The radioisotope thorium-229 (Th) is renowned for its extraordinarily low-energy, long-lived nuclear first-excited state. This isomeric state can be excited by vacuum ultraviolet (VUV) lasers and Th has been proposed as a reference transition for ultra-precise nuclear clocks. To assess the feasibility and performance of the nuclear clock concept, time-controlled excitation and depopulation of the Th isomer are imperative.
View Article and Find Full Text PDFThis paper presents an absolute X-ray photon energy measurement method that uses a Bond diffractometer. The proposed system enables the prompt and rapid in situ measurement of photon energies over a wide energy range. The diffractometer uses a reference silicon single-crystal plate and a highly accurate angle encoder called SelfA.
View Article and Find Full Text PDFWe report the observation of two-photon emission from a coherently excited vibrational state of solid parahydrogen, which is also a known quantum solid. Coherence between the ground and the excited states is prepared by stimulated Raman scattering using two visible laser pulses. The two-photon emission is triggered by another mid-infrared laser pulse.
View Article and Find Full Text PDFThe coherence decay of the v = 2 vibrational state (vibrons) of solid parahydrogen was measured via time-resolved coherent anti-Stokes Raman spectroscopy. We found that the decay curve has a non-exponential time profile in the time scale of 200 ns at a low temperature below 5 K and a low orthohydrogen impurity concentration (~0.01%).
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