Superconductors play a crucial role in the advancement of high-field electromagnets. Unfortunately, their performance can be compromised by thermomagnetic instabilities, wherein the interplay of rapid magnetic and slow heat diffusion can result in catastrophic flux jumps, eventually leading to irreversible damage. This issue has long plagued high-J NbSn wires at the core of high-field magnets.
View Article and Find Full Text PDFIn the pursuit of advancing spin-wave optics, the propagation of magnetostatic surface spin-waves is investigated in a uniform permalloy waveguide with in-situ nanopatterned grooves created through Atomic Force Microscopy nanolithography and Focused Ion Beam etching. The study unveils that the introduction of narrow constrictions and grooves leads to a non-monotonic reduction of the transmitted spin-wave signal intensity as the spin-wave pathway is shrinked. The remarkable feature that a stronger signal extinction is obtained for a narrow groove compared to a spin-waveguide interrupted by a full gap, where only inefficient transport through dipolar coupling is allowed, is highlighted.
View Article and Find Full Text PDFThe energy landscape of multiply connected superconducting structures is ruled by fluxoid quantization due to the implied single-valuedness of the complex wave function. The transitions and interaction between these energy states, each defined by a specific phase winding number, are governed by classical and/or quantum phase slips. Understanding these events requires the ability to probe, noninvasively, the state of the ring.
View Article and Find Full Text PDFJ Colloid Interface Sci
November 2024
Hypothesis: Metallic nanowires, particularly polyol-grown silver nanowires, exhibit a morphological instability at temperatures significantly lower than their bulk melting point. This instability is commonly named after Rayleigh's description of the morphological instability of liquid jets, even though it has been shown that its quantitative predictions are not consistent with experimental measurements. In 1996, McCallum et al.
View Article and Find Full Text PDFAgainst the background of the current healthcare and climate emergencies, surface enhanced Raman scattering (SERS) is becoming a highly topical technique for identifying and fingerprinting molecules, e.g., within viruses, bacteria, drugs, and atmospheric aerosols.
View Article and Find Full Text PDFThe adsorption and desorption kinetics of molecules is of significant fundamental and applied interest. In this paper, we present a new method to quantify the energy barriers for the adsorption and desorption of gas molecules on few-atom clusters, by exploiting reaction induced changes of the doping level of a graphene substrate. The method is illustrated for oxygen adsorption on Au clusters.
View Article and Find Full Text PDFIn a multi-branch metallic interconnect we demonstrate the possibility to induce targeted modifications of the material properties by properly selecting the intensity and polarity of the applied current. We illustrate this effect in Y-shape multiterminal devices made of Nb on sapphire for which we show that the superconducting critical current can be lowered in a controlled manner at a preselected junction. We further observe the gradual appearance of Fraunhofer-like critical current oscillations with magnetic field which indicates the gradual modification of a superconducting weak link.
View Article and Find Full Text PDFManipulating the superconducting states of high transition temperature (high-T) cuprate superconductors in an efficient and reliable way is of great importance for their applications in next-generation electronics. Here, employing ionic liquid gating, a selective control of volatile and non-volatile superconductivity is achieved in pristine insulating PrCuO (PCO) films, based on two distinct mechanisms. Firstly, with positive electric fields, the film can be reversibly switched between superconducting and non-superconducting states, attributed to the carrier doping effect.
View Article and Find Full Text PDFThe past years have witnessed major advancements in all-electrical doping control on cuprates. In the vast majority of cases, the tuning of charge carrier density has been achieved electric field effect by means of either a ferroelectric polarization or using a dielectric or electrolyte gating. Unfortunately, these approaches are constrained to rather thin superconducting layers and require large electric fields in order to ensure sizable carrier modulations.
View Article and Find Full Text PDFBacterial infections are one of the leading causes of disease worldwide. Conventional antibiotics are becoming less efficient, due to antibiotic-resistant bacterial strains. Therefore, the development of novel antibacterial materials and advanced treatment strategies are becoming increasingly important.
View Article and Find Full Text PDFWe report on metal-assisted chemical etching of Si for the synthesis of mechanically stable, hybrid crystallographic orientation Si superstructures with high aspect ratio, above 200. This method sustains high etching rates and facilitates reproducible results. The protocol enables the control of the number, angle, and location of the kinks via successive etch-quench sequences.
View Article and Find Full Text PDFAs the most sensitive magnetic field sensor, the superconducting quantum interference device (SQUID) became an essential component in many applications due to its unmatched performance. Through recently achieved miniaturization, using state-of-the-art fabrication methods, this fascinating device extended its functionality and became an important tool in nanomaterial characterization. Here, we present an accessible and yet powerful technique of targeted atom displacement in order to reduce the size of the weak links of a DC nano-SQUID beyond the limits of conventional lithography.
