A general scheme to get insight and to control postcollision interaction (PCI) by means of sequential double ionization with two high-frequency pulses is discussed. In particular, we propose to consider PCI of a slow photoelectron released by the pump pulse from a neutral atom with a fast photoelectron released by the time-delayed probe pulse from the created ion. This scheme is exemplified by the ab initio calculations performed for the prototypical helium atom.
View Article and Find Full Text PDFA unified view on linear response of interacting systems utilizing multiconfigurational time-dependent Hartree methods is presented. The cases of one-particle and two-particle response operators for identical particles and up to all-system response operators for distinguishable degrees-of-freedom are considered. The working equations for systems of identical bosons and identical fermions, as well for systems of distinguishable particles are explicitly derived.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
August 2012
The tunneling process in a many-body system is a phenomenon which lies at the very heart of quantum mechanics. It appears in nature in the form of α-decay, fusion and fission in nuclear physics, and photoassociation and photodissociation in biology and chemistry. A detailed theoretical description of the decay process in these systems is a very cumbersome problem, either because of very complicated or even unknown interparticle interactions or due to a large number of constituent particles.
View Article and Find Full Text PDFExperiments on ultracold attractive Bose-Einstein condensates (BECs) have demonstrated that at low dimensions atomic clouds can form localized objects, propagating for long times without significant changes in their shapes and attributed to bright matter-wave solitons, which are coherent objects. We consider the dynamics of bright soliton trains from the perspective of many-boson physics. The fate of matter-wave soliton trains is actually to quickly lose their coherence and become macroscopically fragmented BECs.
View Article and Find Full Text PDFThe quantum dynamics of a one-dimensional bosonic Josephson junction is studied by solving the time-dependent many-boson Schrödinger equation numerically exactly. Already for weak interparticle interactions and on short time scales, the commonly employed mean-field and many-body methods are found to deviate substantially from the exact dynamics. The system exhibits rich many-body dynamics such as enhanced tunneling and a novel equilibration phenomenon of the junction depending on the interaction, which is attributed to a quick loss of coherence.
View Article and Find Full Text PDFThe dynamics of attractive ultracold bosonic clouds in one dimension is studied by solving the many-particle time-dependent Schrödinger equation. The initially coherent wave packet can dynamically dissociate into two parts when its energy exceeds a threshold value. Noticeably, the time-dependent Gross-Pitaevskii theory does not show up the splitting.
View Article and Find Full Text PDFIt is well known that attractive condensates do not posses a stable ground state in three dimensions. The widely used Gross-Pitaevskii theory predicts the existence of metastable states up to some critical number N(cr)(GP) of atoms. It is demonstrated here that fragmented metastable states exist for atom numbers well above N(cr)(GP).
View Article and Find Full Text PDFWe show that the successful and formally exact multiconfigurational time-dependent Hartree method (MCTDH) takes on a unified and compact form when specified for systems of identical particles (MCTDHF for fermions MCTDHB for bosons). In particular the equations of motion for the orbitals depend explicitly and solely on the reduced one- and two-body density matrices of the system's many-particle wave function. We point out that this appealing representation of the equations of motion opens up further possibilities for approximate propagation schemes.
View Article and Find Full Text PDFAn essentially exact approach to compute the wave function in the time-dependent many-boson Schrödinger equation is derived and employed to study accurately the process of splitting a trapped condensate. As the trap transforms from a single to double well the ground state changes from a coherent to a fragmented state. We follow the role played by many-body excited states during the splitting process.
View Article and Find Full Text PDFThe density of two initially independent condensates which are allowed to expand and overlap can show interferences as a function of time due to interparticle interaction. Two situations are separately discussed and compared: (1) all atoms are identical and (2) each condensate consists of a different kind of atoms. Illustrative examples are presented.
View Article and Find Full Text PDFMixtures of cold bosonic atoms in optical lattices undergo demixing on different length scales with increasing interspecies repulsion. As a general rule, the stronger the intraspecies interactions, the shorter is this length scale. The wealth of phenomena is documented by illustrative examples on both superfluids and Mott insulators.
View Article and Find Full Text PDFQuantum phases and phase transitions of weakly to strongly interacting bosonic atoms in deep to shallow optical lattices are described by a single multiorbital mean-field approach in real space. For weakly interacting bosons in one dimension, the critical value of the superfluid to Mott insulator (MI) transition found is in excellent agreement with many-body treatments of the Bose-Hubbard model. For strongly interacting bosons, (i) additional MI phases appear, for which two (or more) atoms residing in each site undergo a Tonks-Girardeau-like transition and localize, and (ii) on-site excitation becomes the excitation lowest in energy.
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