Highly efficient deep UV generation by four-wave mixing in gas-filled hollow-core photonic crystal fiber.

We report on a highly efficient experimental scheme for the generation of deep-ultraviolet (UV) ultrashort light pulses using four-wave mixing in gas-filled kagomé-style photonic crystal fiber. By pumping with ultrashort, few microjoule pulses centered at 400 nm, we generate an idler pulse at 266 nm and amplify a seeded signal at 800 nm. We achieve remarkably high pump-to-idler energy conversion efficiencies of up to 38%.

Monitoring the Wobbe Index of Natural Gas Using Fiber-Enhanced Raman Spectroscopy.

The fast and reliable analysis of the natural gas composition requires the simultaneous quantification of numerous gaseous components. To this end, fiber-enhanced Raman spectroscopy is a powerful tool to detect most components in a single measurement using a single laser source. However, practical issues such as detection limit, gas exchange time and background Raman signals from the fiber material still pose obstacles to utilizing the scheme in real-world settings.

Broadband high-resolution multi-species CARS in gas-filled hollow-core photonic crystal fiber.

We report the use of coherent anti-Stokes Raman spectroscopy (CARS) in gas-filled hollow-core photonic crystal fiber (HC-PCF) for trace gas detection. The long optical path-lengths yield a 60 dB increase in the signal level compared with free-space arrangements. This enables a relatively weak supercontinuum (SC) to be used as Stokes seed, along with a ns pump pulse, paving the way for broadband (>4000  cm) single-shot CARS with an unprecedented resolution of ∼100  MHz.

Generation of spectral clusters in a mixture of noble and Raman-active gases: publisher's note.

This note points out a correction to a typographical error in the published version of the article [Opt. Lett.41, 5543 (2016)OPLEDP0146-959210.

Generation of spectral clusters in a mixture of noble and Raman-active gases.

We report a novel scheme for the generation of dense clusters of Raman sidebands. The scheme uses a broadband-guiding hollow-core photonic crystal fiber (HC-PCF) filled with a mixture of H, D, and Xe for efficient interaction between the gas mixture and a green laser pump pulse (532 nm, 1 ns) of only 5 μJ of energy. This results in the generation from noise of more than 135 rovibrational Raman sidebands covering the visible spectral region with an average spacing of only 2.

Raman-induced temporal condensed matter physics in gas-filled photonic crystal fibers.

Raman effect in gases can generate an extremely long-living wave of coherence that can lead to the establishment of an almost perfect temporal periodic variation of the medium refractive index. We show theoretically and numerically that the equations, regulate the pulse propagation in hollow-core photonic crystal fibers filled by Raman-active gas, are exactly identical to a classical problem in quantum condensed matter physics - but with the role of space and time reversed - namely an electron in a periodic potential subject to a constant electric field. We are therefore able to infer the existence of Wannier-Stark ladders, Bloch oscillations, and Zener tunneling, phenomena that are normally associated with condensed matter physics, using purely optical means.

Raman amplification of pure side-seeded higher-order modes in hydrogen-filled hollow-core PCF.

We use Raman amplification in hydrogen-filled hollow-core kagomé photonic crystal fiber to generate high energy pulses in pure single higher-order modes. The desired higher-order mode at the Stokes frequency is precisely seeded by injecting a pulse of light from the side, using a prism to select the required modal propagation constant. An intense pump pulse in the fundamental mode transfers its energy to the Stokes seed pulse with measured gains exceeding 60 dB and output pulse energies as high as 8 µJ.

Selective excitation of higher order modes in hollow-core PCF via prism-coupling.

Prism-coupling through the microstructured cladding is used to selectively excite individual higher order modes in hollow-core photonic crystal fibers (PCFs). Mode selection is achieved by varying the angle between the incoming beam and the fiber axis, in order to match the axial wavevector component to that of the desired mode. The technique allows accurate measurement of the effective indices and transmission losses of modes of arbitrary order, even those with highly complex transverse field distributions that would be extremely difficult to excite by conventional endfire coupling.

Manipulation of coherent Stokes light by transient stimulated Raman scattering in gas filled hollow-core PCF.

Transient stimulated Raman scattering is investigated in methane-filled hollow-core photonic crystal fiber. Using frequency-chirped ps-pulses at 1.06 microm as pump and tunable CW-radiation as Stokes seed, the vibrational excitation of the CH(4) molecules can be controlled on the sub T(2) time-scale.