum regression theorem (QRT) is the most widely used tool for calculating multitime correlation functions for the assessment of quantum emitters. It is an approximate method based on a Markov assumption for environmental coupling. In this Letter we quantify properties of photons emitted from a single quantum dot coupled to phonons.

Phonon-Induced Enhancement of Photon Entanglement in Quantum Dot-Cavity Systems.

We report on simulations of the degree of polarization entanglement of photon pairs simultaneously emitted from a quantum dot-cavity system that demand revisiting the role of phonons. Since coherence is a fundamental precondition for entanglement and phonons are known to be a major source of decoherence, it seems unavoidable that phonons can only degrade entanglement. In contrast, we demonstrate that phonons can cause a degree of entanglement that even surpasses the corresponding value for the phonon-free case.

Emission-Frequency Separated High Quality Single-Photon Sources Enabled by Phonons.

We demonstrate theoretically that the single-photon purity of photons emitted from a quantum dot exciton prepared by phonon-assisted off-resonant excitation can be significantly higher in a wide range of parameters than that obtained by resonant preparation for otherwise identical conditions. Despite the off-resonant excitation, the brightness stays on a high level. These surprising findings exploit the fact that the phonon-assisted preparation is a two-step process where phonons first lead to a relaxation between laser-dressed states while high exciton occupations are reached only with a delay to the laser pulse maximum by adiabatically undressing the dot states.

Superanomalous Skin Effect for Surface Plasmon Polaritons.

It is commonly assumed that surface plasmon-polariton (SPP) excitations on a metal-dielectric interface decay exponentially inside the metallic sample. Here, we show that in a wide spectral interval the SPP field decays much slower, being inversely proportional to the distance to the interface modified by an additional logarithmic factor. This dependence differs from the standard anomalous skin effect and is provisionally referred to as superanomalous.

Stationary Phonon Squeezing by Optical Polaron Excitation.

We demonstrate that a stationary squeezed phonon state can be prepared by a pulsed optical excitation of a semiconductor quantum well. Unlike previously discussed scenarios for generating squeezed phonons, the corresponding uncertainties become stationary after the excitation and do not oscillate in time. The effect is caused by two-phonon correlations within the excited polaron.

Phonon limited superconducting correlations in metallic nanograins.

Conventional superconductivity is inevitably suppressed in ultra-small metallic grains for characteristic sizes smaller than the Anderson limit. Experiments have shown that above the Anderson limit the critical temperature may be either enhanced or reduced when decreasing the particle size, depending on the superconducting material. In addition, there is experimental evidence that whether an enhancement or a reduction is found depends on the strength of the electron-phonon interaction in the bulk.

Phonon-assisted population inversion of a single InGaAs/GaAs quantum dot by pulsed laser excitation.

We demonstrate a new method to realize the population inversion of a single InGaAs/GaAs quantum dot excited by a laser pulse tuned within the neutral exciton phonon sideband. In contrast to the conventional method of inverting a two-level system by performing coherent Rabi oscillation, the inversion is achieved by rapid thermalization of the optically dressed states via incoherent phonon-assisted relaxation. A maximum exciton population of 0.

The role of phonons for exciton and biexciton generation in an optically driven quantum dot.

For many applications of semiconductor quantum dots in quantum technology, well-controlled state preparation of the quantum dot states is mandatory. Since quantum dots are embedded in the semiconductor matrix, their interaction with phonons often plays a major role in the preparation process. In this review, we discuss the influence of phonons on three basically different optical excitation schemes that can be used for the preparation of exciton, biexciton and superposition states: a resonant excitation leading to Rabi rotations in the excitonic system, an excitation with chirped pulses exploiting the effect of adiabatic rapid passage and an off-resonant excitation giving rise to a phonon-assisted state preparation.

Energy transport and coherence properties of acoustic phonons generated by optical excitation of a quantum dot.

The energy transport of acoustic phonons generated by the optical excitation of a quantum dot as well as the coherence properties of these phonons are studied theoretically both for the case of a pulsed excitation and for a continuous wave (CW) excitation switched on instantaneously. For a pulsed excitation, depending on pulse area and pulse duration, a finite number of phonon wave packets is emitted, while for the case of a CW excitation a sequence of wave packets with decreasing amplitude is generated after the excitation has been switched on. We show that the energy flow associated with the generated phonons is partly related to coherent phonon oscillations and partly to incoherent phonon emission.

