Long-term effects of silver nanoparticles and mineral nutrition components on the photosynthetic processes, chloroplast ultrastructure and productivity of Solanum lycopersicum plants.

The effects of silver nanoparticles (AgNPs), both alone and in combination with mineral nutrients, on the growth and photosynthesis of Solanum lycopersicum plants during ontogeny were studied. The experiment involved weekly applications of 10 μmol of AgNPs for 15 weeks in a greenhouse over a summer period. A comprehensive characterization of the AgNPs was performed via TEM, ESI/EELS, and zeta potential measurements before and throughout the experiment.

Bragg-like microcavity formed by collision of single-cycle self-induced transparency light pulses in a resonant medium.

The coherent interaction of extremely short light pulses with a resonant medium can result in the formation of population difference gratings. Such gratings have been created by pulses that are π/2 or smaller. This paper demonstrates that a microcavity with Bragg-like mirrors can be formed by colliding two single-cycle attosecond self-induced transparency pulses in the center of a two-level medium.

Sub-10 fs unipolar pulses of a tailored waveshape from a multilevel resonant medium.

We theoretically demonstrate the possibility to tune the temporal waveform of unipolar pulses of femtosecond duration emitted from a multilevel resonant medium. This is achieved through the control of the medium response by a properly adjusted sequence of half-cycle unipolar or quasi-unipolar driving pulses and the spatial density profile of resonant centers along the medium layer. We show the production of unipolar optical pulses of varying profiles, like rectangular or triangular ones, from an extended layer of a multilevel medium.

Generation of an ultrahigh-repetition-rate optical half-cycle pulse train in the nested quantum wells.

We propose a simple quantum system, namely, a nested quantum-well structure, which is able to generate a train of half-cycle pulses of a few-femtosecond duration when driven by a static electric field. We theoretically investigate the emission of such a structure and its dependence on the parameters of the quantum wells. It is shown that the production of a regular output pulse train with tunable properties and the pulse repetition frequencies of tens of terahertz is possible in certain parameter ranges.

Micellar and solubilizing properties of rhamnolipids.

We studied the micellar and solubilizing properties of aqueous solutions of unfractionated rhamnolipids produced by Pseudomonas aeruginosa. We used nuclear magnetic resonance (NMR) diffusometry, dynamic light scattering, and conductometry to measure the critical micelle concentration (CMC) of rhamnolipid solutions and determined the effective hydrodynamic radii of rhamnolipid monomers and micelles. Based on selective measurements of the self-diffusion coefficients of molecules, performed by NMR diffusometry, the solubilizing properties of rhamnolipids were studied depending on their concentration in solution; aromatic hydrocarbons, benzene, toluene, ethylbenzene, and para-xylene were taken as solubilizates.

Self-Stopping of Light.

Here, we show that light can bring itself to a complete standstill (self-stop) via self-interaction mediated by the resonant nonlinearity in a fully homogeneous medium. An intense few-cycle pulse, entering the medium, may reshape to form a strongly coupled light-matter bundle, in which the energy is transferred from light to the medium and back periodically on the single-cycle scale. Such oscillating structure can decelerate, alter its propagation direction, and even completely stop, depending on the state of its internal degrees of freedom.

Dynamic and molecular association in premicellar aqueous solutions of dicarboxylate amino acid-based surfactant as studied by H NMR.

We examined a series of amino acid-based surfactants with two carboxylic groups separated by a spacer of one, two, or three carbon atoms with sodium and calcium counterions in the premicellar concentration region near the CMC. H nuclear magnetic resonance (NMR) spectroscopy and NMR diffusometry techniques were used to study the local environment, association, and translational dynamics of the surfactant's molecules. We measured the self-diffusion coefficients of the micelles, calculated the effective hydrodynamic radii, and determined the temperature region in which the premicelles exist.

Temporal differentiation and integration of few-cycle pulses by ultrathin metallic films.

We study theoretically the temporal transformations of few-cycle pulses upon linear interaction with ultrathin metallic films. We show that under certain conditions on the film thickness and the pulse spectrum, one obtains the temporal differentiation of the pulse shape in transmission and the temporal integration in reflection. In contrast to previous studies, these transformations are obtained for the field of few-cycle pulses itself instead of the slowly varying pulse envelope.

Study of the premicellar state in aqueous solutions of sodium dodecyl sulfate by nuclear magnetic resonance diffusion.

Self-diffusion coefficients of sodium dodecyl sulfate (SDS) were measured in aqueous solutions in the premicellar range of the SDS concentrations 7-34.7 mM and temperatures 30-90°C. Average effective hydrodynamic radii and aggregation numbers of SDS in the premicellar region were determined.

Single-cycle pulse compression in dense resonant media.

