Superradiant and Subradiant Cavity Scattering by Atom Arrays.

We realize collective enhancement and suppression of light scattered by an array of tweezer-trapped ^{87}Rb atoms positioned within a strongly coupled Fabry-Pérot optical cavity. We illuminate the array with light directed transverse to the cavity axis, in the low saturation regime, and detect photons scattered into the cavity. For an array with integer-optical-wavelength spacing each atom scatters light into the cavity with nearly identical scattering amplitude, leading to an observed N^{2} scaling of cavity photon number as the atom number increases stepwise from N=1 to N=8.

All-dielectric scale invariant waveguide.

Total internal reflection (TIR) governs the guiding mechanisms of almost all dielectric waveguides and therefore constrains most of the light in the material with the highest refractive index. The few options available to access the properties of lower-index materials include designs that are either lossy, periodic, exhibit limited optical bandwidth or are restricted to subwavelength modal volumes. Here, we propose and demonstrate a guiding mechanism that leverages symmetry in multilayer dielectric waveguides as well as evanescent fields to strongly confine light in low-index materials.

Many-Body Superradiance and Dynamical Mirror Symmetry Breaking in Waveguide QED.

The many-body decay of extended collections of two-level systems remains an open problem. Here, we investigate whether an array of emitters coupled to a one-dimensional bath undergoes Dicke superradiance. This is a process whereby a completely inverted system becomes correlated via dissipation, leading to the release of all the energy in the form of a rapid photon burst.

Dicke Superradiance Requires Interactions beyond Nearest Neighbors.

Photon-mediated interactions within an excited ensemble of emitters can result in Dicke superradiance, where the emission rate is greatly enhanced, manifesting as a high-intensity burst at short times. The superradiant burst is most commonly observed in systems with long-range interactions between the emitters, although the minimal interaction range remains unknown. Here, we put forward a new theoretical method to bound the maximum emission rate by upper bounding the spectral radius of an auxiliary Hamiltonian.

Universality of Dicke superradiance in arrays of quantum emitters.

Dicke superradiance is an example of emergence of macroscopic quantum coherence via correlated dissipation. Starting from an initially incoherent state, a collection of excited atoms synchronizes as they decay, generating a macroscopic dipole moment and emitting a short and intense pulse of light. While well understood in cavities, superradiance remains an open problem in extended systems due to the exponential growth of complexity with atom number.

Enhanced tunable second harmonic generation from twistable interfaces and vertical superlattices in boron nitride homostructures.

Broken symmetries induce strong even-order nonlinear optical responses in materials and at interfaces. Unlike conventional covalently bonded nonlinear crystals, van der Waals (vdW) heterostructures feature layers that can be stacked at arbitrary angles, giving complete control over the presence or lack of inversion symmetry at a crystal interface. Here, we report highly tunable second harmonic generation (SHG) from nanomechanically rotatable stacks of bulk hexagonal boron nitride (BN) crystals and introduce the term twistoptics to describe studies of optical properties in twistable vdW systems.

Many-Body Signatures of Collective Decay in Atomic Chains.

Fully inverted atoms placed at exactly the same location synchronize as they deexcite, and light is emitted in a burst (known as "Dicke's superradiance"). We investigate the role of finite interatomic separation on correlated decay in mesoscopic chains and provide an understanding in terms of collective jump operators. We show that the superradiant burst survives at small distances, despite Hamiltonian dipole-dipole interactions.

Optical waveguiding by atomic entanglement in multilevel atom arrays.

The optical properties of subwavelength arrays of atoms or other quantum emitters have attracted significant interest recently. For example, the strong constructive or destructive interference of emitted light enables arrays to function as nearly perfect mirrors, support topological edge states, and allow for exponentially better quantum memories. In these proposals, the assumed atomic structure was simple, consisting of a unique electronic ground state.

Cavity quantum electrodynamics with atom-like mirrors.

It has long been recognized that atomic emission of radiation is not an immutable property of an atom, but is instead dependent on the electromagnetic environment and, in the case of ensembles, also on the collective interactions between the atoms. In an open radiative environment, the hallmark of collective interactions is enhanced spontaneous emission-super-radiance-with non-dissipative dynamics largely obscured by rapid atomic decay. Here we observe the dynamical exchange of excitations between a single artificial atom and an entangled collective state of an atomic array through the precise positioning of artificial atoms realized as superconducting qubits along a one-dimensional waveguide.

Atom-atom interactions around the band edge of a photonic crystal waveguide.

Tailoring the interactions between quantum emitters and single photons constitutes one of the cornerstones of quantum optics. Coupling a quantum emitter to the band edge of a photonic crystal waveguide (PCW) provides a unique platform for tuning these interactions. In particular, the cross-over from propagating fields [Formula: see text] outside the bandgap to localized fields [Formula: see text] within the bandgap should be accompanied by a transition from largely dissipative atom-atom interactions to a regime where dispersive atom-atom interactions are dominant.

3D plasmonic chiral colloids.

3D plasmonic chiral colloids are synthesized through deterministically grouping of two gold nanorod AuNRs on DNA origami. These nanorod crosses exhibit strong circular dichroism (CD) at optical frequencies which can be engineered through position tuning of the rods on the origami. Our experimental results agree qualitatively well with theoretical predictions.

Three-dimensional plasmonic chiral tetramers assembled by DNA origami.

Molecular chemistry offers a unique toolkit to draw inspiration for the design of artificial metamolecules. For a long time, optical circular dichroism has been exclusively the terrain of natural chiral molecules, which exhibit optical activity mainly in the UV spectral range, thus greatly hindering their significance for a broad range of applications. Here we demonstrate that circular dichroism can be generated with artificial plasmonic chiral nanostructures composed of the minimum number of spherical gold nanoparticles required for three-dimensional (3D) chirality.

Alternating Plasmonic Nanoparticle Heterochains Made by Polymerase Chain Reaction and Their Optical Properties.

Organization of nanoparticles (NPs) of different materials into superstructures of higher complexity represents a key challenge in nanotechnology. Polymerase chain reaction (PCR) was used in this study to fabricate chains consisting of plasmonic NPs of different sizes, thus denoted heterochains. The NPs in such chains are connected by DNA oligomers, alternating in a sequence big-small-big-small-.

Stimulated light emission and inelastic scattering by a classical linear system of rotating particles.

The rotational dynamics of particles subject to external illumination is found to produce light amplification and inelastic scattering at high rotation velocities. Light emission at frequencies shifted with respect to the incident light by twice the rotation frequency dominates over elastic scattering within a wide range of light and rotation frequencies. Remarkably, net amplification of the incident light is produced in this classical linear system via stimulated emission.

Multiphoton absorption and emission by interaction of swift electrons with evanescent light fields.

We introduce a theory to describe the interaction of swift electrons with strong evanescent light fields. This allows us to explain recent experimental results of multiple energy losses and gains for electrons passing near illuminated nanostructures. A complex evolution of the electron state over attosecond time scales is unveiled, giving rise to non-Poissonian distributions of multiphoton features in the electron spectra.

Rotating beams in isotropic optical system.

Based on the ray transformation matrix formalism, we propose a simple method for generation of paraxial beams performing anisotropic rotation in the phase space during their propagation through isotropic optical systems. The widely discussed spiral beams are the particular case of these beams. The propagation of these beams through the symmetric fractional Fourier transformer is demonstrated by numerical simulations.