As the trajectory toward the graphene era continues, there is a compelling need to harness 2D technology further for the transformation of three-dimensional (3D) materials production and applications. Here, we resolve this challenge for one of the most widely utilized 3D materials in modern electronics─gold─using graphene-inspired fabrication technology that allows us to develop a multistep production method of ultrathin gold films. Such films demonstrate continuous morphology, low sheet resistance (10 Ω/sq), and high transparency (80%), offering opportunities in a variety of technological and scientific sectors.
View Article and Find Full Text PDFThe lattice geometry of natural materials and the structural geometry of artificial materials are crucial factors determining their physical properties. Most materials have predetermined geometries that lead to fixed physical characteristics. Here, the demonstration of a carbon nanotube network serves as an example of a system with controllable orientation achieving on-demand optical properties.
View Article and Find Full Text PDFThe emergence of van der Waals (vdW) materials resulted in the discovery of their high optical, mechanical, and electronic anisotropic properties, immediately enabling countless novel phenomena and applications. Such success inspired an intensive search for the highest possible anisotropic properties among vdW materials. Furthermore, the identification of the most promising among the huge family of vdW materials is a challenging quest requiring innovative approaches.
View Article and Find Full Text PDFNature is abundant in material platforms with anisotropic permittivities arising from symmetry reduction that feature a variety of extraordinary optical effects. Principal optical axes are essential characteristics for these effects that define light-matter interaction. Their orientation - an orthogonal Cartesian basis that diagonalizes the permittivity tensor, is often assumed stationary.
View Article and Find Full Text PDFDynamicallyprogrammable metasurfaces capable of manipulating terahertz (THz) wavefronts in various manners depending on external controls are highly desired for next-generation wireless communication systems and new tools for THz diagnostics. Such metasurfaces may utilize the insulator-to-metal transition in , which can be induced both electrically and optically. Optical control is especially convenient for individual addressing to each meta-atom, but it is hampered by the high optical switching threshold of .
View Article and Find Full Text PDFNanomaterials (Basel)
April 2023
During the last years, giant optical anisotropy has demonstrated its paramount importance for light manipulation. In spite of recent advances in the field, the achievement of continuous tunability of optical anisotropy remains an outstanding challenge. Here, we present a solution to the problem through the chemical alteration of halogen atoms in single-crystal halide perovskites.
View Article and Find Full Text PDFVan der Waals (vdW) heterostructures pave the way to achieve the desired material properties for a variety of applications. In this way, new scientific and industrial challenges and fundamental questions arise. One of them is whether vdW materials preserve their original optical response when assembled in a heterostructure.
View Article and Find Full Text PDFSnS and SnSe have recently been shown to have a wide range of applications in photonic and optoelectronic devices. However, because of incomplete knowledge about their optical characteristics, the use of SnS and SnSe in optical engineering remains challenging. Here, we addressed this problem by establishing SnS and SnSe linear and nonlinear optical properties in the broad (300-3300 nm) spectral range.
View Article and Find Full Text PDFNoble transition metal dichalcogenides (TMDCs) such as PtS and PtSe show significant potential in a wide range of optoelectronic and photonic applications. Noble TMDCs, unlike standard TMDCs such as MoS and WS, operate in the ultrawide spectral range from ultraviolet to mid-infrared wavelengths; however, their properties remain largely unexplored. Here, we measured the broadband (245-3300 nm) optical constants of ultrathin PtS and PtSe films to eliminate this gap and provide a foundation for optoelectronic device simulation.
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