The Kathmandu valley experiences an average wintertime PM concentration of ∼100 μg m and daily peaks over 200 μg m. We present ambient nonrefractory PM chemical composition, and concentration measured by a mini aerosol mass spectrometer (mAMS) sequentially at Dhulikhel (on the valley exterior), then urban Ratnapark, and finally suburban Lalitpur in winter 2018. At all sites, organic aerosol (OA) was the largest contributor to combined PM (C-PM) (49%) and black carbon (BC) was the second largest contributor (21%).
View Article and Find Full Text PDFThe Kathmandu Valley in Nepal experiences poor air quality, especially in the dry winter season. In this study, we investigated the concentration, chemical composition, and sources of fine and coarse particulate matter (PM, PM, and PM) at three sites within or near the Kathmandu Valley during the winter of 2018 as part of the second Nepal Ambient Monitoring and Source Testing Experiment (NAMaSTE 2). Daily PM concentrations were very high throughout the study period, ranging 72-149 μg m at the urban Ratnapark site in Kathmandu, 88-161 μg m at the suburban Lalitpur site, and 40-74 μg m at rural Dhulikhel on the eastern rim of the Kathmandu Valley.
View Article and Find Full Text PDFUnit mass resolution mass spectral profiles of nonrefractory submicron aerosol were retrieved from undersampled atmospheric emission sources common to South Asia using a "mini" aerosol mass spectrometer. Emission sources including wood- and dung-fueled cookstoves, agricultural residue burning, garbage burning, engine exhaust, and coal-fired brick kilns were sampled during the 2015 Nepal Ambient Monitoring and Source Testing Experiment (NAMaSTE) campaign. High-resolution peak fitting estimates of the mass spectra were used to characterize ions found within each source profile and help identify mass spectral signatures unique to aerosol emissions from the investigated source types.
View Article and Find Full Text PDFThis paper reports the chemical and light extinction characteristics of fine aerosol (PM) during the winter period (2017-18) at Lumbini, Nepal, a rural site on the Indo Gangetic Plains. A modified IMPROVE algorithm was employed to reconstruct light extinction by chemical constituents of aerosol. The fine aerosol levels impacted visibility adversely during daytime, but during nighttime visibility was controlled by fog droplets rather than by aerosols.
View Article and Find Full Text PDFEnviron Sci Technol
August 2020
Increasing air pollution in South Asia has serious consequences for air quality and human/ecosystem health within the region. South Asia, including India and Nepal, suffers from severe air pollution, including high concentrations of aerosols, as well as gaseous pollutants. One of the often-neglected sources contributing to the regional air pollution is garbage burning.
View Article and Find Full Text PDFThis study presents a comprehensive analysis of organic carbon (OC), elemental carbon (EC), and particularly the light absorption characteristics of EC and water-soluble brown carbon (WS-BrC) in total suspended particles in the Kathmandu Valley from April 2013 to January 2018. The mean OC, EC, and water-soluble organic carbon (WSOC) concentrations were 34.8 ± 27.
View Article and Find Full Text PDFTotal suspended particles (TSP) were collected in Lumbini from April 2013 to March 2016 to better understand the characteristics of carbonaceous aerosol (CA) concentrations, compositions and sources and their light absorption properties in rural region of severe polluted Indo-Gangetic Plain (IGP). Extremely high TSP (203.9 ± 109.
View Article and Find Full Text PDFCarbonaceous aerosols (CAs) scatter and absorb incident solar radiation in the atmosphere, thereby influencing the regional climate and hydrological cycle, particularly in the Third Pole (TP). Here, we present the characteristics of CAs at 19 observation stations from the Atmospheric Pollution and Cryospheric Change network to obtain a deep understanding of pollutant status in the TP. The organic carbon (OC) and elemental carbon (EC) concentrations decreased noticeably inwards from outside to inland of the TP, consistent with their emission load and also affected by transport process and meteorological condition.
View Article and Find Full Text PDFThe Tibetan Plateau and its surroundings are known as the Third Pole (TP). This region is noted for its high rates of glacier melt and the associated hydrological shifts that affect water supplies in Asia. Atmospheric pollutants contribute to climatic and cryospheric changes through their effects on solar radiation and the albedos of snow and ice surfaces; moreover, the behavior and fates within the cryosphere and environmental impacts of environmental pollutants are topics of increasing concern.
View Article and Find Full Text PDFBrown carbon (BrC) has recently emerged as an important light-absorbing aerosol. This study provides interannual and seasonal variations in light absorption properties, chemical composition, and sources of water-soluble BrC (WS-BrC) based on PM samples collected in Godavari, Nepal, from April 2012 to May 2014. The mass absorption efficiency of WS-BrC at 365 nm (MAE) shows a clear seasonal variability, with the highest MAE of 1.
View Article and Find Full Text PDFFor the first time, aerosol optical properties are measured over Lumbini, Nepal, with CIMEL sunphotometer of the Aerosol Robotic Network (AERONET) program. Lumbini is a sacred place as the birthplace of Lord Buddha, and thus a UNESCO world heritage site, located near the northern edge of the central Indo-Gangetic Plains (IGP) and before the Himalayan foothills (and Himalayas) to its north. Average aerosol optical depth (AOD) is found to be 0.
View Article and Find Full Text PDFThe Kathmandu Valley, located in the Himalayan foothills in Nepal, is heavily polluted. In order to investigate ambient particulate-bound mercury (Hg) in the Kathmandu Valley, a total 64 total suspended particulates (TSP) samples were collected from a sub-urban site in the Kathmandu Valley, the capital region of Nepal during a sampling period of an entire year (April 2013-April 2014). They were analyzed for ambient particulate-bound Hg (PBM) using thermal desorption combined with cold vapor atomic spectroscopy.
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