Proposed robust and high-fidelity preparation of excitons and biexcitons in semiconductor quantum dots making active use of phonons.

It is demonstrated how the exciton and the biexciton state of a quantum dot can be prepared with high fidelity on a picosecond time scale by driving the dot with a strong laser pulse that is tuned above the exciton resonance for exciton preparation and in resonance with the exciton transition for biexciton preparation. The proposed protocols make use of the phonon-induced relaxation towards photon dressed states in optically driven quantum dots and combine the simplicity of traditional Rabi oscillation schemes with the robustness of adiabatic rapid passage schemes. Our protocols allow for an on-demand, fast, and almost perfect state preparation even at strong carrier-phonon interaction where other schemes fail.

Lattice fluctuations at a double phonon frequency with and without squeezing: an exactly solvable model of an optically excited quantum dot.

Time-dependent lattice fluctuations of an optically excited strongly confined quantum dot are investigated with the aim to analyze the characteristics commonly used for identifying the presence of squeezed phonon states. It is demonstrated that the appearance of fluctuations oscillating with twice the phonon frequency, commonly regarded as a clear indication of squeezed states, cannot be considered as such. The source of the discrepancy with earlier investigations is discussed.

All-optical spin manipulation of a single manganese atom in a quantum dot.

For a CdTe quantum dot doped with a single Mn atom we analyze the dynamics of the Mn spin when the dot is excited by ultrashort laser pulses. Because of the exchange interaction with the Mn atom, electron and hole spins can flip and induce a change of the Mn spin. Including both heavy and light-hole excitons and using suitable pulse sequences, angular momentum can be transferred from the light to the Mn system while the exciton system returns to its ground state.

Nonmonotonic field dependence of damping and reappearance of Rabi oscillations in quantum dots.

The dynamics of strongly confined laser driven semiconductor quantum dots coupled to phonons is studied theoretically by calculating the time evolution of the reduced density matrix using a numerical path integral method. We explore the cases of long pulses, strong dot-phonon and dot-laser coupling, and high temperatures, which, up to now, have been inaccessible. We find that the phonon-induced damping of Rabi rotations is a nonmonotonic function of the laser field that is increasing at low fields and decreasing at high fields.

Estimating the memory time induced by exciton-exciton scattering.

It is shown that lower bounds for the effective memory time induced by two-pair correlations can be estimated by monitoring changes of the shape of excitonic four-wave-mixing spectra. Experimentally we demonstrate a memory time of at least 540 fs for a ZnSe single quantum well. Microscopic calculations reveal that this lower bound is not sharp.

Coherent nonlinear optical response of single quantum dots studied by ultrafast near-field spectroscopy.

The nonlinear response of single GaAs quantum dots is studied in femtosecond near-field pump-probe experiments. At negative time delays, transient reflectivity spectra show pronounced oscillatory structure around the quantum dot exciton line, providing the first evidence for a perturbed free induction decay of the excitonic polarization. Phase-disturbing Coulomb interactions between the excitonic polarization and continuum excitations dominate the optical nonlinearity on ultrafast time scales.

Influence of two-pair continuum correlations following resonant excitation of excitons.

The memory structure induced by coherent transitions to the exciton-exciton scattering continuum is shown to have significant influence on spectrally resolved four-wave-mixing signals even under selective excitation of 1s excitons. Comparisons between experiments and calculations that account nonperturbatively for these quantum kinetic Coulomb correlations demonstrate large compensations between mean-field contributions and transitions to the two-pair continuum. Experiments with different polarizations of the laser pulses show that two-pair continuum correlations are responsible for delay-time dependent shifts of the excitonic emission as well as for substantial deformations of the line shape.

Demonstration of sixth-order coulomb correlations in a semiconductor single quantum well.

Six-wave mixing in a ZnSe quantum well is investigated and compared with microscopic theory. We demonstrate that sixth-order Coulomb correlations have a significant qualitative impact on the nonlinear optical response. Six-wave mixing is shown to be a uniquely sensitive tool for investigation of correlations beyond the four-point level.