Self-propelled nanoparticles moving through liquids offer the possibility of creating advanced applications where such nanoswimmers can operate as artificial molecular-sized motors. Achieving control over the motion of nanoswimmers is a crucial aspect for their reliable functioning. While the directionality of micron-sized swimmers can be controlled with great precision, steering nano-sized active particles poses a real challenge.
View Article and Find Full Text PDFCollective particle transport across periodic energy landscapes is ubiquitously present in many condensed matter systems spanning from vortices in high-temperature superconductors, frictional atomic sliding, driven skyrmions to biological and active matter. Here we report the emergence of fast solitons propagating against a rotating optical landscape. These experimentally observed solitons are stable cluster waves that originate from a coordinated particle exchange process which occurs when the number of trapped microparticles exceeds the number of potential wells.
View Article and Find Full Text PDFSingle-file transport occurs in various scientific fields, including diffusion through nanopores, nanofluidic devices, and cellular processes. We here investigate the impact of polydispersity on particle currents for single-file Brownian motion of hard spheres when they are driven through periodic potentials by a constant drag force. Through theoretical analysis and extensive Brownian dynamics simulations, we unveil the behavior of particle currents for random binary mixtures.
View Article and Find Full Text PDFSingle-file diffusion refers to the Brownian motion in narrow channels where particles cannot pass each other. In such processes, the diffusion of a tagged particle is typically normal at short times and becomes subdiffusive at long times. For hard-sphere interparticle interaction, the time-dependent mean squared displacement of a tracer is well understood.
View Article and Find Full Text PDFWe propose a simulation method for Brownian dynamics of hard rods in one dimension for arbitrary continuous external force fields. It is an event-driven procedure based on the fragmentation and mergers of clusters formed by particles in contact. It allows one to treat particle interactions in addition to the hard-sphere exclusion as long as the corresponding interaction forces are continuous functions of the particle coordinates.
View Article and Find Full Text PDFThe flow-driven transport of interacting micron-sized particles occurs in many soft matter systems spanning from the translocation of proteins to moving emulsions in microfluidic devices. Here we combine experiments and theory to investigate the collective transport properties of colloidal particles along a rotating ring of optical traps. In the corotating reference frame, the particles are driven by a vortex flow of the surrounding fluid.
View Article and Find Full Text PDFCatalytically active macromolecules are envisioned as key building blocks in the development of artificial nanomotors. However, theory and experiments report conflicting findings regarding their dynamics. The lack of consensus is mostly caused by the limited understanding of the specifics of self-propulsion mechanisms at the nanoscale.
View Article and Find Full Text PDFSolitons are commonly known as waves that propagate without dispersion. Here, we show that they can occur for driven overdamped Brownian dynamics of hard spheres in periodic potentials at high densities. The solitons manifest themselves as periodic sequences of different assemblies of particles moving in the limit of zero noise, where transport of single particles is not possible.
View Article and Find Full Text PDFThe physics of self-propelled objects at the nanoscale is a rapidly developing research field where recent experiments have focused on the motion of individual catalytic enzymes. Contrary to the experimental advancements, theoretical understanding of the possible self-propulsion mechanisms at these scales is limited. A particularly puzzling question concerns the origins of the reportedly high diffusivities of the individual enzymes.
View Article and Find Full Text PDFHydrodynamic interactions between fluid-dispersed particles are ubiquitous in soft matter and biological systems and they give rise to intriguing collective phenomena. While it was reported that these interactions can facilitate force-driven particle motion over energetic barriers, here we show the opposite effect in a flow-driven system, i.e.
View Article and Find Full Text PDFSingle-file transport in pore-like structures constitutes an important topic for both theory and experiment. For hardcore interacting particles, a good understanding of the collective dynamics has been achieved recently. Here, we study how softness in the particle interaction affects the emergent transport behavior.
View Article and Find Full Text PDFRecent measurements of the durations of nonequilibrium processes provide valuable information on microscopic mechanisms and energetics. Theory for corresponding experiments to date is well-developed for single-particle systems only. Little is known for interacting systems in nonequilibrium environments.