View Article and Find Full Text PDFElectromigration has evolved from an important cause of failure in electronic devices to an appealing method, capable of modifying the material properties and geometry of nanodevices. Although this technique has been successfully used by researchers to investigate low dimensional systems and nanoscale objects, its low controllability remains a serious limitation. This is in part due to the inherent stochastic nature of the process, but also due to the inappropriate identification of the relevant control parameters.
View Article and Find Full Text PDFWe demonstrate the in situ engineering of superconducting nanocircuitry by targeted modulation of material properties through high applied current densities. We show that the sequential repetition of such customized electro-annealing in a niobium (Nb) nanoconstriction can broadly tune the superconducting critical temperature T and the normal-state resistance R in the targeted area. Once a sizable R is reached, clear magneto-resistance oscillations are detected along with a Fraunhofer-like field dependence of the critical current, indicating the formation of a weak link but with further adjustable characteristics.
View Article and Find Full Text PDFThe electromigration process has the potential capability to move atoms one by one when properly controlled. It is therefore an appealing tool to tune the cross section of monoatomic compounds with ultimate resolution or, in the case of polyatomic compounds, to change the stoichiometry with the same atomic precision. As demonstrated here, a combination of electromigration and anti-electromigration can be used to reversibly displace atoms with a high degree of control.
View Article and Find Full Text PDFThe main dissipation mechanism in superconducting nanowires arises from phase slips. Thus far, most of the studies focus on long nanowires where coexisting events appear randomly along the nanowire. In the present work we investigate highly confined phase slips at the contact point of two superconducting leads.
View Article and Find Full Text PDFLocal polarization of a magnetic layer, a well-known method for storing information, has found its place in numerous applications such as the popular magnetic drawing board toy or the widespread credit cards and computer hard drives. Here we experimentally show that a similar principle can be applied for imprinting the trajectory of quantum units of flux (vortices), travelling in a superconducting film (Nb), into a soft magnetic layer of permalloy (Py). In full analogy with the magnetic drawing board, vortices act as tiny magnetic scribers leaving a wake of polarized magnetic media in the Py board.
View Article and Find Full Text PDFSuperconducting nanowires currently attract great interest due to their application in single-photon detectors and quantum-computing circuits. In this context, it is of fundamental importance to understand the detrimental fluctuations of the superconducting order parameter as the wire width shrinks. In this paper, we use controlled electromigration to narrow down aluminium nanoconstrictions.
View Article and Find Full Text PDFThe response of superconducting devices to electromagnetic radiation is a core concept implemented in diverse applications, ranging from the currently used voltage standard to single photon detectors in astronomy. Suprisingly, a sufficiently high power subgap radiation may stimulate superconductivity itself. The possibility of stimulating type II superconductors, in which the radiation may interact also with vortex cores, remains however unclear.
View Article and Find Full Text PDFThe design of many promising, newly emerging classes of photonic metamaterials and subwavelength confinement structures requires detailed knowledge and understanding of the electromagnetic near-field interactions between their building blocks. While the electric field distributions and, respectively, the electric interactions of different nanostructures can be routinely measured, for example, by scattering near-field microscopy, only recently experimental methods for imaging the magnetic field distributions became available. In this paper, we provide direct experimental maps of the lateral magnetic near-field distributions of variously shaped plasmonic nanoantennas by using hollow-pyramid aperture scanning near-field optical microscopy (SNOM).
View Article and Find Full Text PDFFollowing the impact of a single femtosecond light pulse on nickel nanostripes, material deformations-or "nanobumps"-are created. We have studied the dependence of these nanobumps on the length of nanostripes and verified the link with plasmons. More specifically, local electric currents can melt the nanostructures in the hotspots, where hydrodynamic processes give rise to nanobumps.
View Article and Find Full Text PDFWe present direct experimental mapping of the lateral magnetic near-field distribution in plasmonic nanoantennas using aperture scanning near-field optical microscopy (SNOM). By means of full-field simulations it is demonstrated how the coupling of the hollow-pyramid aperture probe to the nanoantenna induces an effective magnetic dipole which efficiently excites surface plasmon resonances only at lateral magnetic field maxima. This excitation in turn affects the detected light intensity enabling the visualization of the lateral magnetic near-field distribution of multiple odd and even order plasmon modes with subwavelength spatial resolution.
View Article and Find Full Text PDFIn response to the incident light's electric field, the electron density oscillates in the plasmonic hotspots producing an electric current. Associated Ohmic losses raise the temperature of the material within the plasmonic hotspot above the melting point. A nanojet and nanosphere ejection can then be observed precisely from the plasmonic hotspots.
View Article and Find Full Text PDFWe have applied the surface-sensitive nonlinear optical technique of magnetization-induced second harmonic generation (MSHG) to plasmonic, magnetic nanostructures made of Ni. We show that surface plasmon contributions to the MSHG signal can reveal the direction of the magnetization. Both the plasmonic and the magnetic nonlinear optical responses can be tuned; our results indicate novel ways to combine nanophotonics, nanoelectronics, and nanomagnetics and suggest the possibility for large magneto-chiral effects in metamaterials.
View Article and Find Full Text PDF