Chiral hybrid metal-halide semiconductors (MHS) pose as ideal candidates for spintronic applications owing to their strong spin-orbit coupling (SOC), and long spin relaxation times. Shedding light on the underlying structure-property relationships is of paramount importance for the targeted synthesis of materials with an optimum performance. Herein, we report the synthesis and optical properties of 1D chiral (-/-THBTD)SbBr (THBTD = 4,5,6,7-tetrahydro-benzothiazole-2,6-diamine) semiconductors using a multifunctional ligand as a countercation and a structure directing agent.
View Article and Find Full Text PDFThe large number of spatial modes supported by standard multimode fibers is a promising platform for boosting the channel capacity of quantum and classical communications by orders of magnitude. However, the practical use of long multimode fibers is severely hampered by modal crosstalk and polarization mixing. To overcome these challenges, we develop and experimentally demonstrate a vectorial time reversal technique, which is accomplished by digitally pre-shaping the wavefront and polarization of the forward-propagating signal beam to be the phase conjugate of an auxiliary, backward-propagating probe beam.
View Article and Find Full Text PDFFree-space optical communication is a promising means to establish versatile, secure and high-bandwidth communication between mobile nodes for many critical applications. While the spatial modes of light offer a degree of freedom to increase the information capacity of an optical link, atmospheric turbulence can introduce severe distortion to the spatial modes and lead to data degradation. Here, we demonstrate experimentally a vector-beam-based, turbulence-resilient communication protocol, namely spatial polarization differential phase shift keying (SPDPSK), that can reliably transmit high-dimensional information through a turbulent channel without the need of any adaptive optics for beam compensation.
View Article and Find Full Text PDFIn this paper we propose a graphene-based metasurface structure that can exhibit tunable electromagnetically-induced-transparency-like (EIT) spectral response at mid-infrared frequencies. The metasurface structure is composed of two subwavelength mono-layer graphene nano-disks coupled with a mono-layer graphene nano-strip. We show that the coupling of the nano-disks' dipole resonance with the quadrupole resonance of the nano-strip can create two split resonances with a transparency window in between at any desired center frequency within a wide frequency range.
View Article and Find Full Text PDF