View Article and Find Full Text PDFSingle-file Brownian motion in periodic structures is an important process in nature and technology, which becomes increasingly amenable for experimental investigation under controlled conditions. To explore and understand generic features of this motion, the Brownian asymmetric simple exclusion process (BASEP) was recently introduced. The BASEP refers to diffusion models where hard spheres are driven by a constant drag force through a periodic potential.
View Article and Find Full Text PDFCoherent quantum oscillators are basic physical systems both in quantum statistical physics and quantum thermodynamics. Their realizations in lab often involve solid-state devices sensitive to changes in ambient temperature. We represent states of the solid-state optomechanical oscillator with temperature-dependent frequency by equivalent states of the mechanical oscillator with temperature-dependent energy levels.
View Article and Find Full Text PDFStochastic motion of particles in a highly unstable potential generates a number of diverging trajectories leading to undefined statistical moments of the particle position. This makes experiments challenging and breaks down a standard statistical analysis of unstable mechanical processes and their applications. A newly proposed approach takes advantage of the local characteristics of the most probable particle motion instead of the divergent averages.
View Article and Find Full Text PDFWe study the driven Brownian motion of hard rods in a one-dimensional cosine potential with a large amplitude compared to the thermal energy. In a closed system, we find surprising features of the steady-state current in dependence of the particle density. The form of the current-density relation changes greatly with the particle size and can exhibit both a local maximum and minimum.
View Article and Find Full Text PDFAccording to the laws of thermodynamics, no heat engine can beat the efficiency of a Carnot cycle. This efficiency traditionally comes with vanishing power output and practical designs, optimized for power, generally achieve far less. Recently, various strategies to obtain Carnot's efficiency at large power were proposed.
View Article and Find Full Text PDFThe trajectories of an overdamped particle in a highly unstable potential diverge so rapidly, that the variance of position grows much faster than its mean. A description of the dynamics by moments is therefore not informative. Instead, we propose and analyze local directly measurable characteristics, which overcome this limitation.
View Article and Find Full Text PDFPhys Rev E
December 2017
We discuss the possibility of reaching the Carnot efficiency by heat engines (HEs) out of quasistatic conditions at nonzero power output. We focus on several models widely used to describe the performance of actual HEs. These models comprise quantum thermoelectric devices, linear irreversible HEs, minimally nonlinear irreversible HEs, HEs working in the regime of low-dissipation, overdamped stochastic HEs and an underdamped stochastic HE.
View Article and Find Full Text PDFWe investigate fluctuations of output work for a class of Stirling heat engines with working fluid composed of interacting units and compare these fluctuations to an average work output. In particular, we focus on engine performance close to a critical point where Carnot's efficiency may be attained at a finite power as reported by M. Campisi and R.
View Article and Find Full Text PDFRecent technological progress in a precise control of optically trapped objects allows much broader ventures to unexplored territory of thermal motion in non-linear potentials. In this work, we exploit an experimental set-up of holographic optical tweezers to experimentally investigate Brownian motion of a micro-particle near the inflection point of the cubic optical potential. We present two complementary views on the non-linear Brownian motion.
View Article and Find Full Text PDFWe discuss the statistics of first-passage times of a Brownian particle moving in a highly unstable nonlinear potential proportional to an odd power of position. We observe temperature-induced shortening of the mean first-passage time and its dependence on the power of nonlinearity. We propose a passage-time fraction as both a simple and experimentally detectable witness of the nonlinearity.
View Article and Find Full Text PDFWe discuss the efficiency of a heat engine operating in a nonequilibrium steady state maintained by two heat reservoirs. Within the general framework of linear irreversible thermodynamics we derive a universal upper bound on the efficiency of the engine operating at arbitrary fixed power. Furthermore, we show that a slight decrease of the power below its maximal value can lead to a significant gain in efficiency.
View Article and Find Full Text PDFPhys Rev E Stat Nonlin Soft Matter Phys
November 2015
A universality in optimization of trade-off between power and efficiency for low-dissipation Carnot cycles is presented. It is shown that any trade-off measure expressible in terms of efficiency and the ratio of power to its maximum value can be optimized independently of most details of the dynamics and of the coupling to thermal reservoirs. The result is demonstrated on two specific trade-off measures.
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