A study of controlling the microwave mitigation properties of ferrite-carbon black/PVA composites by tuning the magnetic microstructure and spin arrangement of the ferrite particles is presented. MCoFeO (M: Ni, Mn & Zn) nano-ferrites (NFs) were synthesized by a solvothermal method and these NFs were used to fabricate NF-CB hybrids and flexible NF-CB/PVA composite films. The magnetic force microscopy studies of the NFs reveal a unique single axis oriented domain structure for Zn-NFs and multi-domain magnetic microstructures for Mn-NFs and Ni-NFs.
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