We propose here a new approach for compression and frequency up-conversion of short optical pulses in the regime of extreme nonlinear optics in optically dense absorbing media, providing an alternative route to attosecond-scale pulses at high frequencies. This method is based on dynamics of self-induced transparency (SIT) pulses of nearly single cycle duration, leading to single-cycle-scale Rabi oscillations in the medium. The sub-cycle components of an incident pulse behave as separate SIT-pulses, approaching each other and self-compressing, resulting in the threefold compression in time and frequency up-conversion by the same factor.

Stable coherent mode-locking based on [Formula: see text] pulse formation in single-section lasers.

Here we consider coherent mode-locking (CML) regimes in single-section cavity lasers, taking place for pulse durations less than atomic population and phase relaxation times, which arise due to coherent Rabi oscillations of the atomic inversion. Typically, CML is introduced for lasers with two sections, the gain and absorber ones. Here we show that, for certain combination of the cavity length and relaxation parameters, a very stable CML in a laser, containing only gain section, may arise.

Micelles of Oxyethylated Isononylphenols in Aqueous Solutions and Hydrophilic-Lipophilic Balance.

We have measured the self-diffusion coefficients and calculated the effective hydrodynamic radii of micelles of ethoxylated isononylphenols in aqueous solutions in the presence of sodium chloride, as well as in their binary mutual mixtures, when approaching cloudy conditions. These cloudy conditions were created by an increase in temperature, a change in the concentration of an electrolyte in the solution, or a mutual ratio of neonols in their binary mixtures. The results are discussed within the concept of the hydrophilic-lipophilic balance.

Selective ultrafast control of multi-level quantum systems by subcycle and unipolar pulses.

The most typical way to optically control population of atomic and molecular systems is to illuminate them with radiation, resonant to the relevant transitions. Here we consider a possibility to control populations with the subcycle and even unipolar pulses, containing less than one oscillation of electric field. Despite the spectrum of such pulses covers several levels at once, we show that it is possible to selectively excite the levels of our choice by varying the driving pulse shape, duration or time delay between consecutive pulses.

Unusual terahertz waveforms from a resonant medium controlled by diffractive optical elements.

Up to now, full tunability of waveforms was possible only in electronics, up to radio-frequencies. Here we propose a new concept of producing few-cycle terahertz (THz) pulses with widely tunable waveforms. It is based on control of the phase delay between different parts of the THz wavefront using linear diffractive optical elements.

Unipolar subcycle pulse-driven nonresonant excitation of quantum systems.

The interaction of subcycle pulses with quantum systems is considered when the pulse duration becomes much smaller than the timescales of electron oscillations. We show analytically that the interaction process in this case is governed by the electric pulse area. The efficient nonresonant excitation of quantum systems by subcycle pulses with a high degree of unipolarity is demonstrated.

Population density gratings induced by few-cycle optical pulses in a resonant medium.

Creation, erasing and ultrafast control of population density gratings using few-cycle optical pulses coherently interacting with resonant medium is discussed. In contrast to the commonly used schemes, here the pulses do not need to overlap in the medium, interaction between the pulses is mediated by excitation of polarization waves. We investigate the details of the dynamics arising in such ultrashort pulse scheme and develop an analytical theory demonstrating the importance of the phase memory effects in the dynamics.

Generation of unipolar half-cycle pulses via unusual reflection of a single-cycle pulse from an optically thin metallic or dielectric layer.

We propose a strikingly simple method to form approximately unipolar half-cycle optical pulses via reflection of a single-cycle optical pulse from a thin flat metallic or dielectric layer. Unipolar pulses in reflection arise due to specifics of one-dimensional pulse propagation. Namely, we show that the field emitted by the layer is proportional to the velocity of the oscillating charges in the medium, instead of their acceleration.

Ultrafast creation and control of population density gratings via ultraslow polarization waves.

In the regime of resonant coherent light-matter interaction, light pulses may interact with each other indirectly via a polarization wave created by the other pulse. We show that such interaction allows fast creation and erasing of high-contrast dynamic population density gratings, as well as control of their period in a few-cycle regime. Our scheme uses counter-propagating optical pulses, which do not cross each other in the medium.

Self-induced transparency mode locking, and area theorem.

Self-induced transparency mode locking (or coherent mode locking, CML), which is based on intracavity self-induced transparency soliton dynamics, potentially allows achievement of nearly single-cycle intracavity pulse durations, much below the phase relaxation time T in a laser which, despite having great promise, has not yet been realized experimentally. We develop a diagram technique which allows us to predict the main features of CML regimes in a generic two-section laser far from the single-cycle limit. We show that CML can arise directly at the first laser threshold if the phase relaxation time is large enough.

Quantum dash based single section mode locked lasers for photonic integrated circuits.

We present the first demonstration of an InAs/InP Quantum Dash based single-section frequency comb generator designed for use in photonic integrated circuits (PICs). The laser cavity is closed using a specifically designed Bragg reflector without compromising the mode-locking performance of the self pulsating laser. This enables the integration of single-section mode-locked laser in photonic integrated circuits as on-chip frequency comb generators.