We report a nonlinear terahertz (THz) detection device based on a metallic bull's-eye plasmonic antenna. The antenna, fabricated with femtosecond laser direct writing and deposited on a nonlinear gallium phosphide (GaP) crystal, focuses incoming THz waveforms within the sub-wavelength bull's eye region to locally enhance the THz field. Additionally, the plasmonic structure minimizes diffraction effects allowing a relatively long interaction length between the transmitted THz field and the co-propagating near-infrared gating pulse used in an electro-optic sampling configuration.
View Article and Find Full Text PDFWe combine parametric frequency upconversion with the single-photon counting technology to achieve terahertz (THz) detection sensitivity down to the zeptojoule (zJ) pulse energy level. Our detection scheme employs a near-infrared ultrafast source, a GaP nonlinear crystal, optical filters, and a single-photon avalanche diode. This configuration is able to resolve 1.
View Article and Find Full Text PDFWe demonstrate a table-top high-field terahertz (THz) source based on optical rectification of a collimated near-infrared pulse in gallium phosphide (GaP) to produce peak fields above 300 kV/cm with a spectrum centered at 2.6 THz. The experimental configuration, based on tilted-pulse-front phase matching, is implemented with a phase grating etched directly onto the front surface of the GaP crystal.
View Article and Find Full Text PDFTerahertz time-domain spectroscopy (THz-TDS) is a powerful technique that enables the characterization of a large range of bulk materials, devices, and products. Although this technique has been increasingly used in research and industry, the standard THz-TDS configuration relying on the use of a near-infrared (NIR) laser source remains experimentally complex and relatively costly, impeding its availability to those without the expertise to build a high-performance setup based on nonlinear optics or without the financial means to acquire a commercial unit. Broadband THz-TDS systems require an even larger financial investment, primarily because the generation and detection of spectral components exceeding 3 THz typically need an ultrafast NIR source delivering sub-100-fs pulses.
View Article and Find Full Text PDFSlow motion movies allow us to see intricate details of the mechanical dynamics of complex phenomena. If the images in each frame are replaced by terahertz (THz) waves, such movies can monitor low-energy resonances and reveal fast structural or chemical transitions. Here, we combine THz spectroscopy as a non-invasive optical probe with a real-time monitoring technique to demonstrate the ability to resolve non-reproducible phenomena at 50k frames per second, extracting each of the generated THz waveforms every 20 μs.
View Article and Find Full Text PDFA detection efficiency measurement system for free-space single-photon detectors has been established at the National Research Council (NRC) Canada. This measurement apparatus incorporates an 850 nm fiber laser source and utilizes a double-attenuation and substitution calibration technique. Detection efficiency calibrations of silicon single-photon avalanche photodiodes (SPADs) at incident photon rates in the range of 1.
View Article and Find Full Text PDFThe application of femtosecond four-wave mixing to the study of fundamental properties of diluted magnetic semiconductors ((s,p)-d hybridization, spin-flip scattering) is described, using experiments on GaMnAs as a prototype III-Mn-V system. Spectrally-resolved and time-resolved experimental configurations are described, including the use of zero-background autocorrelation techniques for pulse optimization. The etching process used to prepare GaMnAs samples for four-wave mixing experiments is also highlighted.
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